The ground-state properties of an ultracold Bose gas in an eightfold symmetric lattice are studied. Mott-insulator, density wave, and supersolid phases are identified. A density wave phase that spontaneously breaks rotational symmetry appears for strong long-range interactions.
Quasicrystals are long-range ordered and yet non-periodic. This interplay results in a wealth of intriguing physical phenomena, such as self-similarity, the inheritance of topological properties from higher dimensions, and the presence of non-trivial structure on all lengthscales. However, quasicrystalline materials are notoriously hard to synthesise, as defects and impurities may greatly alter their final microscopic composition. The field of quantum simulation with ultracold atoms offers a solution to this problem, namely the use of optical lattices – standing waves of light. Optical lattices are free of impurities and therefore ideally suited to study quasicrystals, enabling unprecedented access to observables that are unattainable in condensed matter systems. This study presents the first experimental realisation of a two-dimensional quasicrystalline potential for ultracold atoms, based on an eightfold symmetric optical lattice. Features pertaining to both ordered and disordered phases are observed, from sharp diffraction peaks in the matter-wave interference pattern, to a disorder-induced localised phase emerging at a critical lattice depth V_loc ~ 1.78 E_rec. The localised phase seems to be resilient against moderate interactions, which would make this the first experimental realisation of a 2D Bose glass.
This thesis concerns the physics of ultracold bosons in quasicrystalline lattices, studied by means of quantum simulation using ultracold 39K atoms loaded to an eight-fold rotationally symmetric optical quasicrystal. Quasicrystalline and quasiperiodic systems, thanks to their long-range order and lack of periodicity, exhibit a wealth of interesting properties such as a dense and self-similar momentum space, and a localization transition to Anderson insulator or Bose glass states (in non-interacting or interacting cases respectively) reminiscent of that in disordered systems, whilst lacking the rare regions that typically exist in such systems. Here we will cover experiments into this system’s behaviour in both equilibrium and non-equilibrium settings. First, we focus on mapping out its phase diagram in both weakly and strongly interacting regimes. We observe consistency with numerical predictions for the superfluid-Bose glass phase transition using coherence measurements, as well as finding a region of roughly zero compressibility around where the numerics predicts the existence of a Mott insulator ground state. We also study which regimes of the phase diagram can be ramped through adiabatically, finding that entropy is created upon traversing the Bose glass phase irrespective of ramp duration, which we attribute to its localized nature. Next we look into the dynamics of the system after a quench of the lattice depth in the weakly interacting regime. Upon quenching from the superfluid regime to the Bose glass regime, we observe a quantum walk to higher order diffraction peaks in momentum space whose maximum order is unbounded by kinetic energy thanks to the dense, self-similar nature of the quasicrystal’s momentum space. Quenching in the opposite direction we observe instead a walk between sites in real space for short times by looking at the position (as opposed to momentum) space autocorrelation function of the cloud, finding an expansion rate in agreement with an intuitive estimate based on the Lieb-Robinson bounds of a periodic system. We also look into the timescales of these dynamics in the context of what we might expect from the underlying Hamiltonian, before finally investigating the loss of coherence exhibited by the system after a slower quench of the lattice depth from an initially superfluid cloud. We observe that coherence is lost sooner after the quench for deeper final lattices, with the loss becoming almost instantaneous for quenches that cross the localization transition across the whole cloud. After this we explore the system’s transport dynamics by means of a quench to an excited state at the same time as an additional confining potential is switched off. We observe that unlike in the case of a periodic square lattice, where ballistic expansion that scales with the tunnelling strength occurs in the non-interacting case before becoming slower upon the introduction of interactions thanks to diffusion, in the quasicrystal the transport rate no longer scales with tunnelling strength. Instead we observe a drop relative to the tunnelling rate by 2 − 3 orders of magnitude as the lattice depth is increased from 1Er to 5Er with little dependence on the interaction strength. We also note that the finite rate measured for the deeper lattices is potentially an overestimate since the finite loss rate of atoms makes mass transport indistinguishable from density-dependent losses at that point. Finally, we discuss use of a quantum gas magnification scheme with which to magnify the real space density distribution of our atoms such that it can be measured with single-site resolution. Some preliminary results are presented regarding how the density distribution changes with lattice depth in the weakly interacting regime, in which we observe that as lattice depth increases a higher proportion of atoms occupy deeper sites close to the centre of the quasicrystal’s configuration space, as we might expect.
