Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1811.07200 · Physical Review A

Seeded and unseeded high-order parametric down-conversion

Cameron Okoth, Andrea Cavanna, Nicolas Y. Joly, Maria V. Chekhova

Published Apr 9, 2019• 22 citations
arXivHTMLPDF

Abstract

Spontaneous parametric down-conversion (SPDC) has been one of the foremost tools in quantum optics for over five decades. Over that time, it has been used to demonstrate some of the curious features that arise from quantum mechanics. Despite the success of SPDC, its higher-order analogs have never been observed, even though it has been suggested that they generate far more unique and exotic states than SPDC. An example of this is the emergence of non-Gaussian states without the need for postselection. Here we calculate the expected rate of emission for $n\mathrm{th}$-order SPDC with and without external stimulation (seeding). Focusing primarily on third-order parametric down-conversion, we estimate the photon detection rates in a rutile crystal for both the unseeded and seeded regimes.

DOI
10.1103/physreva.99.043809

Related papers

Scalability of parametric down-conversion for generating higher-order Fock states

Johannes Tiedau, Tim J. Bartley, Georg Harder +4 more

Spontaneous parametric down-conversion (SPDC) is the most widely used method to generate higher-order Fock states ($n\ensuremath{\ge}2$). Yet, a consistent performance analysis from fundamental principles is missing. Here, we address this problem by introducing a framework for state fidelity and generation probability under the consideration of losses and multimode emission. With this analysis we show the fundamental limitations of this process as well as a trade-off between state fidelity and generation rate intrinsic to the probabilistic nature of the process. This identifies the parameter space for which SPDC is useful when generating higher-order Fock states for quantum applications. We experimentally investigate the multiphoton regime of SPDC and demonstrate heralded Fock states up to $|n\ensuremath{\rangle}=4$.

arXiv:1901.03237•Physical Review A•Oct 18, 2019•50 citations

Three-fold coincidence by stimulated parametric down-conversion

Yishai Klein, Alessio D'Errico, Farid Ghobadi +4 more

Parametric down-conversion is a widely used source of nonclassical light in quantum optics and photonic quantum technologies. While stimulated parametric down-conversion with strong classical seeds is well studied, the regime in which stimulation occurs at the single-photon level has hitherto remained largely unexplored experimentally. Here, we study continuous-wave, low-gain down-conversion seeded by a weak coherent field with an average photon number well below one per coherence time. By measuring third-order temporal correlations, we observe a clear enhancement that cannot be accounted for by spontaneous processes or accidental coincidences alone, and is consistent with stimulation involving the seed and the generated photon pair. These results provide time-domain evidence of seed-induced three-photon correlations and suggest new ways to engineer and probe multi-photon states for quantum imaging, sensing, and information processing.

quant-pharXiv:2605.27653•May 28, 2026•0 citations

Second-order correlations and purity of unheralded single photons from spontaneous parametric down-conversion

A. Padhye, K. Muhammed Shafi, C. M. Chandrashekar

Various quantum technology applications require high-purity single photons with high generation rate. Although different methods are employed to generate such photons, heralded single photons from spontaneous parametric down-conversion (SPDC) is the most commonly used approach. Photon generation rate from the heralded single-photon sources are limited by the efficiency of the detectors to record coincidence detection of the photon pairs which are lower than the single-photon counts recorded separately on each detector. In this paper we present a revised expression to calculate second-order temporal correlation function, $g^{(2)}$ for any fixed time window (bin) and report the experimental characterization of purity of unheralded and heralded single photons from the SPDC process. With an appropriate choice of time bin for a given pump power, without heralding we show that higher rate of single photons with $g^{(2)}(0) = 0$ can be generated with very high probability.

arXiv:2207.06984•Jul 14, 2022•0 citations

Three-photon generation by means of third-order spontaneous parametric down-conversion in bulk crystals

N A Borshchevskaya, Konstantin G. Katamadze, S P Kulik +1 more

We investigate the third-order spontaneous parametric down-conversion process in a nonlinear media with inversion centers. Specifically, we analyze in details the three-photon differential count rate in unit frequency and angular regions, total count rate and measurement time for rutile and calcite crystals which have comparatively large cubic susceptibilities. Special attention is given to consideration of limited frequency and angular detection ranges in order to calculate experimentally available detection rate values.

