Quantum computers promise to solve certain problems such as quantum chemistry simulations much more efficiently than their classical counterparts. Although it is still unclear what material system will ultimately host large-scale quantum computers, solid-state systems are promising candidates due to their inherent scalability and advanced fabrication techniques that can be adapted from comparable technologies. Crucially, a future quantum computer will depend on the quality of its most fundamental building block, the quantum bit, or qubit. Qubits, although ideally insensitive to potential noise, are very susceptible to slight changes in their environment. Therefore, they do not only make the building block for quantum computers, but are also precise sensors. One of the most studied solid-state implementations of a qubit is the transmon, a weakly anharmonic oscillator based on superconducting capacitive and nonlinear inductive elements. Typically, Al-AlOx-Al superconductor-insulator-superconductor Josephson junctions are used for the latter. The interaction of the transmon with the control circuitry, typically superconducting resonators, is described by circuit quantum electrodynamics. In this PhD thesis, a more recently demonstrated type of qubit is further developed and studied in detail using circuit quantum electrodynamics. In these qubits, the Josephson element of the transmon is replaced with indium arsenide nanowires, forming a superconductor-normal metalsuperconductor junction. In addition to the standard flux tunability, these qubits can also be voltage tuned. Due to the compatibility of all the materials used with an applied magnetic field, this type of qubit is a good candidate to be used as a precise and accurate sensor in a magnetic field. The goal of this work is to introduce the in-plane magnetic field as a new tuning knob to the toolbox of circuit quantum electrodynamics. Advances in material science, especially the epitaxial growth of an aluminum shell directly on the indium arsenide nanowire, have enabled the fabrication of nanowire transmons with state-of-the-art coherence. An understanding of their workings in a zero-field environment is important before applying a magnetic field. Thus, we characterize the noise these qubits are subject to (Chapter 4) and find a strong coupling of charge two-level systems to their Josephson energy next to the expected weakly coupled flux and voltage noise. Applying a magnetic field reveals that coherence in these qubits can be observed up to 70 mT, substantially above the superconducting gap of bulk aluminum (Chapter 5). Effects limiting the performance include the thick and fully covering aluminum shell, and the alignment and stability of the magnetic field. The use of different nanowires, the installation of a persistent-current vector solenoid and additional magnetic shielding then enables the operation of voltage- and flux-tunable devices in a magnetic field (Chapter 6). This constitutes a good starting point for circuit quantum electrodynamics experiments in a magnetic field, such as the investigation of the microscopic origin of flux-noise.
Quantum computers promise to solve certain problems such as quantum chemistry simulations much more efficiently than their classical counterparts. Although it is still unclear what material system will ultimately host large-scale quantum computers, solid-state systems are promising candidates due to their inherent scalability and advanced fabrication techniques that can be adapted from comparable technologies. Crucially, a future quantum computer will depend on the quality of its most fundamental building block, the quantum bit, or qubit. Qubits, although ideally insensitive to potential noise, are very susceptible to slight changes in their environment. Therefore, they do not only make the building block for quantum computers, but are also precise sensors. One of the most studied solid-state implementations of a qubit is the transmon, a weakly anharmonic oscillator based on superconducting capacitive and nonlinear inductive elements. Typically, Al-AlOx-Al superconductor-insulator-superconductor Josephson junctions are used for the latter. The interaction of the transmon with the control circuitry, typically superconducting resonators, is described by circuit quantum electrodynamics. In this PhD thesis, a more recently demonstrated type of qubit is further developed and studied in detail using circuit quantum electrodynamics. In these qubits, the Josephson element of the transmon is replaced with indium arsenide nanowires, forming a superconductor-normal metalsuperconductor junction. In addition to the standard flux tunability, these qubits can also be voltage tuned. Due to the compatibility of all the materials used with an applied magnetic field, this type of qubit is a good candidate to be used as a precise and accurate sensor in a magnetic field. The goal of this work is to introduce the in-plane magnetic field as a new tuning knob to the toolbox of circuit quantum electrodynamics. Advances in material science, especially the epitaxial growth of an aluminum shell directly on the indium arsenide nanowire, have enabled the fabrication of nanowire transmons with state-of-the-art coherence. An understanding of their workings in a zero-field environment is important before applying a magnetic field. Thus, we characterize the noise these qubits are subject to (Chapter 4) and find a strong coupling of charge two-level systems to their Josephson energy next to the expected weakly coupled flux and voltage noise. Applying a magnetic field reveals that coherence in these qubits can be observed up to 70 mT, substantially above the superconducting gap of bulk aluminum (Chapter 5). Effects limiting the performance include the thick and fully covering aluminum shell, and the alignment and stability of the magnetic field. The use of different nanowires, the installation of a persistent-current vector solenoid and additional magnetic shielding then enables the operation of voltage- and flux-tunable devices in a magnetic field (Chapter 6). This constitutes a good starting point for circuit quantum electrodynamics experiments in a magnetic field, such as the investigation of the microscopic origin of flux-noise.
