Magnetic field compatible circuit quantum electrodynamics with graphene Josephson junctions
James Kroll, Willemijn Uilhoorn, Kian L. van der Enden, Damaz de Jong, Kenji Watanabe, Takashi Taniguchi, Srijit Goswami, Maja C. Cassidy, Leo P. Kouwenhoven
Circuit quantum electrodynamics has proven to be a powerful tool to probe mesoscopic effects in hybrid systems and is used in several quantum computing (QC) proposals that require a transmon qubit able to operate in strong magnetic fields. To address this we integrate monolayer graphene Josephson junctions into microwave frequency superconducting circuits to create graphene based transmons. Using dispersive microwave spectroscopy we resolve graphene's characteristic band dispersion and observe coherent electronic interference effects confirming the ballistic nature of our graphene Josephson junctions. We show that the monoatomic thickness of graphene renders the device insensitive to an applied magnetic field, allowing us to perform energy level spectroscopy of the circuit in a parallel magnetic field of 1 T, an order of magnitude higher than previous studies. These results establish graphene based superconducting circuits as a promising platform for QC and the study of mesoscopic quantum effects that appear in strong magnetic fields.
Circuit quantum electrodynamics has proven to be a powerful tool to probe mesoscopic effects in hybrid systems and is used in several quantum computing (QC) proposals that require a transmon qubit able to operate in strong magnetic fields. To address this we integrate monolayer graphene Josephson junctions into microwave frequency superconducting circuits to create graphene based transmons. Using dispersive microwave spectroscopy we resolve graphene's characteristic band dispersion and observe coherent electronic interference effects confirming the ballistic nature of our graphene Josephson junctions. We show that the monoatomic thickness of graphene renders the device insensitive to an applied magnetic field, allowing us to perform energy level spectroscopy of the circuit in a parallel magnetic field of 1 T, an order of magnitude higher than previous studies. These results establish graphene based superconducting circuits as a promising platform for QC and the study of mesoscopic quantum effects that appear in strong magnetic fields.
The technology of quantum computing is believed to solve certain computational problems significantly faster than classical computers, enabling classically inaccessible problems. However, the technology is still in its infancy and it is still too early to conclude which physical system(s) will form the basis of tomorrow's quantum computer. Small-scale quantum processors, built on the superconducting transmon qubit, demonstrated already the anticipated quantum speed-up. Despite this tremendous milestone, scaling up to a full-fledged quantum computer is far from trivial: with these qubits, the flux-control causes crosstalk between qubits and heating, the room-temperature microwave control is hardly scalable and comes with high energetic radiation, and most importantly, the loss of quantum information in time leads to computational errors. Recent advances in various hybrid semiconductor materials enabled novel voltage-controlled transmons, gatemons, which are less susceptible to heating and crosstalk. Even more exciting, gatemons can be designed to host Majorana zero modes in a way that renders the qubit inherently protected against decoherence. In order to induce Majorana zero modes in such nanowire systems strong magnetic fields are required. Problematically, magnetic fields destroy the superconductivity that these microwave circuits rely on. In this thesis we integrate three types of hybrid Josephson junctions in magnetic field compatible microwave devices. Chapter 4 demonstrates the first graphene-based transmon. Due to the mono-atomic thickness of graphene in combination with magnetic field resilient coplanar waveguide resonators, we are able to operate the transmon circuit at an in-plane magnetic field of 1 Tesla. Chapter 5 embeds an InAs-Al semiconducting nanowire Josephson junction in a high quality factor superconducting transmission line resonator, demonstrating on-chip microwave generation. The gate-controllable semiconducting platform lends itself for fast pulse control, providing a perspective for the coherent on-chip manipulation of artificial two-level systems, in particular superconducting qubits such as transmons. Chapter 6 continues the development of InAs-Al nanowire transmons. The offset-charge-sensitive regime, additional plunger gates and magnetic field compatibility prepares the platform for the detection of coherent coupling between Majorana zero modes, a phenomena which unfortunately still remains unobserved. Additionally, we realise the first InSb-Al gatemon. The higher spin-orbit coupling makes InSb to be a preferred material in the search for Majorana signatures. Chapter 7 reports on the dynamics of quasiparticle tunneling events in real-time across the InAs-Al nanowire junction in a transmon architecture. The magnetic field compatibility of our device up to 1 Tesla together with in-situ voltage-controlled quasiparticle trap engineering, allows us to measure the survival of the charge-parity lifetime up to strong magnetic fields. A result which is extremely important in the research field of topological quantum computing, where the qubit space is defined in the charge-parity.