This thesis contains theoretical research on ultracold quantum gases in spatially periodic potentials, featuring high-frequency periodic driving, long-range interactions, or both. The largest part features deep potentials where the behaviour of the gas is well-described by quantum lattice models. The periodic driving is then integrated out to obtain effective time-independent descriptions. One project investigates emergent long-range interactions in a stationary, weak, spatially periodic potential, where a lattice theory is not appropriate.In two short introductory chapters, the topics of ultracold atoms, optical lattice potentials, periodic driving, and long-range interactions, are sketched, without attempting to give a complete overview. Some experimentally relevant length and energy scales are given, but the main focus is on deriving and constructing theoretical descriptions of ultracold gases in various spatially and/or temporally periodic potentials.The first project presented, is focused on how the single-particle spectrum of a Bose gas in a non-separable two-dimensional square lattice is affected by high-frequency periodic driving; the most striking conclusion is that under suitable circumstances, it develops two inequivalent minima, leading to finite-momentum Bose-Einstein condensation. Perturbative calculations indicate that local interactions induce spontaneous time-reversal symmetry breaking (TRSB) in such a system.The second project investigates the interplay between kinetic frustration and long-range interactions in fermionic gases. Both a mean-field approximation and exact diagonalisations predict that such a system, studied in the more specific realisation of a weakly interacting dipolar fermionic gas in a 2D triangular lattice, also leads to spontaneous TRSB. Furthermore, a density wave could form at quarter filling, where the Fermi surface is perfectly nested. Perhaps more interesting yet, a spatially inhomogeneous TRSB pattern is predicted, confined to the low-density sublattice that emerges in the density wave.The third project revolves around the question of supersolidity in the presence of a gauge field. Applying the Bogolyubov approximation to a variation of the extended Bose-Hubbard model, indicates that combining an artificial staggered magnetic field in a 2D square lattice with nearest-neighbour density-density interactions, not only leads to a supersolid with staggered vortices, but also induces an inhomogeneous distribution of the associated currents around the elementary plaquette.In the fourth project, a one-dimensional Bose gas with strong local interactions in a weak lattice at incommensurate densities is shown to feature excitations corresponding to excess or deficit particles. The excitations interact repulsively at long distances, in spite of the fact that the underlying atoms themselves do not. As a consequence, the incommensurability of the density with the lattice can drive a transition to a density wave and even a supersolid.The four above-mentioned research projects combine bosonic and fermionic gases, weak and strong interactions, perturbative and mean-field approximations, effective field theories and exact diagonalisations. The main overall conclusion is that long-range interactions and high-frequency periodic driving lead to a very diverse range of fascinating phenomena in ultracold lattice gases.
Quasicrystals exhibit exotic properties inherited from the self-similarity of their long-range ordered, yet aperiodic, structure. The recent realization of optical quasicrystal lattices paves the way to the study of correlated Bose fluids in such structures, but the regime of strong interactions remains largely unexplored, both theoretically and experimentally. Here, we determine the quantum phase diagram of two-dimensional correlated bosons in an eightfold quasicrystal potential. Using large-scale quantum Monte Carlo calculations, we demonstrate a superfluid-to-Bose glass transition and determine the critical line. Moreover, we show that strong interactions stabilize Mott insulator phases, some of which have spontaneously broken eightfold symmetry. Our results are directly relevant to current generation experiments and, in particular, drive prospects to the observation of the still elusive Bose glass phase in two dimensions and exotic Mott phases.
Motivated by the recent experiment on the Bose-Einstein condensation of 52Cr atoms with long-range dipolar interactions (Werner J. et al., Phys. Rev. Lett., 94 (2005) 183201), we consider a system of bosons with repulsive nearest and next-nearest neighbor interactions in an optical lattice. The ground state phase diagram, calculated using the Gutzwiller ansatz, shows, apart from the superfluid (SF) and the Mott insulator (MI), two modulated phases, \textit{i.e.}, the charge density wave (CDW) and the supersolid (SS). Excitation spectra are also calculated which show a gap in the insulators, gapless, phonon mode in the superfluid and the supersolid, and a mode softening of superfluid excitations in the vicinity of the modulated phases. We discuss the possibility of observing these phases in cold dipolar atoms and propose experiments to detect them.
Nonstandard Bose-Hubbard models can exhibit rich ground-state phase diagrams, even when considering the one-dimensional limit. Using a self-consistent Gutzwiller diagonalization approach, we study the mean-field ground-state properties of a long-range interacting atomic gas in a one-dimensional optical lattice. We first confirm that the inclusion of long-range two-body interactions to the standard Bose-Hubbard model introduces density-wave and supersolid phases. However, the introduction of pair and density-dependent tunneling can result in new phases with two-site periodic density, single-particle transport, and two-body transport order parameters. These staggered phases are potentially a mean-field signature of the known novel twisted superfluids found via a density-matrix renormalization group approach [Phys. Rev. A 94, 011603(R) (2016)]. We also observe other unconventional phases which are characterized by sign staggered order parameters between adjacent lattice sites.