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arXiv:1907.13592 · Science Advances

Critical slowing down in circuit quantum electrodynamics

Paul Brookes, Giovanna Tancredi, Andrew D. Patterson, Joseph Rahamim, Martina Esposito, Th. K. Mavrogordatos, Peter Leek, Eran Ginossar, Marzena Hanna Szymańska

Published May 19, 2021• 40 citations
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Abstract

Critical slowing down of the time it takes a system to reach equilibrium is a key signature of bistability in dissipative first-order phase transitions. Understanding and characterizing this process can shed light on the underlying many-body dynamics that occur close to such a transition. Here, we explore the rich quantum activation dynamics and the appearance of critical slowing down in an engineered superconducting quantum circuit. Specifically, we investigate the intermediate bistable regime of the generalized Jaynes-Cummings Hamiltonian (GJC), realized by a circuit quantum electrodynamics (cQED) system consisting of a transmon qubit coupled to a microwave cavity. We find a previously unidentified regime of quantum activation in which the critical slowing down reaches saturation and, by comparing our experimental results with a range of models, we shed light on the fundamental role played by the qubit in this regime.

DOI
10.1126/sciadv.abe9492

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Critical slowing down of the time it takes a system to reach equilibrium is a key signature of bistability in dissipative first-order phase transitions. Understanding and characterizing this process can shed light on the underlying many-body dynamics that occur close to such a transition. Here, we explore the rich quantum activation dynamics and the appearance of critical slowing down in an engineered superconducting quantum circuit. Specifically, we investigate the intermediate bistable regime of the generalized Jaynes-Cummings Hamiltonian (GJC), realized by a circuit quantum electrodynamics (cQED) system consisting of a transmon qubit coupled to a microwave cavity. We find a previously unidentified regime of quantum activation in which the critical slowing down reaches saturation and, by comparing our experimental results with a range of models, we shed light on the fundamental role played by the qubit in this regime.
We study the properties of superconducting electrical circuits, realizing cavity quantum electrodynamics. In particular we explore the limit of strong coupling, low dissipation, and elevated temperatures relevant for current and future experiments. We concentrate on the cavity susceptibility as it can be directly experimentally addressed, i.e., as the impedance or the reflection coefficient of the cavity. To this end we investigate the dissipative Jaynes-Cummings model in the strong coupling regime at high temperatures. The dynamics is investigated within the Bloch-Redfield formalism. At low temperatures, when only the few lowest levels are occupied, the susceptibility can be presented as a sum of contributions from independent level-to-level transitions. This corresponds to the secular (random phase) approximation in the Bloch-Redfield formalism. At temperatures comparable to and higher than the oscillator frequency, many transitions become important and a multiple-peak structure appears. We show that in this regime the secular approximation breaks down, as soon as the peaks start to overlap. In other words, the susceptibility is no longer a sum of contributions from independent transitions. We treat the dynamics of the system numerically by exact diagonalization of the Hamiltonian of the qubit plus up to 200 states of the oscillator. We compare the results obtained with and without the secular approximation and find a qualitative discrepancy already at moderate temperatures.
Circuit quantum electrodynamics (cQED), exemplified by a coupled system of a superconducting qubit and a microwave cavity, is a powerful framework for the quantum control and measurement of macroscopic quantum states in solid-state circuits. Quantum circuits based on superconducting qubits have emerged as one of the leading platforms in the pursuit of fault-tolerant quantum computing. Despite significant progress in extending qubit lifetimes, refining experimental protocols, and scaling up quantum processors, errors arising from the control and measurement of superconducting qubits continue to hinder the realization of a universal quantum computer. To investigate the error mechanisms for state-of-the-art qubits, we realize long-lived superconducting transmon qubits that exhibit fluctuating lifetimes, with an average of 0.2 ms and a maximum exceeding 0.4 ms. We then investigate their dominant error mechanism. By introducing novel time-resolved error measurements that are synchronized with the operation of the pulse tube cooler in a dilution refrigerator, we find that mechanical vibrations from the pulse tube induce nonequilibrium dynamics in highly coherent qubits, leading to their correlated bit-flip errors. Our findings not only deepen our understanding of qubit error mechanisms but also provide valuable insights into potential error-mitigation strategies for achieving fault tolerance by decoupling superconducting qubits from their mechanical environments. We also present a novel scheme for operating a cQED system in a regime where the cavity is largely displaced. We find that a qubit drive at the bare cavity frequency can effectively displace the cavity field while minimizing the cavity-drive-induced dephasing and the ac Stark shift. Furthermore, we demonstrate that standard cQED protocols, such as qubit control, readout, and cavity single-photon generation, remain compatible with largely displaced cavity fields, even beyond the critical photon number. These findings open new pathways for exploring cQED dynamics in large-photon-number regimes, including the study of nonlinear phenomena in microwave cavities, the saturation of two-level system baths for extending the coherence of microwave quantum states, and the acceleration of the dispersive readout. Finally, mechanical resonators have emerged as integral components in quantum computing for storing and transducing quantum information. Low-frequency mechanical resonators, with extremely low energy dissipation rates, are particularly interesting for extending the lifetimes of stored quantum information. However, integrating low-frequency mechanical resonators with qubits is challenging because their small energy gaps make coherent energy exchange and ground-state preparation difficult. In this thesis, we report the first steps towards the characterization of a hybrid quantum device, consisting of a Transmon qubit and a circuit optomechanical system, both coupled to a 3D microwave cavity.
