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arXiv:1808.10450 · New Journal of Physics

Reconciliation of quantum local master equations with thermodynamics

Gabriele De Chiara, Gabriel Teixeira Landi, Adam Hewgill, Brendan Reid, Alessandro Ferraro, Augusto J. Roncaglia, Mauro Antezza

Published Oct 31, 2018• 250 citations
arXivHTMLPDF

Abstract

The study of open quantum systems often relies on approximate master equations derived under the assumptions of weak coupling to the environment. However when the system is made of several interacting subsystems such a derivation is in many cases very hard. An alternative method, employed especially in the modeling of transport in mesoscopic systems, consists in using local master equations (LMEs) containing Lindblad operators acting locally only on the corresponding subsystem. It has been shown that this approach however generates inconsistencies with the laws of thermodynamics. In this paper we demonstrate that using a microscopic model of LMEs based on repeated collisions all thermodynamic inconsistencies can be resolved by correctly taking into account the breaking of global detailed balance related to the work cost of maintaining the collisions. We provide examples based on a chain of quantum harmonic oscillators whose ends are connected to thermal reservoirs at different temperatures. We prove that this system behaves precisely as a quantum heat engine or refrigerator, with properties that are fully consistent with basic thermodynamics.

DOI
10.1088/1367-2630/aaecee

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The study of open quantum systems often relies on approximate master equations derived under the assumptions of weak coupling to the environment. However when the system is made of several interacting subsystems such a derivation is in many cases very hard. An alternative method, employed especially in the modeling of transport in mesoscopic systems, consists in using local master equations (LMEs) containing Lindblad operators acting locally only on the corresponding subsystem. It has been shown that this approach however generates inconsistencies with the laws of thermodynamics. In this paper we demonstrate that using a microscopic model of LMEs based on repeated collisions all thermodynamic inconsistencies can be resolved by correctly taking into account the breaking of global detailed balance related to the work cost of maintaining the collisions. We provide examples based on a chain of quantum harmonic oscillators whose ends are connected to thermal reservoirs at different temperatures. We prove that this system behaves precisely as a quantum heat engine or refrigerator, with properties that are fully consistent with basic thermodynamics.
Master equations under appropriate assumptions are efficient tools for the study of open quantum systems. For many-body systems, subsystems of which locally couple to thermal baths and weakly interact with each other, the local approach provides a more convenient description than the global approach. However, these local master equations are believed to generate inconsistencies with the laws of thermodynamics when intersubsystem interactions exist. Here we develop an alternative local master equation by virtue of similar approximations used in deriving the traditional Gorini-Kossakowski-Lindblad-Sudarshan master equation. In particular, we stick to using eigenstates of each subsystem to construct quantum jump operators, and the secular approximation is also employed to modify the intersubsystem interactions. Our results show that violations of thermodynamic laws will be avoided after correcting intersubsystem interactions. Finally, we study a two-qubit heat transfer model and this further shows the validity of our modified master equation.
We investigate the dynamics of a qubit chain locally coupled to a thermal reservoir, modeled through repeated collisions with particles drawn from a heat bath. Under suitable conditions, the resulting Lindblad equation is thermodynamically consistent -- it drives the system toward thermal equilibrium -- while remaining local at short times. This framework reveals a crossover between the global Lindblad equation derived from the secular approximation in weak-coupling theory and the local dissipative models often employed in the literature, which generally fail to ensure thermodynamic consistency.
Local master equations are a widespread tool to model open quantum systems, especially in the context of many-body systems.These equations, however, are believed to lead to thermodynamic anomalies and violation of the laws of thermodynamics.In contrast, here we rigorously prove that local master equations are consistent with thermodynamics and its laws without resorting to a microscopic model, as done in previous works.In particular, we consider a quantum system in contact with multiple baths and identify the relevant contributions to the total energy, heat currents, and entropy production rate.We show that the second law of thermodynamics holds when one considers the proper expression we derive for the heat currents.We confirm the results for the quantum heat currents by using a heuristic argument that connects the quantum probability currents with the energy currents, using an analogous approach as in classical stochastic thermodynamics.We finally use our results to investigate the thermodynamic properties of a set of quantum rotors operating as thermal devices and show that a suitable design of three rotors can work as an absorption refrigerator or a thermal rectifier.For the machines considered here, we also perform an optimization of the system parameters using an algorithm of reinforcement learning.
The study of quantum thermodynamics is key to the development of quantum thermal machines. Here we investigate a system of parametrically driven quantum harmonic oscillators coupled to heat baths via a collision model. Using a thermodynamically consistent local master equation, we derive the heat flows and work power of the working device which can operate as an engine or a refrigerator and analyse their instantaneous and averages efficiencies and coefficients of performance. Studying the regimes of both slow and fast driving of the system, we find that an increased driving frequency can lead to a change of functioning to an accelerator or a heater. Finally, we investigate the effect of squeezing one of the thermal baths: it leads to an apparent higher efficiency compared to the corresponding Carnot value of an equilibrium bath with the same temperature and to sustained entanglement between the working substance oscillators in the limit cycle.
Advances in experimental techniques have opened new routes for harnessing non-equilibrium dynamics in mesoscopic quantum systems. In this context, we study the impact of on-site interactions on the transport properties of a continuous quantum thermal machine composed of two coupled oscillators connected to two thermal reservoirs. In the weak system-reservoir coupling regime, where a long-standing debate concerns which reduced description should be preferred, we first show that the Redfield master equation (RME) provides an accurate and unifying framework that interpolates between two well-known limits: the \textit{local} and \textit{global} master equations. By relying on the Hierarchy of Pure States (HOPS), a numerically exact stochastic method, we then explore the full parameter space and show that interactions can be leveraged to tune the efficiency of the thermal machine at high temperatures (while leaving it essentially unchanged at low temperatures), induce non-reciprocal transport under asymmetric reservoir couplings, and generate steady-state entanglement within the junction. We derive expressions for system-bath correlators, such as heat and particle currents, consistently across different frameworks. Our work features on-site interactions to enhance the versatility of quantum thermodynamic junctions and clarifies the role of non-Markovianity and non-linearities in quantum transport.
Abstract There is a current interest in quantum thermodynamics in the context of open quantum systems. An important issue is the consistency of quantum thermodynamics, in particular the second law of thermodynamics, i.e. the flow of heat from a hot reservoir to a cold reservoir. Here recent emphasis has been on composite system and in particular the issue regarding the application of local or global master equations. In order to contribute to this discussion we discuss two cases, namely as an example a single qubit and as a simple composite system two coupled qubits driven by two heat reservoirs at different temperatures, respectively. Applying a global Lindblad master equation approach we present explicit expressions for the heat currents in agreement with the second law of thermodynamics. The analysis is carried out in the Born–Markov approximation. We also discuss issues regarding the possible presence of coherences in the steady state.