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arXiv:1905.11227 · Physical review. B./Physical review. B

Cavity quantum electrodynamics of strongly correlated electron systems: A no-go theorem for photon condensation

Gian Marcello Andolina, F. M. D. Pellegrino, Vittorio Giovannetti, Allan H. MacDonald, Marco Polini

Published Sep 18, 2019• 144 citations
arXivHTMLPDF

Abstract

In spite of decades of work it has remained unclear whether or not superradiant quantum phases, referred to here as photon condensates, can occur in equilibrium. In this Rapid Communication, we first show that when a nonrelativistic quantum many-body system is coupled to a cavity field, gauge invariance forbids photon condensation. We then present a microscopic theory of the cavity quantum electrodynamics of an extended Falicov-Kimball model, showing that, in agreement with the general theorem, its insulating ferroelectric and exciton condensate phases are not altered by the cavity and do not support photon condensation.

DOI
10.1103/physrevb.100.121109

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In spite of decades of work it has remained unclear whether or not superradiant quantum phases, referred to here as photon condensates, can occur in equilibrium. In this Rapid Communication, we first show that when a nonrelativistic quantum many-body system is coupled to a cavity field, gauge invariance forbids photon condensation. We then present a microscopic theory of the cavity quantum electrodynamics of an extended Falicov-Kimball model, showing that, in agreement with the general theorem, its insulating ferroelectric and exciton condensate phases are not altered by the cavity and do not support photon condensation.
Equilibrium phase transitions between a normal and a photon condensate state (also known as superradiant phase transitions) are a highly debated research topic, where proposals for their occurrence and no-go theorems have chased each other for the past four decades. Previous no-go theorems have demonstrated that gauge invariance forbids second-order phase transitions to a photon condensate state when the cavity-photon mode is assumed to be spatially uniform. First-order phase transitions were previously considered as possible paths to bypass the no-go theorem. In particular, it has been theoretically predicted that a collection of three-level systems coupled to light can display a first-order phase transition to a photon condensate state. Here, we lay down a general no-go theorem, which forbids first-order as well as second-order superradiant phase transitions in a spatially-uniform cavity field. By using the tools of lattice gauge theory, we then derive a fully gauge-invariant model for three-level systems coupled to light. In agreement with the general theorem, our model does not display photon condensation.
Whether or not superradiant phase transitions (photon condensates) can occur in equilibrium systems is a long-debated open question. The realization of photon condensation in a spatially uniform cavity field is forbidden by a ``no-go'' theorem stemming from gauge invariance. Here, bypassing the theorem by considering a spatially varying electromagnetic field, the authors derive a series of criteria for the occurrence of photon condensation. The cases of both three-dimensional and two-dimensional electronic systems are analyzed. This work paves the way for the realization of equilibrium photon condensation in solid-state systems.
The possibility of a superradiant phase transition in light-matter systems is the subject of much debate, due to numerous apparently conflicting no-go and counter no-go theorems. Using an arbitrary-gauge approach we show that a unique phase transition does occur in archetypal many-dipole cavity QED systems, and that it manifests unambiguously via a macroscopic gauge-invariant polarization. We find that the gauge choice controls the extent to which this polarization is included as part of the radiative quantum subsystem and thereby determines the degree to which the abnormal phase is classed as superradiant. This resolves the long-standing paradox of no-go and counter no-go theorems for superradiance, which are shown to refer to different definitions of radiation.
In cavity quantum materials, entangling strongly correlated electrons with quantum light provides a unique opportunity to explore novel quantum phases and phase transitions absent in conventional solid-state materials. In this study, we develop a sign-problem-free fermion-photon hybrid Quantum Monte Carlo (QMC) algorithm, and use it to systematically investigate the ground-state phase diagram of a two-dimensional cavity Hubbard model. It is shown that the interplay between the electron correlation and photon condensation gives rise to intriguing quantum phases ({\it e.g.} superradiant antiferromagnetic and chiral/πππ-flux states), and different quantum phase transitions, such as a first-order superradiant phase transition and a continuous phase transition with Gross-Neveu universality class. The methodology can be readily generalized to more complicated cavity strongly correlated models.
This thesis explores non-equilibrium phenomena in quantum many-body systems, with a focus on correlated electron systems and photon Bose-Einstein condensates. The first part develops the theoretical foundation, beginning with the Lindblad master equation and the construction of non-equilibrium quantum field theory. The two-particle irreducible effective action formalism is introduced, from which the Kadanoff-Baym equations for real-time evolution and the Dyson equation for steady-states are derived. The theoretical groundwork continues with a treatment of strongly correlated electron systems, where non-equilibrium dynamical mean-field theory (DMFT), auxiliary particles, and the non-crossing approximation (NCA) are introduced. These techniques, together with the Lindblad and Kadanoff-Baym approaches, are used throughout the subsequent chapters. The second part presents the main research projects of this thesis. The first two projects are concerned with the fate of the heavy fermion state under irradiation of light. To accurately incorporate light-matter interactions in this case, dipole transitions must be included. In the first project a periodically driven system is considered, where the light can be treated semiclassically. A Floquet DMFT+NCA framework is developed, revealing the mechanisms and conditions under which the heavy fermion state is most strongly suppressed. The second project analyzes a THz spectroscopy experiment performed on CeCu6. In this case a semi-classical treatment of the light field is no longer sufficient, and a full two-time evolution of all the non-equilibrium Green functions is necessary. This approach reveals the microscopic mechanisms underlying the collapse and revival of the Kondo state observed in the experiment. The next project investigates a recent experiment regarding an observation of a non-Hermitian phase transition in EuO. The equilibrium properties of EuO are first analyzed, and then an exciton model is constructed that gives rise to the non-Hermitian phase transition, in good agreement with experimental observations. In the final project, a photon Bose-Einstein condensate in a dye-filled microcavity is studied. A stabilization mechanism, distinct from thermalization, is revealed which admits a condensate phase for orders of magnitude longer than the experimentally relevant timescales.
We investigate the equilibrium behavior of a superconducting circuit QED system containing a large number of artificial atoms. It is shown that the currently accepted standard description of circuit QED via an effective model fails in an important aspect: it predicts the possibility of a superradiant phase transition, even though a full microscopic treatment reveals that a no-go theorem for such phase transitions known from cavity QED applies to circuit QED systems as well. We generalize the no-go theorem to the case of (artificial) atoms with many energy levels and thus make it more applicable for realistic cavity or circuit QED systems.