Quantum phase transitions play an important role in many-body systems and have been a research focus in conventional condensed-matter physics over the past few decades. Artificial atoms, such as superconducting qubits that can be individually manipulated, provide a new paradigm of realising and exploring quantum phase transitions by engineering an on-chip quantum simulator. Here we demonstrate experimentally the quantum critical behaviour in a highly controllable superconducting circuit, consisting of four qubits coupled to a common resonator mode. By off-resonantly driving the system to renormalize the critical spin-field coupling strength, we have observed a four-qubit nonequilibrium quantum phase transition in a dynamical manner; that is, we sweep the critical coupling strength over time and monitor the four-qubit scaled moments for a signature of a structural change of the system's eigenstates. Our observation of the nonequilibrium quantum phase transition, which is in good agreement with the driven Tavis-Cummings theory under decoherence, offers new experimental approaches towards exploring quantum phase transition-related science, such as scaling behaviours, parity breaking and long-range quantum correlations.
One of the most studied model systems in quantum optics is a two-level atom strongly coupled to a single mode of the electromagnetic field stored in a cavity, a research field named cavity quantum electrodynamics or CQED. CQED has recently received renewed attention due to its implementation with superconducting artificial atoms and coplanar resonators in the so-called circuit quantum electrodynamics (cQED) architecture. In cQED, the couplings can be much stronger than in CQED due to the design flexibility of superconducting circuits and to the enhanced field confinement in one-dimensional cavities. This enabled the realization of fundamental quantum physics and quantum information processing experiments with a degree of control comparable to that obtained in CQED. The purpose of this chapter is to investigate the situation where the resonator to which the atom is coupled is made nonlinear with a Kerr-type nonlinearity, causing its energy levels to be nonequidistant. The system is then described by a nonlinear Jaynes-Cummings Hamiltonian. This considerably enriches the physics since a pumped nonlinear resonator displays bistability, parametric amplification, and squeezing. The interplay of strong coupling and these nonlinear effects constitutes a novel model system for quantum optics that can be implemented experimentally with superconducting circuits. This chapter is organized as follows. In a first section we present the system consisting of a superconducting Kerr nonlinear resonator strongly coupled to a transmon qubit. In the second section, we describe the response of the sole nonlinear resonator to an external drive. In the third section, we show how the resonator bistability can be used to perform a high-fidelity readout of the transmon qubit. In the last section, we investigate the quantum backaction exerted by the intracavity field on the qubit.
We follow the passage from complex amplitude bistability to phase bistability in the driven dissipative Jaynes-Cummings oscillator. Quasi -distribution functions in the steady state are employed, for varying qubit-cavity detuning and drive parameters, in order to track a first-order dissipative quantum phase transition up to the critical point marking a second-order transition and spontaneous symmetry breaking. We demonstrate the photon blockade breakdown in the dispersive regime, and find that the coexistence of cavity states in the regime of quantum bistability is accompanied by pronounced qubit-cavity entanglement. Focusing on the effect of quantum-activated switching for both coupled degrees of freedom, we move from a region of minimal entanglement in the dispersive regime, where we derive analytical perturbative results, to the threshold behaviour of spontaneous dressed-state polarization at resonance.
Abstract Superconducting quantum circuits are a leading platform for quantum-information processing, but their development requires expertise spanning device design, microfabrication, cryogenic operation, microwave control, and quantum characterization. In this work, we report the realization of a flux-tunable superconducting transmon platform and present an integrated workflow encompassing design, fabrication, measurement, and numerical modeling. The device consists of an Al/AlOx/AlAl/AlO_x/AlAl/AlOx​/Al transmon coupled to a three-dimensional microwave cavity operating in the circuit quantum electrodynamics (cQED) dispersive regime. Two-tone spectroscopy reveals a fundamental transition frequency of ω01=5.0122 GHz\omega _{01}=5.0122~\textrm{GHz}ω01​=5.0122 GHz and an anharmonicity of α/2π=−202.4 MHz\alpha /2\pi =-202.4~\textrm{MHz}α/2π=−202.4 MHz , corresponding to EJ/EC≈82.9E_J/E_C \approx 82.9EJ​/EC​≈82.9 . Flux spectroscopy yields a cavity-qubit coupling strength of g/2π=260 MHzg/2\pi = 260~\textrm{MHz}g/2π=260 MHz , while the cavity linewidth gives a loaded quality factor of QL=6127Q_L=6127QL​=6127 and a Purcell limit of T1Purcell≈82 μsT_1^{\textrm{Purcell}}\approx 82~\mu \textrm{s}T1Purcell​≈82 μs . Time-domain measurements yield coherence times of T1=17.4 μsT_1 = 17.4~\mu \textrm{s}T1​=17.4 μs and T2∗=5.8 μsT_2^* = 5.8~\mu \textrm{s}T2∗​=5.8 μs . To investigate coherence and dissipation in the device, the experimental observations are analyzed within a Lindblad master-equation framework describing cavity photon loss and thermal excitation, qubit energy relaxation, and pure dephasing processes. Using a set of experimentally extracted parameters, the model reproduces the measured spectroscopic and time-domain observables, providing a quantitative description of the open-system dynamics of the transmon-cavity platform. The analysis shows that the measured coherence is primarily limited by pure dephasing and energy-relaxation processes, whereas thermal excitation plays a minor role under the experimental conditions. Inspired by the broader framework of quantum dissipation in macroscopic quantum systems pioneered by Caldeira and collaborators, this approach enables a quantitative analysis of relaxation and dephasing processes in superconducting quantum circuits. Beyond the characterization of a single device, the present work demonstrates the establishment of the expertise, infrastructure, and experimental workflow required for the design, fabrication, measurement, and modeling of superconducting quantum circuits, contributing to the development of quantum technologies in Brazil and related applications.