Josephson junctions (JJ) are a fundamental component of microwave quantum circuits, such as tunable cavities, qubits, and parametric amplifiers. Recently developed encapsulated graphene JJs, with supercurrents extending over micron distance scales, have exciting potential applications as a new building block for quantum circuits. Despite this, the microwave performance of this technology has not been explored. Here, we demonstrate a microwave circuit based on a ballistic graphene JJ embedded in a superconducting cavity. We directly observe a gate-tunable Josephson inductance through the resonance frequency of the device and, using a detailed RF model, we extract this inductance quantitatively. We also observe the microwave losses of the device, and translate this into sub-gap resistances of the junction at μeV energy scales, not accessible in DC measurements. The microwave performance we observe here suggests that graphene Josephson junctions are a feasible platform for implementing coherent quantum circuits.
Integrating two-dimensional (2D) materials into circuit quantum electrodynamics (cQED) devices is an emerging field in recent years. This integration not only facilitates the exploration of potential applications in quantum information processing but also enables the study of material's fundamental properties using microwave techniques. While most studies employ 2D coplanar architectures with scalability potential, three-dimensional (3D) cavity-based cQED devices, due to their simpler design, offer the advantage of a quicker turnaround to probe the composite Josephson junctions (JJs). Here, we construct the first flux-tunable, 3D cavity-compatible superconducting quantum circuit based on 2D materials, featuring a graphene superconducting quantum interference device (SQUID) shunted by a capacitor that is accessible by both dc and microwave probes. We have shown how flux-modulated cavity frequency can be linked to the SQUID critical current under the influence of Fraunhofer's pattern. In addition, we extracted the symmetry information of the SQUIDs based on dc analysis, and correlated this with the flux-modulated cavity frequency observed in microwave measurements. Our platform can extend to topological materials, holding the prospect of establishing valid topological JJs with a dc probe while allowing a fast microwave probe to avoid quasiparticle poisoning.
Majorana bound states (MBSs) are novel particles predicted to be created when superconductor/semiconductor hybrid structures with strong spin-orbit coupling are subjected to strong magnetic fields. Expected to exhibit non-Abelian exchange statistics, they could form the basis of a new kind of quantum computer that is inherently protected from environmental noise, a common problem that has frustrated other quantum computing platforms. The current techniques used to measure these particles are highly sensitive, having provided the best evidence yet for their existence, but they are intrinsically too slow to form the basis of a useful quantum computer. To remedy this, this thesis integrates exotic materials into high frequency superconducting circuits that have been engineered to be resilient to strong magnetic fields, creating hybrid devices that potentially allow for fast and precise measurement and control of MBSs and their properties. Several proposals to demonstrate the novel exchange statistics of MBSs use a specific type of superconducting qubit, the `transmon', for fast readout of the state of the MBSs. Problematically, the strong magnetic fields required to induce MBSs would destroy the superconductivity traditional transmons rely on, preventing them from operating as intended. To resolve this, the key constituent components of the transmon, the superconducting resonator and the Josephson junction have been engineered separately to become resilient to strong magnetic fields. Chapter 4 explores how nanofabrication techniques and careful consideration of the properties of thin superconducting films can be used to engineer superconducting co-planar waveguide resonators that remain operational in strong parallel magnetic fields of \\SI{6}{\\tesla} and perpendicular magnetic fields of \\SI{20}{\\milli \\tesla}, an order of magnitude greater than previously reported. Building on the results of Chapter 4, Chapter 5 utilises a graphene based Josephson junction, where the monoatomic thickness of the graphene provides an inherent protection against parallel magnetic fields, allowing us to demonstrate operation of a transmon circuit at a parallel magnetic field of \\SI{1}{\\tesla}. Advances in nanowire material growth intended to improve the signatures of MBS are used in Chapter 6 to create a low power, highly coherent on-chip microwave source. With broad potential applications in superconducting circuits, it demonstrates a platform well suited for the detection of unique radiation that MBSs are predicted to emit. The thesis is concluded by Chapter 7, which describes the engineering and development of a nanowire based transmon qubit capable of measuring key properties of MBSs in the qubit's energy spectrum.
