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arXiv:2003.05645 · Physical review. B./Physical review. B

Topological phase transition to Abelian anyon phases due to off-diagonal exchange interaction in the Kitaev spin liquid state

Daichi Takikawa, Satoshi Fujimoto

Published Nov 9, 2020• 17 citations
arXivHTMLPDF

Abstract

We investigate how the Kitaev spin liquid state described by Majorana fermions coupled with ${Z}_{2}$ gauge fields is affected by non-Kitaev interactions which exist in real candidate materials of the Kitaev magnet. It is found that the off-diagonal exchange interaction referred to as the ${\mathrm{\ensuremath{\Gamma}}}^{\ensuremath{'}}$ term dramatically changes the Majorana band structure in the case of the antiferromagnetic Kitaev interaction and gives rise to a topological phase transition from a non-Abelian topological phase with the Chern number equal to $\ifmmode\pm\else\textpm\fi{}1$ to an Abelian phase with the Chern number equal to $\ifmmode\pm\else\textpm\fi{}2$, in which the ${Z}_{2}$ vortices behave as Abelian anyons. On the other hand, other non-Kitaev interactions such as the Heisenberg interaction and the $\mathrm{\ensuremath{\Gamma}}$ term only affect the bandwidth of the Majorana band as long as the spin liquid state is not destabilized.

DOI
10.1103/physrevb.102.174414

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We study a mixed-state topological transition in the non-Abelian Kitaev spin liquid driven by a bond-dephasing channel. In the vectorized picture, bond dephasing maps onto interactions between two time-reversed fractionalized Majorana systems coupled to gapped Z2\mathbb Z_2Z2​ gauge fields, enabling sign-problem-free Monte Carlo simulations. We show that increasing dephasing condenses an inter-copy fermion pair, converting Ising⊠Ising‾{\rm Ising}\boxtimes\overline{\rm{Ising}}Ising⊠Ising​ to toric-code order in the Choi state and yielding intrinsically mixed-state topological order upon unfolding. More interestingly, at a temporal interface between topological and trivial Kitaev states, a Chern-number mismatch enforces a gapless Majorana mode. Dephasing then drives a mixed-state topological transition at which the gapless mode develops emergent N=1\mathcal N=1N=1 supersymmetry. Our Monte Carlo simulations yield ν=1.27(3)ν=1.27(3)ν=1.27(3) and ηb≃ηf≃0.40η_b\simeqη_f\simeq0.40ηb​≃ηf​≃0.40, consistent with the exact supersymmetric values 5/45/45/4 and 2/52/52/5. The supersymmetric partners are fractionalized and appear physically as distinct gauge-invariant spin strings, providing concrete observables for future experiments.
The competition between fractionalized spin-liquid states and magnetically ordered phases is an important paradigm in frustrated magnetism. Spin-orbit coupled Mott insulators with Ising-like magnetic anisotropies, such as Kitaev materials, are a particularly rich playground to explore this competition. In this work, we use effective field theory methods to show that a direct quantum phase transition can occur in two-dimensional (2D) Ising spin systems between a topologically ordered chiral spin liquid and a phase with magnetic long-range order. Such a transition can be protected by lattice symmetries and is described by a theory of massless Majorana fields coupled to non-Abelian SO(N)\text{SO}(N)SO(N) gauge fields with a Chern-Simons term. We further show that Euclidean Majorana zero modes bound to Z2{\mathbb{Z}}_{2}Z2​ monopole-instantons in the emergent non-Abelian gauge field are key to understanding spontaneous symmetry breaking in the ordered phase.
We microscopically construct an Abelian mutual Chern-Simons lattice gauge theory for magnetic field-tuned topological transitions in the Kitaev model and obtain a complete characterization of the phases, including their quasiparticles. At low fields for both ferro (FM) and antiferromagnetic (AFM) Kitaev interactions, we demonstrate non-Abelian Ising topological order (ITO), and explicitly construct the Majorana anyon as an intrinsic excitation---a twist defect in our Abelian gauge theory. For the AFM case, an Abelian chiral phase appears at intermediate fields with trivial topological order and fermionic bulk excitations. Remarkably, both the ITO phase and the intermediate phase have the same chiral central charge c=1/2,c=1/2,c=1/2, implying no change in the quantized thermal Hall response across the transition. For the FM case, there is a direct transition from ITO to a partially polarized nontopological phase. Our paper completes the proof of Kitaev's original proposal of the low-field ITO, with c=1/2c=1/2c=1/2 going beyond his mean-field arguments by including the crucial effect of the gauge fluctuations, and provides a resolution of the debate surrounding the intermediate field phase in the AFM case.
Temperature evolution of the spin correlation and excitation spectrum is investigated for a Kitaev model defined on a decorated honeycomb lattice by using the quantum Monte Carlo simulation in the Majorana fermion representation. The ground state of this quantum spin model is given by two kinds of chiral spin liquids: one is topologically trivial with Abelian anyon excitations, and the other is topologically nontrivial with non-Abelian anyon excitations. While lowering temperature, the model exhibits several crossovers in the paramagnetic state, which originate from the fractionalization of quantum spins into Majorana fermions, in addition to a phase transition associated with time reversal symmetry breaking. We show that the spin correlation develops around the crossover temperatures, whereas it shows a slight change at the critical temperature, as in other Kitaev-type models. We also calculate the excitation spectrum in terms of Majorana fermions, and find that the excitation gap in the non-Abelian phase is fragile against thermal fluctuations of the Z2Z_2Z2​ fluxes, while that in the Abelian phase remains open.