arXiv:1508.03291•Laser Physics Letters•Oct 16, 2015•31 citations

Stimulated parametric down-conversion at the single-photon level

Yishai Klein, Alessio Errico, Roohollah Ghobadi +4 more

Parametric down-conversion is a widely used source of nonclassical light in quantum optics and photonic quantum technologies. While stimulated parametric down-conversion with strong classical seeds is well studied, the elementary physical mechanism of stimulation by individual photons has remained largely unexplored experimentally. Here, we study continuous-wave, low-gain down-conversion seeded by an ultra-weak coherent field with an average photon number well below one per coherence time. By measuring third-order temporal correlations, we access the regime in which the single-photon component of the seed can stimulate the emission of a photon pair, giving rise to a temporally correlated three-photon event. We observe a clear enhancement that cannot be explained by spontaneous processes or accidental coincidences alone, providing time-domain evidence of the fundamental stimulation mechanism at the single-photon level. Beyond its fundamental significance, these results suggest new ways to characterize seed–PDC mode overlap, phase matching, and weak nonlinear coupling in regimes where bright stimulated-emission measurements are not appropriate. Multimode and interferometric extensions could enable correlation-based imaging and phase-sensitive spectroscopy.

Optica•Oct 8, 2026•0 citations

Experimental Realization of Spontaneous Parametric Down Conversion

Mahmood Hasani, Mobin Motaharifar

Spontaneous Parametric Down-Conversion (SPDC) is a cornerstone phenomenon in nonlinear optics, where an incident high-energy photon is transformed into a pair of lower-energy photons. This quantum process serves as a fundamental tool for generating entangled photon pairs, heralded single photons, and squeezed light, making it indispensable in the realms of quantum communication, quantum computing, and precision metrology. In this paper, we present a comprehensive study on the theoretical foundations and practical realization of an SPDC experimental setup, developed for the first time at the Photonics Research Laboratory at Amirkabir University of Technology. Our setup features a self-grown potassium dihydrogen phosphate (KDP) nonlinear crystal, illuminated by a 450 nm blue laser, to achieve parametric down-conversion into infrared photon pairs at 900 nm. By integrating a custom-designed transimpedance amplifier with a BPX65 photodiode, we have successfully amplified and detected the weak SPDC signal, demonstrating the feasibility of achieving high sensitivity with low-cost, widely available components. The experimental results align closely with theoretical predictions, showcasing the effectiveness of the system in detecting photon pairs with minimal resources. This study underscores the accessibility and scalability of SPDC technology, providing a blueprint for constructing versatile quantum optics experiments in resource-limited settings. By bridging the gap between theoretical insight and experimental realization, we aim to inspire further exploration of SPDC's potential in both foundational research and practical applications, laying the groundwork for future innovations in quantum technologies.