The technology of quantum computing is believed to solve certain computational problems significantly faster than classical computers, enabling classically inaccessible problems. However, the technology is still in its infancy and it is still too early to conclude which physical system(s) will form the basis of tomorrow's quantum computer. Small-scale quantum processors, built on the superconducting transmon qubit, demonstrated already the anticipated quantum speed-up. Despite this tremendous milestone, scaling up to a full-fledged quantum computer is far from trivial: with these qubits, the flux-control causes crosstalk between qubits and heating, the room-temperature microwave control is hardly scalable and comes with high energetic radiation, and most importantly, the loss of quantum information in time leads to computational errors. Recent advances in various hybrid semiconductor materials enabled novel voltage-controlled transmons, gatemons, which are less susceptible to heating and crosstalk. Even more exciting, gatemons can be designed to host Majorana zero modes in a way that renders the qubit inherently protected against decoherence. In order to induce Majorana zero modes in such nanowire systems strong magnetic fields are required. Problematically, magnetic fields destroy the superconductivity that these microwave circuits rely on. In this thesis we integrate three types of hybrid Josephson junctions in magnetic field compatible microwave devices. Chapter 4 demonstrates the first graphene-based transmon. Due to the mono-atomic thickness of graphene in combination with magnetic field resilient coplanar waveguide resonators, we are able to operate the transmon circuit at an in-plane magnetic field of 1 Tesla. Chapter 5 embeds an InAs-Al semiconducting nanowire Josephson junction in a high quality factor superconducting transmission line resonator, demonstrating on-chip microwave generation. The gate-controllable semiconducting platform lends itself for fast pulse control, providing a perspective for the coherent on-chip manipulation of artificial two-level systems, in particular superconducting qubits such as transmons. Chapter 6 continues the development of InAs-Al nanowire transmons. The offset-charge-sensitive regime, additional plunger gates and magnetic field compatibility prepares the platform for the detection of coherent coupling between Majorana zero modes, a phenomena which unfortunately still remains unobserved. Additionally, we realise the first InSb-Al gatemon. The higher spin-orbit coupling makes InSb to be a preferred material in the search for Majorana signatures. Chapter 7 reports on the dynamics of quasiparticle tunneling events in real-time across the InAs-Al nanowire junction in a transmon architecture. The magnetic field compatibility of our device up to 1 Tesla together with in-situ voltage-controlled quasiparticle trap engineering, allows us to measure the survival of the charge-parity lifetime up to strong magnetic fields. A result which is extremely important in the research field of topological quantum computing, where the qubit space is defined in the charge-parity.
A practical quantum computer demands a physical quantum bit (qubit) that is scalable, has a well-defined initial state, and brings together coherence with reliable control and read-out. A compelling idea is to put together a locally protected Majorana qubit with a superconducting qubit. The superconducting qubit is used to read out the Majorana states while the Majorana qubit may act as a quantum memory. This thesis presents a series of studies on quantum transport in semiconducting nanowires coupled to superconductors to investigate various platforms for realizing Majorana. These studies are followed by microwave measurements on superconducting circuits compatible with semiconducting-superconducting heterostructures. We first evaluate the potential of Ge/Si core/shell nanowires by achieving induced superconductivity as well as estimating spin-orbit coupling. Next we explore the transport mediated by Andreev bound states formed in InSb nanowire quantum. A subgap negative differential conductance is investigated together with the coalescing Andreev resonances at zero bias relevant for the correct interpretation of Majorana experiments done on the same structures. We conclude our studies of semiconducting nanowires by exploring tunnel junctions in Sn-InSb nanowires that are prepared by in-situ shadowing using nearby nanowires and flakes. Tin shells are found to induce a hard superconducting gap persisting up to high magnetic fields. We observe the two-electron charging effect from a small superconducting island of Sn-InSb. This effect is attributed to charge parity stability, which makes this nanowire system an intriguing candidate for superconducting and topological quantum circuits. These Sn-InSb junctions are then used as the nonlinear element in a transmon qubit design where we observe a dispersive coupling between this nanowire Josephson junction and a superconducting resonator. We also present our progress towards building a magnetic field resilient superconducting circuit that allows integration with semiconducting and topological structures. In the last chapter, InSb semiconducting nanowires are utilized as shadow masks prior to superconductor deposition on an InAs quantum well. We study Josephson current properties in Josephson junctions made from these nanowire shadows. Our results point to highly transparent junctions that can be developed further for hybrid superconductor-semiconductor qubit systems.
