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arXiv:2303.13498 · Physical review. B./Physical review. B

Sign structure of the t − t ′ − J model and its physical consequences

Xin Lu, Jiaxin Zhang, Shou-Shu Gong, D. N. Sheng, Zheng-Yu Weng

Published Oct 10, 2024• 15 citations
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Abstract

Understanding the doped Mott insulator is a central challenge in condensed matter physics. In this work, we first explicitly identify a new sign structure in the $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model on the square lattice that replaces the conventional Fermi statistics for weakly interacting electrons. Then we show that the singular, i.e., the phase-string part of the sign structure in the partition function can be precisely turned off in a modified model. The density matrix renormalization group method is then employed to study these two models comparatively on finite-size systems, which is designed to unveil the consequences of the phase-string component. We find that the hole pairing is present not only in the quasi-long-range superconducting phase but also in the stripe phase of the $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model. However, once the phase-string is switched off, both the superconducting and stripe orders together with the underlying hole pairing disappear. The corresponding ground state reduces to a trivial Fermi-liquid-like state with small hole Fermi pockets that is decoupled from the antiferromagnetic spin background. It is in sharp contrast to the original $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model where large Fermi surfaces can be restored in the stripe phase found at ${t}^{\ensuremath{'}}/t<0$ or the superconducting phase at ${t}^{\ensuremath{'}}/t>0$ in the six-leg ladder calculation. Our study clearly demonstrates that the strong correlation effect in doped Mott insulator should be mainly attributed to the long-range quantum entanglement between the spin and charge, which is, nonperturbatively, beyond a simple spin-charge separation under the no double occupancy constraint.

