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arXiv:1903.01279 · Physical Review Letters

Tuning Topological Orders by a Conical Magnetic Field in the Kitaev Model

Ming-Hong Jiang, Shuang Liang, Wei Chen, Yang Qi, Jian‐Xin Li, Qiang-Hua Wang

Published Oct 23, 2020• 25 citations
arXivHTMLPDF

Abstract

We show that a conical magnetic field H=(1,1,1)H can be used to tune the topological order and hence, anyon excitations of the Z_{2} quantum spin liquid in the isotropic antiferromagnetic Kitaev model. A novel topological order, featured with Chern number C=4 and Abelian anyon excitations, is induced in a narrow range of intermediate fields H_{c1}≤H≤H_{c2}. On the other hand, the C=1 Ising-topological order with non-Abelian anyon excitations, as previously known to be present at small fields, is found here to survive up to H_{c1}. The results are obtained by developing and applying a Z_{2} mean field theory that works at finite fields and is asymptotically exact in the zero field limit and the associated variational quantum Monte Carlo.

DOI
10.1103/physrevlett.125.177203

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We show that a conical magnetic field H=(1,1,1)H can be used to tune the topological order and hence, anyon excitations of the Z_{2} quantum spin liquid in the isotropic antiferromagnetic Kitaev model. A novel topological order, featured with Chern number C=4 and Abelian anyon excitations, is induced in a narrow range of intermediate fields H_{c1}≤H≤H_{c2}. On the other hand, the C=1 Ising-topological order with non-Abelian anyon excitations, as previously known to be present at small fields, is found here to survive up to H_{c1}. The results are obtained by developing and applying a Z_{2} mean field theory that works at finite fields and is asymptotically exact in the zero field limit and the associated variational quantum Monte Carlo.
We microscopically construct an Abelian mutual Chern-Simons lattice gauge theory for magnetic field-tuned topological transitions in the Kitaev model and obtain a complete characterization of the phases, including their quasiparticles. At low fields for both ferro (FM) and antiferromagnetic (AFM) Kitaev interactions, we demonstrate non-Abelian Ising topological order (ITO), and explicitly construct the Majorana anyon as an intrinsic excitation---a twist defect in our Abelian gauge theory. For the AFM case, an Abelian chiral phase appears at intermediate fields with trivial topological order and fermionic bulk excitations. Remarkably, both the ITO phase and the intermediate phase have the same chiral central charge c=1/2,c=1/2,c=1/2, implying no change in the quantized thermal Hall response across the transition. For the FM case, there is a direct transition from ITO to a partially polarized nontopological phase. Our paper completes the proof of Kitaev's original proposal of the low-field ITO, with c=1/2c=1/2c=1/2 going beyond his mean-field arguments by including the crucial effect of the gauge fluctuations, and provides a resolution of the debate surrounding the intermediate field phase in the AFM case.
Non-Abelian anyons in quantum spin liquids (QSLs) provide a promising route to fault-tolerant topological quantum computation. In the exactly solvable Kitaev honeycomb model, such anyons of the QSL state can be bound to nonmagnetic spin vacancies and endowed with non-Abelian statistics by an infinitesimal magnetic field. Here, we investigate how this approach for stabilizing non-Abelian anyons extends to a finite magnetic field represented by a proper Zeeman term. Through large-scale density-matrix renormalization group simulations, we compute the vacancy-anyon binding energy as a function of magnetic field for both the ferromagnetic and antiferromagnetic Kitaev models. We find that anyon binding remains robust within the entire QSL phase for the ferromagnetic Kitaev model but breaks down already inside this phase for the antiferromagnetic Kitaev model. To compute a binding energy several orders of magnitude below the magnetic energy scale, we introduce both a refined definition and an extrapolation scheme based on carefully tailored perturbations.
The Kitaev spin liquid, stabilized as the ground state of the Kitaev honeycomb model, is a paradigmatic example of a topological Z2{\mathbb{Z}}_{2}Z2​ quantum spin liquid. The fate of the Kitaev spin liquid in presence of an external magnetic field is at present, a subject of intense scrutiny due to recent experimental signatures pointing to a Z2{\mathbb{Z}}_{2}Z2​ topological phase in certain materials, as well as theoretical studies predicting the emergence of a quantum spin liquid phase of debated nature. In this work, we employ hierarchical mean-field theory, a method based on the use of clusters preserving relevant symmetries and short-range quantum correlations, to investigate the quantum phase diagram of the antiferromagnetic Kitaev's model in a [111] magnetic field. By using clusters of 24 sites, we predict that the Kitaev spin liquid transits through two intermediate phases, characterized by emerging stripe and chiral orders, respectively, before entering the trivial partially polarized phase, differing from previous studies. We assess our results by performing exact diagonalization and computing the scaling of different observables, including the many-body Chern number and other topological quantities, thus establishing hierarchical mean-field theory as a method to study models of frustrated quantum magnetism potentially hosting topological quantum spin liquids.
Non-Abelian anyonic excitations of quantum spin liquids have potential for application to topological quantum computation, but designing logical operations requires developing protocols to faithfully create, move, and read out such quasiparticles. In this paper, we test two such protocols for manipulating Z 2 fluxes (“visons”) of ferromagnetic and antiferromagnetic Kitaev models perturbed by a small uniform magnetic field. We show that a protocol that employs a driving magnetic field locally applied to the sites of the lattice suffers from significant unavoidable errors. These errors, accumulating over time, prevent reaching high probabilities of generating and displacing flux pairs. However, individual spin couplings can also be turned on and off, thus it is possible to create and displace fluxes with nearly 100 % probability. We show that braiding non-Abelian anyons can be achieved with good precision with our second protocol. We comment on the feasibility of our protocols in solid-state devices and quantum emulators.
We investigate how the Kitaev spin liquid state described by Majorana fermions coupled with Z2{Z}_{2}Z2​ gauge fields is affected by non-Kitaev interactions which exist in real candidate materials of the Kitaev magnet. It is found that the off-diagonal exchange interaction referred to as the ${\mathrm{\ensuremath{\Gamma}}}^{\ensuremath{'}}$ term dramatically changes the Majorana band structure in the case of the antiferromagnetic Kitaev interaction and gives rise to a topological phase transition from a non-Abelian topological phase with the Chern number equal to $\ifmmode\pm\else\textpm\fi{}1$ to an Abelian phase with the Chern number equal to $\ifmmode\pm\else\textpm\fi{}2$, in which the Z2{Z}_{2}Z2​ vortices behave as Abelian anyons. On the other hand, other non-Kitaev interactions such as the Heisenberg interaction and the $\mathrm{\ensuremath{\Gamma}}$ term only affect the bandwidth of the Majorana band as long as the spin liquid state is not destabilized.
Recent numerical studies indicate that the antiferromagnetic Kitaev honeycomb lattice model undergoes a magnetic-field-induced quantum phase transition into a new spin-liquid phase. This intermediate-field phase has been previously characterized as a gapless spin liquid. By implementing a recently developed variational approach based on the exact fractionalized excitations of the zero-field model, we demonstrate that the field-induced spin liquid is gapped and belongs to Kitaev's 16-fold way. Specifically, the low-field non-Abelian liquid with Chern number C = ±1 transitions into an Abelian liquid with C = ±4. The critical field and the field-dependent behaviors of key physical quantities are in good quantitative agreement with published numerical results. Furthermore, we derive an effective field theory for the field-induced critical point which readily explains the ostensibly gapless nature of the intermediate-field spin liquid.