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arXiv:1811.03907 · Physical Review Letters

Microwave-Cavity-Detected Spin Blockade in a Few-Electron Double Quantum Dot

Andreas Landig, Jonne Koski, Pasquale Scarlino, Christian Reichl, W. Wegscheider, Andreas J. Wallraff, K. Ensslin, Thomas Ihn

Published May 29, 2019• 23 citations
arXivHTMLPDF

Abstract

We investigate spin states of few electrons in a double quantum dot by coupling them to a magnetic field resilient NbTiN microwave resonator. The electric field of the resonator couples to the electric dipole moment of the charge states in the double dot. For a two-electron state the spin-triplet state has a vanishing electric dipole moment and can therefore be distinguished from the spin-singlet state. This way the charge dipole sensitivity of the resonator response is converted to a spin selectivity. We thereby investigate Pauli spin blockade known from transport experiments at finite source-drain bias. In addition we find an unconventional spin-blockade triggered by the absorption of resonator photons.

DOI
10.1103/physrevlett.122.213601

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We investigate spin states of few electrons in a double quantum dot by coupling them to a magnetic field resilient NbTiN microwave resonator. The electric field of the resonator couples to the electric dipole moment of the charge states in the double dot. For a two-electron state the spin-triplet state has a vanishing electric dipole moment and can therefore be distinguished from the spin-singlet state. This way the charge dipole sensitivity of the resonator response is converted to a spin selectivity. We thereby investigate Pauli spin blockade known from transport experiments at finite source-drain bias. In addition we find an unconventional spin-blockade triggered by the absorption of resonator photons.
Both quantum transport measurements in the Pauli blockade regime and microwave cavity transmission measurements are important tools for spin-qubit readout and characterization. Based on a generalized input-output theory we derive a theoretical framework to investigate how a double quantum dot (DQD) in a transport setup interacts with a coupled microwave resonator while the current through the DQD is rectified by Pauli blockade. We show that the output field of the resonator can be used to infer the leakage current and thus obtain insight into the blockade mechanisms. In the case of a silicon DQD, we show how the valley quasidegeneracy can impose limitations on this scheme. We also demonstrate that a large number of unknown DQD parameters including (but not limited to) the valley splitting can be estimated from the resonator response simultaneous to a transport experiment, providing more detailed knowledge about the microscopic environment of the DQD. Furthermore, we describe and quantify a back action of the resonator photons on the steady-state leakage current.
A Pauli spin blockade in quantum dot systems occurs when the charge transport is allowed only for some spin states, and it has been an efficient tool in spin-based qubit devices in semiconductors. We theoretically investigate a Pauli spin blockade in a triple quantum dot molecule consisting of three identical quantum dots in a semiconductor in the presence of an external magnetic field through the molecule. When the three-electron state is on resonance with two- or four-electron states, the Aharonov–Bohm oscillation and the Zeeman splitting lead to a periodic spin blockade effect. We focus on the spin blockade at a two- and three-electron resonance and show that we can tune the magnetic field to selectively allow only either a spin-singlet or spin-triplet state to add an additional electron from tunnel-coupled leads. This spin blockade maintains the three quantum dots at the optimal sweet spot against the charge noise, demonstrating its potential as an efficient readout scheme for the qubits in quantum dot systems.
Serial double quantum dots created in semiconductor nanostructures provide a versatile platform for investigating two-electron spin quantum states, which can be tuned by electrostatic gating and an external magnetic field. In this Rapid Communication, we directly measure the supercurrent reversal between adjacent charge states of an InAs nanowire double quantum dot with superconducting leads, in good agreement with theoretical models. In the even charge parity sector, we observe a supercurrent blockade with increasing magnetic field, corresponding to the spin singlet to triplet transition. Our results demonstrate a direct spin to supercurrent conversion, the superconducting equivalent of the Pauli spin blockade. This effect can be exploited in hybrid quantum architectures coupling the quantum states of spin systems and superconducting circuits.
Combining superconducting resonators and quantum dots has triggered tremendous progress in quantum information, however, attempts at coupling a resonator to even charge parity spin qubits have resulted only in weak spin-photon coupling. Here, we integrate a zincblende InAs nanowire double quantum dot with strong spin-orbit interaction in a magnetic-field resilient, high-quality resonator. The quantum confinement in the nanowire is achieved using deterministically grown wurtzite tunnel barriers. Our experiments on even charge parity states and at large magnetic fields, allow us to identify the relevant spin states and to measure the spin decoherence rates and spin-photon coupling strengths. We find an anti-crossing between the resonator mode in the single photon limit and a singlet-triplet qubit with a spin-photon coupling strength of g/2π = 139 ± 4 MHz. This coherent coupling exceeds the resonator decay rate κ/2π = 19.8 ± 0.2 MHz and the qubit dephasing rate γ/2π = 116 ± 7 MHz, putting our system in the strong coupling regime.
Strong coupling of semiconductor spin qubits to superconducting microwave resonators was recently demonstrated [X. Mi et al., Nature 555, 599 (2018); A. J. Landig et al., Nature 560, 179 (2018); N. Samkharadze et al., Science 359, 1123 (2018); T. Cubaynes et al., NPJ Quant. Inf. 5, 47 (2019)]. These breakthroughs pave the way for quantum information processing that combines the long coherence times of solid-state spin qubits with the long-distance connectivity, fast control, and fast high-fidelity quantum-non-demolition readout of existing superconducting qubit implementations. Here we theoretically analyze and optimize the dispersive readout of a single spin in a semiconductor double quantum dot (DQD) coupled to a microwave resonator via its electric dipole moment. The strong spin-photon coupling arises from the motion of the electron spin in a local magnetic field gradient. We calculate the signal-to-noise ratio (SNR) of the readout accounting for both Purcell spin relaxation and spin relaxation arising from intrinsic electric noise within the semiconductor. We express the maximum achievable SNR in terms of the cooperativity associated with these two dissipation processes. We find that while the cooperativity increases with the strength of the dipole coupling between the DQD and the resonator, it does not depend on the strength of the magnetic field gradient. We then optimize the SNR as a function of experimentally tunable DQD parameters. We identify wide regions of parameter space where the unwanted backaction of the resonator photons on the qubit is small. Moreover, we find that the coupling of the resonator to other DQD transitions can enhance the SNR by at least a factor of two, a ``straddling'' effect [J. Koch et al., Phys. Rev. A 76, 042319 (2007)] that occurs only at nonzero energy detuning of the DQD double-well potential. We estimate that with current technology, single-shot readout fidelities in the range 82--95% can be achieved within a few $\ensuremath{\mu}\mathrm{s}$ of readout time without requiring the use of Purcell filters.
As an application in circuit quantum electrodynamics coupled systems, superconducting resonators play an important role in high-sensitivity measurements in a superconducting-semiconductor hybrid architecture. Taking advantage of a high-impedance $\mathrm{Nb}\text{\ensuremath{-}}\mathrm{Ti}\text{\ensuremath{-}}\mathrm{N}$ resonator, we perform excited-state spectroscopy on a GaAs\mathrm{Ga}\mathrm{As}GaAs double quantum dot (DQD) by applying voltage pulses to one gate electrode. The pulse train modulates the DQD energy detuning and gives rise to charge state transitions at zero detuning. Benefiting from the outstanding sensitivity of the resonator, we distinguish different spin-state transitions in the energy spectrum according to the Pauli exclusion principle. Furthermore, we experimentally study how the interdot tunneling rate modifies the resonator response. The experimental results are consistent with the simulated spectra based on our model.