•Dec 14, 2024•0 citations
Spontaneous parametric down-conversion (SPDC) has been one of the foremost tools in quantum optics for over five decades. Over that time, it has been used to demonstrate some of the curious features that arise from quantum mechanics. Despite the success of SPDC, its higher-order analogs have never been observed, even though it has been suggested that they generate far more unique and exotic states than SPDC. An example of this is the emergence of non-Gaussian states without the need for postselection. Here we calculate the expected rate of emission for nthn\mathrm{th}nth-order SPDC with and without external stimulation (seeding). Focusing primarily on third-order parametric down-conversion, we estimate the photon detection rates in a rutile crystal for both the unseeded and seeded regimes.
Spontaneous parametric down-conversion (SPDC) is the most widely used method to generate higher-order Fock states ($n\ensuremath{\ge}2$). Yet, a consistent performance analysis from fundamental principles is missing. Here, we address this problem by introducing a framework for state fidelity and generation probability under the consideration of losses and multimode emission. With this analysis we show the fundamental limitations of this process as well as a trade-off between state fidelity and generation rate intrinsic to the probabilistic nature of the process. This identifies the parameter space for which SPDC is useful when generating higher-order Fock states for quantum applications. We experimentally investigate the multiphoton regime of SPDC and demonstrate heralded Fock states up to $|n\ensuremath{\rangle}=4$.
Parametric down-conversion is a widely used source of nonclassical light in quantum optics and photonic quantum technologies. While stimulated parametric down-conversion with strong classical seeds is well studied, the regime in which stimulation occurs at the single-photon level has hitherto remained largely unexplored experimentally. Here, we study continuous-wave, low-gain down-conversion seeded by a weak coherent field with an average photon number well below one per coherence time. By measuring third-order temporal correlations, we observe a clear enhancement that cannot be accounted for by spontaneous processes or accidental coincidences alone, and is consistent with stimulation involving the seed and the generated photon pair. These results provide time-domain evidence of seed-induced three-photon correlations and suggest new ways to engineer and probe multi-photon states for quantum imaging, sensing, and information processing.
Various quantum technology applications require high-purity single photons with high generation rate. Although different methods are employed to generate such photons, heralded single photons from spontaneous parametric down-conversion (SPDC) is the most commonly used approach. Photon generation rate from the heralded single-photon sources are limited by the efficiency of the detectors to record coincidence detection of the photon pairs which are lower than the single-photon counts recorded separately on each detector. In this paper we present a revised expression to calculate second-order temporal correlation function, g(2)g^{(2)}g(2) for any fixed time window (bin) and report the experimental characterization of purity of unheralded and heralded single photons from the SPDC process. With an appropriate choice of time bin for a given pump power, without heralding we show that higher rate of single photons with g(2)(0)=0g^{(2)}(0) = 0g(2)(0)=0 can be generated with very high probability.
We investigate the third-order spontaneous parametric down-conversion process in a nonlinear media with inversion centers. Specifically, we analyze in details the three-photon differential count rate in unit frequency and angular regions, total count rate and measurement time for rutile and calcite crystals which have comparatively large cubic susceptibilities. Special attention is given to consideration of limited frequency and angular detection ranges in order to calculate experimentally available detection rate values.
Parametric down-conversion is a widely used source of nonclassical light in quantum optics and photonic quantum technologies. While stimulated parametric down-conversion with strong classical seeds is well studied, the elementary physical mechanism of stimulation by individual photons has remained largely unexplored experimentally. Here, we study continuous-wave, low-gain down-conversion seeded by an ultra-weak coherent field with an average photon number well below one per coherence time. By measuring third-order temporal correlations, we access the regime in which the single-photon component of the seed can stimulate the emission of a photon pair, giving rise to a temporally correlated three-photon event. We observe a clear enhancement that cannot be explained by spontaneous processes or accidental coincidences alone, providing time-domain evidence of the fundamental stimulation mechanism at the single-photon level. Beyond its fundamental significance, these results suggest new ways to characterize seed–PDC mode overlap, phase matching, and weak nonlinear coupling in regimes where bright stimulated-emission measurements are not appropriate. Multimode and interferometric extensions could enable correlation-based imaging and phase-sensitive spectroscopy.
Spontaneous Parametric Down-Conversion (SPDC) is a cornerstone phenomenon in nonlinear optics, where an incident high-energy photon is transformed into a pair of lower-energy photons. This quantum process serves as a fundamental tool for generating entangled photon pairs, heralded single photons, and squeezed light, making it indispensable in the realms of quantum communication, quantum computing, and precision metrology. In this paper, we present a comprehensive study on the theoretical foundations and practical realization of an SPDC experimental setup, developed for the first time at the Photonics Research Laboratory at Amirkabir University of Technology. Our setup features a self-grown potassium dihydrogen phosphate (KDP) nonlinear crystal, illuminated by a 450 nm blue laser, to achieve parametric down-conversion into infrared photon pairs at 900 nm. By integrating a custom-designed transimpedance amplifier with a BPX65 photodiode, we have successfully amplified and detected the weak SPDC signal, demonstrating the feasibility of achieving high sensitivity with low-cost, widely available components. The experimental results align closely with theoretical predictions, showcasing the effectiveness of the system in detecting photon pairs with minimal resources. This study underscores the accessibility and scalability of SPDC technology, providing a blueprint for constructing versatile quantum optics experiments in resource-limited settings. By bridging the gap between theoretical insight and experimental realization, we aim to inspire further exploration of SPDC's potential in both foundational research and practical applications, laying the groundwork for future innovations in quantum technologies.