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arXiv:2605.27653

Three-fold coincidence by stimulated parametric down-conversion

Yishai Klein, Alessio D'Errico, Farid Ghobadi, Dilip Paneru, Nazanin Dehghan, Eliahu Cohen, Ebrahim Karimi

quant-phSubmitted May 26, 2026• Announced May 28, 2026• 0 citations
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Abstract

Parametric down-conversion is a widely used source of nonclassical light in quantum optics and photonic quantum technologies. While stimulated parametric down-conversion with strong classical seeds is well studied, the regime in which stimulation occurs at the single-photon level has hitherto remained largely unexplored experimentally. Here, we study continuous-wave, low-gain down-conversion seeded by a weak coherent field with an average photon number well below one per coherence time. By measuring third-order temporal correlations, we observe a clear enhancement that cannot be accounted for by spontaneous processes or accidental coincidences alone, and is consistent with stimulation involving the seed and the generated photon pair. These results provide time-domain evidence of seed-induced three-photon correlations and suggest new ways to engineer and probe multi-photon states for quantum imaging, sensing, and information processing.

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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•Jun 1, 2019•0 citations
Parametric down-conversion is a widely used source of nonclassical light in quantum optics and photonic quantum technologies. While stimulated parametric down-conversion with strong classical seeds is well studied, the regime in which stimulation occurs at the single-photon level has hitherto remained largely unexplored experimentally. Here, we study continuous-wave, low-gain down-conversion seeded by a weak coherent field with an average photon number well below one per coherence time. By measuring third-order temporal correlations, we observe a clear enhancement that cannot be accounted for by spontaneous processes or accidental coincidences alone, and is consistent with stimulation involving the seed and the generated photon pair. These results provide time-domain evidence of seed-induced three-photon correlations and suggest new ways to engineer and probe multi-photon states for quantum imaging, sensing, and information processing.
Parametric down-conversion is a widely used source of nonclassical light in quantum optics and photonic quantum technologies. While stimulated parametric down-conversion with strong classical seeds is well studied, the elementary physical mechanism of stimulation by individual photons has remained largely unexplored experimentally. Here, we study continuous-wave, low-gain down-conversion seeded by an ultra-weak coherent field with an average photon number well below one per coherence time. By measuring third-order temporal correlations, we access the regime in which the single-photon component of the seed can stimulate the emission of a photon pair, giving rise to a temporally correlated three-photon event. We observe a clear enhancement that cannot be explained by spontaneous processes or accidental coincidences alone, providing time-domain evidence of the fundamental stimulation mechanism at the single-photon level. Beyond its fundamental significance, these results suggest new ways to characterize seed–PDC mode overlap, phase matching, and weak nonlinear coupling in regimes where bright stimulated-emission measurements are not appropriate. Multimode and interferometric extensions could enable correlation-based imaging and phase-sensitive spectroscopy.
Heralded single-photon sources are the most commonly used sources for optical quantum technology applications. There is strong demand for accurate prediction of their spectral features and temporal correlations with ever-increasing precision. This is particularly important in connection with the intrinsically stochastic photon-pair generation process in heralded sources. Here we present a complete theoretical description of the temporal correlation of a signal-idler, signal-signal, and signal-signal-idler coincidences of photons generated by continuous-wave pumped cavity-enhanced spontaneous parametric down-conversion. The theory excellently predicts the measurements, which has been experimentally confirmed in our setup utilizing single-photon detectors with high temporal resolution. This enables us to resolve and analyze the multiphoton correlation functions in great detail.
We study the process of seeded or stimulated third-order parametric down-conversion as an extension of our previous work on spontaneous parametric down-conversion (TOSPDC). We present general expressions for the spectra and throughputs expected for the cases where the seed field or fields overlap either only one or two of the TOSPDC modes and allow for both pump and seed to be either monochromatic or pulsed. We present a numerical study for a particular source design, showing that doubly overlapped seeding can lead to a considerably greater generated flux as compared with singly overlapped seeding. We, furthermore, show that doubly overlapped seeding permits stimulated emission tomography for the reconstruction of the three-photon TOSPDC joint spectral intensity. We hope that our paper will guide future experimental efforts based on the process of third-order parametric down-conversion.
We present a full triple-coincidence analysis of photon-pair states generated by spontaneous parametric down-conversion. By increasing the coherence time of the source with the help of an intracavity setup, our measurements are not spoiled by detection time jitter. Signal-idler, but also thermal signal-signal, correlations are clearly resolved in this regime. Via introduction of an artificial coincidence window, we discuss in detail the transition to the previously studied cases where typically no single-arm correlation is observed. We investigate the heralded antibunching characteristics to show that in our system further studies of continuously generated photon states, possibly higher-photon-number entangled states, can be performed with respect to their (non)applicability in quantum information tasks.
Strongly driven nonlinear optical processes such as spontaneous parametric down-conversion and spontaneous four-wave mixing can produce multiphoton nonclassical beams of light which have applications in quantum information processing and sensing. In contrast to the low-gain regime, new physical effects arise in a high-gain regime due to the interactions between the nonclassical light and the strong pump driving the nonlinear process. Here, we describe and experimentally observe a gain-induced group delay between the multiphoton pulses generated in a high-gain type-II spontaneous parametric down-conversion source. Since the group delay introduces distinguishability between the generated photons, it will be important to compensate for it when designing quantum interference devices in which strong optical nonlinearities are required.
Quantum correlations, where two or more parties exhibit strong correlations in a particular degree of freedom are important resources for fundamental science [1], such as the exploration of non-locality and entanglement, as well as non-classical technologies including quantum computation, quantum key distribution and quantum metrology. One typical way to generate correlated photon pairs is to use the spontaneous four-wave mixing process, with demonstrations on various platforms [2]. So far, single-photon stimulated four-wave mixing (FWM) has been demonstrated in optical fibers [3]. Here we show induced correlation by single photon seeded FWM through exploiting the orthogonal polarization modes in an integrated ring resonator [4]. We allow two different four-wave mixing processes to occur simultaneously with the same signal frequency mode but different idler frequency modes (see Fig.1(a)). The single-photon induced FWM process, named here seeded FWM, was created through the link of type-0 SFWM and type-2 SFWM. In the type-0 process, two excitation photons from the same field are converted into two new photons, signal and idler, with the same polarization as the pump field. While in the type-2 FWM, two annihilated photons, each one from a different polarized pump field, namely TE and TM, generate an orthogonal-polarized photon pair. More importantly, spatial and temporal overlapping of two processes and their sharing of one common resonance lead to correlation between the other two signal photons, one from each process. For example, an idler photon created in type-0 FWM seeds the type-2 FWM process or vice versa, i.e. the TM idler photon in Fig. 1, induces correlation between the signal TM and TE photons. This is proven by the observation of a clear coincidence peak for both signal photons in Fig.1(b). Furthermore, we confirmed our observation via power-dependent correlation measurements (see Fig.1 (c)). We summarized the true coincidence count (C) and its coincidence to accidental ratio (CAR) when only the TE pump power is increased while maintaining the TM mode pump power (black squares), and both pump powers are increased with a constant ratio (blue dots). We found that the seeded FWM scales with the square of both pump powers (C ∝ PjePtm) and that the CAR reach its maxima of 1.5 at the available pump power, indicating thermal statistics. Our findings are relevant to the fundamental understanding of spontaneous parametric effects as well as single-photon induced processes and single photon cloning.