Controlling the energy spectrum of quantum-coherent superconducting circuits, i.e., the energies of excited states, the circuit anharmonicity, and the states' charge dispersion, is essential for designing performant qubits. This control is usually achieved by adjusting the circuit's geometry. In situ control is traditionally obtained via an external magnetic field, in the case of tunnel Josephson junctions. More recently, semiconductor-weak-links-based Josephson junctions have emerged as an alternative building block with the advantage of tunability via the electric-field effect. Gate-tunable Josephson junctions have been succesfully integrated in superconducting circuits using, for instance, semiconducting nanowires or two-dimensional electron gases. In this Letter we demonstrate, in a graphene superconducting circuit, a large gate tunability of qubit properties: frequency, anharmonicity, and charge dispersion. We rationalize these features using a model considering the transmission of Cooper pairs through Andreev bound states. Noticeably, we show that the high transmission of Cooper pairs in such weak link strongly suppresses the charge dispersion. Our Letter illustrates the potential for graphene-based qubits as versatile building blocks in advanced quantum circuits.
Quantum computers promise to solve certain problems such as quantum chemistry simulations much more efficiently than their classical counterparts. Although it is still unclear what material system will ultimately host large-scale quantum computers, solid-state systems are promising candidates due to their inherent scalability and advanced fabrication techniques that can be adapted from comparable technologies. Crucially, a future quantum computer will depend on the quality of its most fundamental building block, the quantum bit, or qubit. Qubits, although ideally insensitive to potential noise, are very susceptible to slight changes in their environment. Therefore, they do not only make the building block for quantum computers, but are also precise sensors. One of the most studied solid-state implementations of a qubit is the transmon, a weakly anharmonic oscillator based on superconducting capacitive and nonlinear inductive elements. Typically, Al-AlOx-Al superconductor-insulator-superconductor Josephson junctions are used for the latter. The interaction of the transmon with the control circuitry, typically superconducting resonators, is described by circuit quantum electrodynamics. In this PhD thesis, a more recently demonstrated type of qubit is further developed and studied in detail using circuit quantum electrodynamics. In these qubits, the Josephson element of the transmon is replaced with indium arsenide nanowires, forming a superconductor-normal metalsuperconductor junction. In addition to the standard flux tunability, these qubits can also be voltage tuned. Due to the compatibility of all the materials used with an applied magnetic field, this type of qubit is a good candidate to be used as a precise and accurate sensor in a magnetic field. The goal of this work is to introduce the in-plane magnetic field as a new tuning knob to the toolbox of circuit quantum electrodynamics. Advances in material science, especially the epitaxial growth of an aluminum shell directly on the indium arsenide nanowire, have enabled the fabrication of nanowire transmons with state-of-the-art coherence. An understanding of their workings in a zero-field environment is important before applying a magnetic field. Thus, we characterize the noise these qubits are subject to (Chapter 4) and find a strong coupling of charge two-level systems to their Josephson energy next to the expected weakly coupled flux and voltage noise. Applying a magnetic field reveals that coherence in these qubits can be observed up to 70 mT, substantially above the superconducting gap of bulk aluminum (Chapter 5). Effects limiting the performance include the thick and fully covering aluminum shell, and the alignment and stability of the magnetic field. The use of different nanowires, the installation of a persistent-current vector solenoid and additional magnetic shielding then enables the operation of voltage- and flux-tunable devices in a magnetic field (Chapter 6). This constitutes a good starting point for circuit quantum electrodynamics experiments in a magnetic field, such as the investigation of the microscopic origin of flux-noise.