DOI
10.1103/physrevb.110.165127

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Understanding the doped Mott insulator is a central challenge in condensed matter physics. In this work, we first explicitly identify a new sign structure in the t\ensuremath-t\ensuremath′\ensuremath-Jt\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}Jt\ensuremath-t\ensuremath′\ensuremath-J model on the square lattice that replaces the conventional Fermi statistics for weakly interacting electrons. Then we show that the singular, i.e., the phase-string part of the sign structure in the partition function can be precisely turned off in a modified model. The density matrix renormalization group method is then employed to study these two models comparatively on finite-size systems, which is designed to unveil the consequences of the phase-string component. We find that the hole pairing is present not only in the quasi-long-range superconducting phase but also in the stripe phase of the t\ensuremath-t\ensuremath′\ensuremath-Jt\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}Jt\ensuremath-t\ensuremath′\ensuremath-J model. However, once the phase-string is switched off, both the superconducting and stripe orders together with the underlying hole pairing disappear. The corresponding ground state reduces to a trivial Fermi-liquid-like state with small hole Fermi pockets that is decoupled from the antiferromagnetic spin background. It is in sharp contrast to the original t\ensuremath-t\ensuremath′\ensuremath-Jt\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}Jt\ensuremath-t\ensuremath′\ensuremath-J model where large Fermi surfaces can be restored in the stripe phase found at t\ensuremath′/t<0{t}^{\ensuremath{'}}/t<0t\ensuremath′/t<0 or the superconducting phase at t\ensuremath′/t>0{t}^{\ensuremath{'}}/t>0t\ensuremath′/t>0 in the six-leg ladder calculation. Our study clearly demonstrates that the strong correlation effect in doped Mott insulator should be mainly attributed to the long-range quantum entanglement between the spin and charge, which is, nonperturbatively, beyond a simple spin-charge separation under the no double occupancy constraint.
We apply the fermionic tensor network (TN) state method to understand the strongly correlated nature in a doped Mott insulator. We conduct a comparative study of the $\ensuremath{\sigma}t\text{\ensuremath{-}}J$ model, in which the no-double-occupancy constraint remains unchanged but the quantum phase string effect associated with doped holes is precisely switched off. Thus, the ground state of the $\ensuremath{\sigma}t\text{\ensuremath{-}}J$ model can serve as a well-controlled reference state of the standard $t\text{\ensuremath{-}}J$ model. In the absence of the phase string, the spin long-range antiferromagnetic (AFM) order is found to be essentially decoupled from the doped holes, and the latter contribute to a Fermi-liquid-like compressibility and a coherent single-particle propagation with a markedly reduced pairing tendency. In contrast, our TN calculations of the $t\text{\ensuremath{-}}J$ model indicate that the AFM order decreases much faster with doping and the single-particle propagation of doped holes gets substantially suppressed, concurrently with a much stronger charge compressibility at small doping and significantly amplified Cooper pairing tendencies. These findings demonstrate that quantum many-body interference from phase strings plays a pivotal role in the $t\text{\ensuremath{-}}J$ model, mediating long-range entanglement between spin and charge degrees of freedom, which might hold the key mechanism for high-Tc{T}_{c}Tc​ cuprates.
The mechanism of superconductivity in a purely interacting electron system has been one of the most challenging issues in condensed matter physics. In the BCS theory, the Landau's Fermi liquid is the ground state of weakly interacting fermions dictated by the fermion sign structure, and the superconducting instability only occurs when an additional pairing force is added. By contrast, as shown by density matrix renormalization group calculation, a quasi-one-dimensional superconducting state (specifically a Luther-Emery state) is an intrinsic ground state of the $t\ensuremath{-}J$ two-leg ladder and four-leg cylinder at finite doping. Such a Luther-Emery state with pairing can be directly turned into a Fermi-gas-like normal state without pairing by merely switching off the phase-string signs hidden in the model via two schemes, which reduce the sign structure to the trivial fermion signs associated with doped holes. It thus demonstrates a new pairing paradigm in a model-doped Mott insulator as due to the generic phase-string sign structure. Finally, as an example, the latter is explicitly shown to lead to a ``stringlike'' pairing force after adiabatically connecting to a strong anisotropic limit of the model.
Unravelling competing orders emergent in doped Mott insulators and their interplay with unconventional superconductivity is one of the major challenges in condensed matter physics. To explore the possible superconducting state in a doped Mott insulator, we study the square-lattice t-J model with both the nearest-neighbor and next-nearest-neighbor electron hoppings and spin interactions. By using the state-of-the-art density matrix renormalization group calculation with imposing charge U(1) and spin SU(2) symmetries on the six-leg cylinders, we establish a quantum phase diagram including three phases: a stripe charge density wave phase, a superconducting phase without static charge order, and a superconducting phase coexistent with a weak charge stripe order. Crucially, we demonstrate that the superconducting phase has a power-law pairing correlation that decays much slower than the charge density and spin correlations, which is a quasi-1D descendant of the uniform d-wave superconductor in two dimensions. These findings reveal that enhanced charge and spin fluctuations with optimal doping is able to produce robust d-wave superconductivity in doped Mott insulators, providing a foundation for connecting theories of superconductivity to models of strongly correlated systems.
Cooper pairing instability in a Fermi liquid is well understood by the BCS theory, but pairing mechanism for doped Mott insulators still remains elusive. Previously it has been shown by density matrix renormalization group (DMRG) method that a single doped hole is always self-localized due to the quantum destructive interference of the phase string signs hidden in the t-J ladders. Here we report a DMRG investigation of hole binding in the same model, where a novel pairing-glue scheme beyond the BCS realm is discovered. Specifically, we show that, in addition to spin pairing due to superexchange interaction, the strong frustration of the phase string signs on the kinetic energy gets effectively removed by pairing the charges, which results in strong binding of two holes. By contrast, if the phase string signs are "switched off" artificially, the pairing strength diminishes significantly even if the superexchange coupling remains the same. In the latter, unpaired holes behave like coherent quasiparticles with pairing drastically weakened, whose sole origin may be attributed to the resonating-valence-bond (RVB) pairing of spins. Such non-BCS pairing mechanism is therefore beyond the RVB picture and may shed important light on the high-T(c) cuprate superconductors.
We report results of large-scale ground-state density matrix renormalization group (DMRG) calculations on t-[Formula: see text]-J cylinders with circumferences 6 and 8. We determine a rough phase diagram that appears to approximate the two-dimensional (2D) system. While for many properties, positive and negative [Formula: see text] values ([Formula: see text]) appear to correspond to electron- and hole-doped cuprate systems, respectively, the behavior of superconductivity itself shows an inconsistency between the model and the materials. The [Formula: see text] (hole-doped) region shows antiferromagnetism limited to very low doping, stripes more generally, and the familiar Fermi surface of the hole-doped cuprates. However, we find [Formula: see text] strongly suppresses superconductivity. The [Formula: see text] (electron-doped) region shows the expected circular Fermi pocket of holes around the [Formula: see text] point and a broad low-doped region of coexisting antiferromagnetism and d-wave pairing with a triplet p component at wavevector [Formula: see text] induced by the antiferromagnetism and d-wave pairing. The pairing for the electron low-doped system with [Formula: see text] is strong and unambiguous in the DMRG simulations. At larger doping another broad region with stripes in addition to weaker d-wave pairing and striped p-wave pairing appears. In a small doping region near [Formula: see text] for [Formula: see text], we find an unconventional type of stripe involving unpaired holes located predominantly on chains spaced three lattice spacings apart. The undoped two-leg ladder regions in between mimic the short-ranged spin correlations seen in two-leg Heisenberg ladders.
How the ground-state nature can be dramatically changed by the distinct underlying spin correlation is a central issue of doped Mott insulators.The two-leg XXZ ladder provides a prototypical spin background, which can be tuned from a long-range Néel order to a short-range spin liquid via the superexchange anisotropy, giving rise to a complex phase diagram at finite doping.By density matrix renormalization group method, we show that although the charge is always self-localized in the Néel ordered phase, a second insulating phase emerges in which the doped holes become paired but remain localized while the transverse spin-spin correlation reduces to short-ranged one to make the Néel order classical.Only when the Néel order totally disappears by further reducing anisotropy does the pairing become truly coherent as characterized by a Luther-Emery state.In sharp contrast, the pairing is totally absent in the in-plane ferromagnetic XXZ regime, where a direct transition from the charge self-localization in the Néel ordered phase to a Fermi-gas-like state in the spin liquid phase is found.A consistent physical picture is briefly discussed.