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arXiv:2207.06984

Second-order correlations and purity of unheralded single photons from spontaneous parametric down-conversion

A. Padhye, K. Muhammed Shafi, C. M. Chandrashekar

Published Jul 14, 2022• 0 citations
arXivHTMLPDF

Abstract

Various quantum technology applications require high-purity single photons with high generation rate. Although different methods are employed to generate such photons, heralded single photons from spontaneous parametric down-conversion (SPDC) is the most commonly used approach. Photon generation rate from the heralded single-photon sources are limited by the efficiency of the detectors to record coincidence detection of the photon pairs which are lower than the single-photon counts recorded separately on each detector. In this paper we present a revised expression to calculate second-order temporal correlation function, $g^{(2)}$ for any fixed time window (bin) and report the experimental characterization of purity of unheralded and heralded single photons from the SPDC process. With an appropriate choice of time bin for a given pump power, without heralding we show that higher rate of single photons with $g^{(2)}(0) = 0$ can be generated with very high probability.

DOI
10.48550/arxiv.2207.06984

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Various quantum technology applications require high-purity single photons with high generation rate. Although different methods are employed to generate such photons, heralded single photons from spontaneous parametric down-conversion (SPDC) is the most commonly used approach. Photon generation rate from the heralded single-photon sources are limited by the efficiency of the detectors to record coincidence detection of the photon pairs which are lower than the single-photon counts recorded separately on each detector. In this paper we present a revised expression to calculate second-order temporal correlation function, g(2)g^{(2)}g(2) for any fixed time window (bin) and report the experimental characterization of purity of unheralded and heralded single photons from the SPDC process. With an appropriate choice of time bin for a given pump power, without heralding we show that higher rate of single photons with g(2)(0)=0g^{(2)}(0) = 0g(2)(0)=0 can be generated with very high probability.
Heralded single-photon sources are the most commonly used sources for optical quantum technology applications. There is strong demand for accurate prediction of their spectral features and temporal correlations with ever-increasing precision. This is particularly important in connection with the intrinsically stochastic photon-pair generation process in heralded sources. Here we present a complete theoretical description of the temporal correlation of a signal-idler, signal-signal, and signal-signal-idler coincidences of photons generated by continuous-wave pumped cavity-enhanced spontaneous parametric down-conversion. The theory excellently predicts the measurements, which has been experimentally confirmed in our setup utilizing single-photon detectors with high temporal resolution. This enables us to resolve and analyze the multiphoton correlation functions in great detail.
Heralded single photon sources are the subject of intense research owing to their usefulness in metrology and quantum information. These are often created using a pair of photons produced by spontaneous parametric downconversion (SPDC), from which one photon is used to certify the presence of the other. However, multiple-pair production and detector dark counts limit the quality of such sources. Here, we investigate whether cascading two downconversion events to precertify the presence of a photon pair would allow us to reduce these effects. Using analytical calculations and simulations, we find that higher purity photons, as quantified by the heralded second order correlation function, can be obtained for some detector performance ranges.
Single photons exhibit nonclassical, counterintuitive behavior that can be exploited in the developing field of quantum technology. They are needed for various applications such as quantum key distribution, optical quantum information processing, quantum computing, intensity measurement standards, and others yet to be discovered in this developing field. This drives the current intensive research into the realization of true deterministic sources of single photons on demand. Lacking such a source, many researchers default to the well-established workhorse: spontaneous parametric down-conversion that generates entangled signal-idler pairs. Since this source is thermal statistical in nature, it is common to use a detected idler photon to herald the production of a signal photon. The need exists to determine the quality of the single photons generated in the heralded signal beam. Quite often, the literature reports a heralded second-order coherence function of the signal photons conditioned on the idler photons using readily available single-photon detectors. In this work we examine the applicability of this technique to single-photon characterization and the consequences of the fact that the most commonly used single-photon detectors are not photon-number resolving. Our results show that this method using non-photon-resolving detectors can only be used to characterize the signal-idler correlations rather than the nature of the signal-photon state alone.
The generation of high purity single photons and entangled photon pairs is a crucial first step in many quantum optics experiments, including those that require quantum teleportation [1], entanglement swapping [2], and the generation of multi-photon entanglement [3]. The most widely used and established approach for creating photon pairs is spontaneous parametric down conversion (SPDC) - where pump photons undergo a non-linear optical process to create a down-converted photon pair [4]. Traditionally, the generation of high-purity heralded single photons required severe spectral filtering, introducing additional loss. However, through careful engineering of spectral correlations of the down-converted photon pairs one can circumvent the need for filtering and avoid the accompanying reduction in heralding efficiency.
Cavity-enhanced spontaneous parametric down-conversion (SPDC) can be used to implement heralded single-photon sources with narrow bandwidth down to tens of megahertz, thus compatible with atom-based quantum memories. In this work, we propose and study the cavities that are either singly resonant at the frequency of only one of the generated photons or doubly resonant at the frequency of one generated photon and for the pump field. We derive analytical expressions for the generation rate and the spectral brightness as a function of the main structure parameters. Our analysis shows that by exploiting counterpropagating SPDC inside a cavity with properly designed distributed Bragg reflectors, pure narrow-band heralded single photons can be generated. In particular, when a pulsed pump illuminates a 1-mm-long singly resonant cavity, the bandwidth of the resonant and the nonresonant photons will be 120 MHz and 5.7 GHz, respectively, with heralded single-photon purity as high as 0.993. Due to its small absorption probability inside the cavity, the heralding efficiency can approach unity if the nonresonant partner is used as a heralded single photon. Finally, we also show that continuous-wave excitation of a 1-cm-long cavity resonant for the pump and copropagating fields can provide photon pairs in a narrow bandwidth of 10 MHz with spectral brightness as high as $2\ifmmode\times\else\texttimes\fi{}{10}^{6}$ $({\text{s}\phantom{\rule{4.pt}{0ex}}\text{mW}\phantom{\rule{4.pt}{0ex}}\text{MHz})}^{\ensuremath{-}1}$. This source can efficiently couple with quantum memories and can find applications in quantum information processing and communication.
Low-photon-number sources can exhibit non-classical, counterintuitive behavior that can be exploited in the developing field of quantum technology. Single photons play a special role in this arena since they represent the ultimate lowphoton- number source. They are considered an important element in various applications such as quantum key distribution, optical quantum information processing, quantum computing, intensity measurement standards, and others yet to be discovered in this developing field. True deterministic sources of single photons on demand are currently an area of intensive research, but have not been demonstrated in a practical setting. As a result, researchers commonly default to the well-established workhorse: spontaneous parametric down-conversion generating entangled signal-idler pairs. Since this source is thermal-statistical in nature, it is common to use a detected idler photon to herald the production of a signal photon. The need exists to determine the quality of the single photons generated in the heralded signal beam. Quite often, the literature reports a "heralded second-order coherence function" of the signal photons conditioned on the idler photons using readily available single-photon detectors. In this work, we examine the applicability of this technique to single-photon characterization and the consequences of the fact that the most commonly used single-photon detectors are not photon-number resolving. Our results show that this method using non-photonresolving detectors can only be used to characterize the signal-idler correlations rather than the nature of the signalphoton state alone.