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arXiv:1905.10697 · Physical Review Letters

Uniqueness of the Phase Transition in Many-Dipole Cavity Quantum Electrodynamical Systems

Adam Stokes, Ahsan Nazir

Published Sep 30, 2020• 45 citations
arXivHTMLPDF

Abstract

The possibility of a superradiant phase transition in light-matter systems is the subject of much debate, due to numerous apparently conflicting no-go and counter no-go theorems. Using an arbitrary-gauge approach we show that a unique phase transition does occur in archetypal many-dipole cavity QED systems, and that it manifests unambiguously via a macroscopic gauge-invariant polarization. We find that the gauge choice controls the extent to which this polarization is included as part of the radiative quantum subsystem and thereby determines the degree to which the abnormal phase is classed as superradiant. This resolves the long-standing paradox of no-go and counter no-go theorems for superradiance, which are shown to refer to different definitions of radiation.

DOI
10.1103/physrevlett.125.143603

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The possibility of a superradiant phase transition in light-matter systems is the subject of much debate, due to numerous apparently conflicting no-go and counter no-go theorems. Using an arbitrary-gauge approach we show that a unique phase transition does occur in archetypal many-dipole cavity QED systems, and that it manifests unambiguously via a macroscopic gauge-invariant polarization. We find that the gauge choice controls the extent to which this polarization is included as part of the radiative quantum subsystem and thereby determines the degree to which the abnormal phase is classed as superradiant. This resolves the long-standing paradox of no-go and counter no-go theorems for superradiance, which are shown to refer to different definitions of radiation.
A potential phase transition between a normal ground state and a photon-condensed ground state in many-dipole light-matter systems is a topic of considerable controversy, exacerbated by conflicting no-go and counter no-go theorems and often ill-defined models. We contribute to the clarification of this long-lasting debate by analyzing two specific arrangements of atoms, including a three-dimensional cubic lattice and a cavity-embedded square lattice layer—which provides a physical model for single-mode cavity QED with coupled dipoles in the thermodynamic limit. These models are shown to significantly differ from the standard Dicke model and, in the thermodynamic limit, give rise to renormalized Hopfield models. We show that a ferroelectric phase transition can, in principle, still occur and the description of the abnormal phase beyond the critical point requires the inclusion of nonlinear terms in the Holstein-Primakoff mapping. We also demonstrate how our model agrees with recent experiments.
In spite of decades of work it has remained unclear whether or not superradiant quantum phases, referred to here as photon condensates, can occur in equilibrium. In this Rapid Communication, we first show that when a nonrelativistic quantum many-body system is coupled to a cavity field, gauge invariance forbids photon condensation. We then present a microscopic theory of the cavity quantum electrodynamics of an extended Falicov-Kimball model, showing that, in agreement with the general theorem, its insulating ferroelectric and exciton condensate phases are not altered by the cavity and do not support photon condensation.
Equilibrium phase transitions between a normal and a photon condensate state (also known as superradiant phase transitions) are a highly debated research topic, where proposals for their occurrence and no-go theorems have chased each other for the past four decades. Previous no-go theorems have demonstrated that gauge invariance forbids second-order phase transitions to a photon condensate state when the cavity-photon mode is assumed to be spatially uniform. First-order phase transitions were previously considered as possible paths to bypass the no-go theorem. In particular, it has been theoretically predicted that a collection of three-level systems coupled to light can display a first-order phase transition to a photon condensate state. Here, we lay down a general no-go theorem, which forbids first-order as well as second-order superradiant phase transitions in a spatially-uniform cavity field. By using the tools of lattice gauge theory, we then derive a fully gauge-invariant model for three-level systems coupled to light. In agreement with the general theorem, our model does not display photon condensation.
We investigate the equilibrium behavior of a superconducting circuit QED system containing a large number of artificial atoms. It is shown that the currently accepted standard description of circuit QED via an effective model fails in an important aspect: it predicts the possibility of a superradiant phase transition, even though a full microscopic treatment reveals that a no-go theorem for such phase transitions known from cavity QED applies to circuit QED systems as well. We generalize the no-go theorem to the case of (artificial) atoms with many energy levels and thus make it more applicable for realistic cavity or circuit QED systems.
The long-standing debate whether the phase transition in the Dicke model can be realized with dipoles in electromagnetic fields is still an unsettled one. The well-known statement often referred to as the ``no-go theorem'' asserts that the so-called A2{A}^{2}A2 term, missing from the Dicke model, is relevant and prevents the system from undergoing a phase transition. At variance with this common belief, in this paper we prove that the Dicke model does give a proper description of the interaction of light field with the internal excitation of atoms. The phase transition and the spontaneous formation of a transverse-electric mean field cannot be excluded by principle. We point out that the proper treatment of the single-mode approximation is crucial, wherefore we present a systematic derivation of the dipole gauge inside a perfect Fabry-P\'erot cavity from first principles. Besides the impact on the debate around the Dicke phase transition, such a cleanup of the theoretical ground of cavity QED is important because currently there are many emerging experimental approaches to reach strong or even ultrastrong coupling between dipoles and photons, which demand a correct treatment of the Dicke model parameters.