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arXiv:1908.00312 · Physical review. B./Physical review. B

Microscopic model for magnetoelectric coupling through lattice distortions

D. C. Cabra, A. Dobry, C. J. Gazza, G. L. Rossini

Published Oct 28, 2019• 7 citations
arXivHTMLPDF

Abstract

We propose a microscopic magnetoelectric model in which the coupling between spins and electric dipoles is mediated by lattice distortions. The magnetic sector is described by a spin $S=1/2$ Heisenberg model coupled directly to the lattice via a standard spin-Peierls term and indirectly to the electric dipole variables via the distortion of the surrounding electronic clouds. Electric dipoles are described by Ising variables for simplicity. We show that the effective magnetoelectric coupling which arises due to the interconnecting lattice deformations is quite efficient in one-dimensional arrays. More precisely, we show using bosonization and extensive density matrix renormalization group numerical simulations that increasing the magnetic field above the spin-Peierls gap, a massive polarization switch-off occurs due to the proliferation of soliton pairs. We also analyze the effect of an external electric field when the magnetic system is in a gapped (plateau) phase and show that the magnetization can be electrically switched between clearly distinct values. More general quasi-one-dimensional models and two-dimensional systems are also discussed.

DOI
10.1103/physrevb.100.161111

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We propose a microscopic magnetoelectric model in which the coupling between spins and electric dipoles is mediated by lattice distortions. The magnetic sector is described by a spin S=1/2S=1/2S=1/2 Heisenberg model coupled directly to the lattice via a standard spin-Peierls term and indirectly to the electric dipole variables via the distortion of the surrounding electronic clouds. Electric dipoles are described by Ising variables for simplicity. We show that the effective magnetoelectric coupling which arises due to the interconnecting lattice deformations is quite efficient in one-dimensional arrays. More precisely, we show using bosonization and extensive density matrix renormalization group numerical simulations that increasing the magnetic field above the spin-Peierls gap, a massive polarization switch-off occurs due to the proliferation of soliton pairs. We also analyze the effect of an external electric field when the magnetic system is in a gapped (plateau) phase and show that the magnetization can be electrically switched between clearly distinct values. More general quasi-one-dimensional models and two-dimensional systems are also discussed.
We present a novel mechanism for the appearance of magnetization plateaus in quasi-one-dimensional quantum spin systems, which is induced by the coupling to the underlying lattice. We investigate in detail a simple model of a frustrated spin-1/2 Heisenberg chain coupled to adiabatic phonons under an external magnetic field, but the present mechanism is expected to be more general. Using field theoretic methods complemented by extensive density matrix renormalization group techniques, we show that magnetization plateaus at nontrivial rational values of the magnetization can be stabilized by the lattice coupling. We suggest that such a scenario could be relevant for some low dimensional frustrated spin-Peierls compounds.
Effects of spin-Peierls fluctuation are examined in models of one-dimensional conductors. One-dimensional strongly correlated systems coupled to dynamical lattice distortion or polarization are examined by quantum Monte Carlo studies. Excitations are given by spinless charge solitons and neutral spin solitons when the system is doped away from a Mott insulator. A pairing mechanism due to a dynamical spin-Peierls fluctuation is discussed. Numerical results on the spin gap formation and the enhancement of pairing correlations in a dimerized t-J model and doped spin-1 Heisenberg model in one dimension are summarized.
We study the interplay of electric and magnetic order in the one-dimensional Heisenberg spin-12\frac{1}{2}21​ XXZ chain with large Ising anisotropy in the presence of the Dzyaloshinskii-Moriya (DM) interaction and with longitudinal and transverse magnetic fields, interpreting the DM interaction as a coupling between the local electric polarization and an external electric field. We obtain the ground state phase diagram using the density matrix renormalization group method and compute various ground state quantities like the magnetization, staggered magnetization, electric polarization and spin correlation functions, etc. In the presence of both longitudinal and transverse magnetic fields, there are three different phases corresponding to a gapped N\'eel phase with antiferromagnetic (AF) order, gapped saturated phase, and a critical incommensurate gapless phase. The external electric field modifies the phase boundaries but does not lead to any new phases. Both external magnetic fields and electric fields can be used to tune between the phases. We also show that the transverse magnetic field induces a vector chiral order in the N\'eel phase (even in the absence of an electric field) which can be interpreted as an electric polarization in a direction parallel to the AF order.
Summary: The interplay of charge, spin and lattice degrees of freedom is studied for quasi-one-dimensional electron and spin systems coupled to quantum phonons. Special emphasis is put on the influence of the lattice dynamics on the Peierls transition. Using exact diagonalization techniques the ground-state and spectral properties of the Holstein model of spinless fermions and of a frustrated Heisenberg model with magneto-elastic coupling are analyzed on finite chains. In the non-adiabatic regime a (T = 0) quantum phase transition from a gapless Luttinger-liquid/spin-fluid state to a gapped dimerized phase occurs at a nonzero critical value of the electron/spin-phonon interaction. To study the nature of the spin-Peierls transition at finite temperatures for the infinite system, an alternative Green’s function approach is applied to the magnetostrictive XY model. With increasing phonon frequency the structure factor shows a remarkable crossover from soft-mode to central-peak behaviour. The results are discussed in relation to recent experiments on CuGeO3. 1
We consider a simple integrable model of a spin chain exhibiting the magnetoelectric effect (MEE). Starting from the periodic S=1/2S=1/2S=1/2 XXZ chain with Dzyaloshinskii-Moriya terms, which we consider as a local electric polarization in the spirit of the Katsura-Nagaosa-Baladsky (KNB) mechanism, we perform the mapping onto the conventional XXZ chain with twisted boundary conditions. Using the techniques of quantum transfer matrix and nonlinear integral equations we obtain the magnetization, electric polarization, and magnetoelectric tensor as functions of magnetic and electric field for arbitrary temperatures. We investigate these dependencies as well as the thermal behavior of the above-mentioned physical quantities, especially in the low-temperature regime. We found several regimes of polarization. Adjusting the magnetic field one can switch the system from one regime to another. The features of the critical properties connected with the MEE are also illustrated.
This thesis demonstrates that arrays of electric dipoles are good analogs for quantum magnets. We center our investigation on a recently developed experiment, in which rubidium-87 atoms are trapped in optical tweezers and then excited into two distinct electronic Rydberg states. The electric dipole-dipole interaction between these Rydberg atoms is mathematically modeled by a spin Hamiltonian with easy-plane anisotropy, and coupling strength decaying as the inverse cube of the distance. We approximately solve for the ground state of this model Hamiltonian on each of the eleven Archimedean lattices, through large-scale density matrix renormalization group calculations. For the kagome lattice, we gather extensive numerical evidence for an emergent quantum spin liquid, similar to that occurring in the canonical Heisenberg model of quantum magnetism. We predict this spin liquid to be of 𝑈(1) Dirac type, and propose new protocols for experimentally preparing and characterizing it. Our theoretical calculations support the collaborative design and analysis of experiments studying dipolar Rydberg atoms in square, circular, and kagome arrays. These respectively result in observations of continuous symmetry breaking, Tomonaga-Luttinger liquid behavior, and an atomic spin liquid candidate.