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arXiv:1811.10484 · Optics Letters

Phase transfer between three visible lasers for coherent population trapping

Mathieu Collombon, G. Hagel, Cyril Chatou, Didier Guyomarc’h, Didier Ferrand, M. Houssin, C. Champenois, Martina Knoop

Published Feb 4, 2019• 9 citations
arXivHTMLPDF

Abstract

Stringent conditions on the phase relation of multiple photons are a prerequisite for novel protocols of high-resolution coherent spectroscopy. In a recent experiment, we have implemented an interrogation process of a Ca+-ion cloud based on three-photon coherent population trapping, with the potential to serve as a frequency reference in the THz range. This high-resolution interrogation has been made possible by phase-locking both laser sources for cooling and repumping of the trapped ions to a clock laser at 729 nm by means of an optical frequency comb. The clock laser, a titanium-sapphire laser built in our lab locked onto two high-finesse cavities reaches a linewidth of a few Hertz and a frequency stability below 10−14 at 1 s, performances which can be copied onto the two other sources. In this paper, we discuss the performances of the phase transfer between the three involved lasers via the optical frequency comb.

DOI
10.1364/ol.44.000859

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Stringent conditions on the phase relation of multiple photons are a prerequisite for novel protocols of high-resolution coherent spectroscopy. In a recent experiment, we have implemented an interrogation process of a Ca+-ion cloud based on three-photon coherent population trapping, with the potential to serve as a frequency reference in the THz range. This high-resolution interrogation has been made possible by phase-locking both laser sources for cooling and repumping of the trapped ions to a clock laser at 729 nm by means of an optical frequency comb. The clock laser, a titanium-sapphire laser built in our lab locked onto two high-finesse cavities reaches a linewidth of a few Hertz and a frequency stability below 10−14 at 1 s, performances which can be copied onto the two other sources. In this paper, we discuss the performances of the phase transfer between the three involved lasers via the optical frequency comb.
The authors significantly extend the optical technique of coherent population trapping (CPT) using three photons, based on a dark resonance of trapped Ca+{}^{+}+ ions. CPT with three photons is an important approach for high-precision measurements, as it opens up the use of large ensembles of trapped ions, rather than individual atoms. Furthermore, an atomic terahertz frequency reference based on three visible lasers can be derived from this technique. Terahertz spectroscopy is a rapidly growing field with a host of applications, and recent studies point to a clear need for frequency standards in this range.
We demonstrate phase locking of a 729 nm diode laser to a 1542 nm master laser via an erbium-doped-fiber frequency comb, using a transfer-oscillator feedforward scheme which suppresses the effect of comb noise in an unprecedented 1.8 MHz bandwidth. We illustrate its performance by carrying out coherent manipulations of a trapped calcium ion with 99 % fidelity even at few-μs timescales. We thus demonstrate that transfer-oscillator locking can provide sufficient phase stability for high-fidelity quantum logic manipulation even without pre-stabilization of the slave diode laser.
Quantum technologies are nowadays emerging as enabling tools for practical applications, such as quantum sensing, quantum computing and quantum metrology. Lasers play a central role in many of these technological platforms, e.g. for atomic clocks, ion-based or neutral atom-based quantum computers or atom interferometers. Here we present a complete laser system to cool, trap and control strontium atoms in an optical lattice or in tweezer arrays. A sub-Hz linewidth master laser, locked to a high-finesse optical cavity provides the frequency reference for an ultra-low noise comb. The rack-mounted laser system consists of all cooling, repumping, and clock lasers stabilized to the optical frequency comb. Each of the involved laser frequencies can therefore be tuned and mapped in the frequency domain with a high degree of stability. The system is controlled via a software interface, allowing to operate the cold-atom-based physics package autonomously. The system is tailored for the operation of 88Sr or 87Sr optical lattice clocks, or for quantum computing applications, but other sub-Hz lasers could be obtained by phase locking additional clock laser frequencies to the ultra-stable comb, enabling convenient and accurate optical frequency ratio measurements. The laser system architecture and the relevant characterization measurements will be presented, proposing some user-cases such as quantum computing and atom interferometry on strontium atoms. This represents a technological leap for quantum optics, allowing to explore further applications of quantum sensors outside a traditional lab.
We present a coherent population trapping clock system based on laser-cooled 87Rb atoms. The clock consists of a frequency-stabilized CPT interrogation laser and a cooling laser as well as a compact magneto-optical trap, a high-performance microwave synthesizer, and a signal detection system. The resonance signal in the continuous wave regime exhibits an absorption contrast of ∼ 50%. In the Ramsey interrogation method, the linewidth of the central fringe is 31.25 Hz. The system achieves fractional frequency stability of 2.4 × 10 − 11 / τ , which goes down to 1.8 × 10−13 at 20000 s. The results validate that cold atom interrogation can improve the long-term frequency stability of coherent population trapping clocks and holds the potential for developing compact/miniature cold atoms clocks.
Atoms confined in the optical lattice can be interrogated with Doppler- and recoil-free operation. However, if not properly controlled, the optical lattice may limit clock accuracy. To improve the lattice-light-shift uncertainty, the cooling and trapping lasers' frequency stability is optimized, and the atom's signal stability is enhanced. A ring-cavity Ti:sapphire laser is locked to the optical frequency comb, which is referenced to a 578 nm ultra-stable laser, and the beat note's stability is on the order of 10−16. Using a 10 cm Fabry–Pérot cavity referenced to the Ti:sapphire laser, the optical frequency stability is transferred to the 399 nm cooling laser, creating favorable conditions for evaluating the lattice-light-shift accurately. We reevaluate lattice-light-shift in our 171Yb optical lattice clock with an uncertainty of 8.1 × 10−18, which is an order lower than our previous result, and the magic frequency is determined to be 394 798 266.6(1.3) MHz.
We describe a phase-coherent laser system designed for use in experiments involving coherently prepared atomic media. We implement a simple technique based on a sample-and-hold circuit together with a reset of the integrating electronics that makes it possible to scan continuously the relative frequency between the lasers of over tens of gigahertz while keeping them phase locked. The system consists of three external-cavity diode lasers operating around 795 nm. A low-power laser serves as a frequency reference for two high-power lasers which are phased locked with an optical phase-locked loop. We measured the residual phase noise of the system to be less than 0.04 rad(2). In order to show the application of the system towards atomic coherence experiments, we used it to implement electromagnetically induced transparency in a rubidium vapor cell and obtained a reduction in the absorption coefficient of 92%.