Majorana bound states (MBSs) are novel particles predicted to be created when superconductor/semiconductor hybrid structures with strong spin-orbit coupling are subjected to strong magnetic fields. Expected to exhibit non-Abelian exchange statistics, they could form the basis of a new kind of quantum computer that is inherently protected from environmental noise, a common problem that has frustrated other quantum computing platforms. The current techniques used to measure these particles are highly sensitive, having provided the best evidence yet for their existence, but they are intrinsically too slow to form the basis of a useful quantum computer. To remedy this, this thesis integrates exotic materials into high frequency superconducting circuits that have been engineered to be resilient to strong magnetic fields, creating hybrid devices that potentially allow for fast and precise measurement and control of MBSs and their properties. Several proposals to demonstrate the novel exchange statistics of MBSs use a specific type of superconducting qubit, the `transmon', for fast readout of the state of the MBSs. Problematically, the strong magnetic fields required to induce MBSs would destroy the superconductivity traditional transmons rely on, preventing them from operating as intended. To resolve this, the key constituent components of the transmon, the superconducting resonator and the Josephson junction have been engineered separately to become resilient to strong magnetic fields. Chapter 4 explores how nanofabrication techniques and careful consideration of the properties of thin superconducting films can be used to engineer superconducting co-planar waveguide resonators that remain operational in strong parallel magnetic fields of \\SI{6}{\\tesla} and perpendicular magnetic fields of \\SI{20}{\\milli \\tesla}, an order of magnitude greater than previously reported. Building on the results of Chapter 4, Chapter 5 utilises a graphene based Josephson junction, where the monoatomic thickness of the graphene provides an inherent protection against parallel magnetic fields, allowing us to demonstrate operation of a transmon circuit at a parallel magnetic field of \\SI{1}{\\tesla}. Advances in nanowire material growth intended to improve the signatures of MBS are used in Chapter 6 to create a low power, highly coherent on-chip microwave source. With broad potential applications in superconducting circuits, it demonstrates a platform well suited for the detection of unique radiation that MBSs are predicted to emit. The thesis is concluded by Chapter 7, which describes the engineering and development of a nanowire based transmon qubit capable of measuring key properties of MBSs in the qubit's energy spectrum.
We present an experimental study of flux- and gate-tunable nanowire transmons with state-of-the-art relaxation time allowing quantitative extraction of flux and charge noise coupling to the Josephson energy. We evidence coherence sweet spots for charge, tuned by voltage on a proximal side gate, where first order sensitivity to switching two-level systems and background 1/f noise is minimized. Next, we investigate the evolution of a nanowire transmon in a parallel magnetic field up to 70 mT, the upper bound set by the closing of the induced gap. Several features observed in the field dependence of qubit energy relaxation and dephasing times are not fully understood. Using nanowires with a thinner, partially covering Al shell will enable operation of these circuits up to 0.5 T, a regime relevant for topological quantum computation and other applications.
Superconducting quantum computing is a solid state quantum computing technology based on Josephson junction circuits. It becomes one of the most promising candidates for realizing practical quantum computer/simulator, because of its scalability, easy to coupling and control, compatibility to semiconductor technologies, etc. As the complicated electromagnetic environment in solid state metal and insulator, superconducting quantum bits (qubits) suffered from shot coherence time since its early development. In this review, we described some recently developed superconducting qubit structures, including Transmon/Xmon, Fluxonium and C-shunt flux qubit. Although these new qubit structures have very different circuit parameters and energy scales, they all find their way to effectively suppress environmental noises. As a result, their coherence time were improved significantly. Transmon, a transmission-line shunted plasma oscillation qubit, was now among the most popular structures for building a multi-qubit superconducting quantum circuit. It introduced a relatively large shunt capacitor to remarkably reduce the charge dispersion. Although the non-linearity is also decreased, by operating in a properly chosen EJ/Ec, transmon can greatly reduce the charge noise while only sacrificing a small amount of non-linearity. Xmon can be considered as a modified version of transmon. It is designed and optimized for multi-qubit operation and measurement with separate X/Y and Z control lines for each qubit, and a readout bus (a transmission line or a low-Q bandpass filter) for simultaneous readout of all the qubits. Fluxonium provide another solution for suppressing the charge noise in Cooper-pair box (CPB). It introduces a large shunt inductance to filter low-frequency offset charge in the small capacitor of the phase-slip junction (the small junction). To keep the qubit operating in the charge region, the shunt inductor should be large enough to keep the impedance larger than the superconducting impedance quantum RQ~1 kΩ. As a result, the inductance can only be provided by a large series of Josephson junctions. Fluxonium keeps the advantage of high anharmonicity of CPB. In addition, it introduces another degree of freedom: external flux Φext. Quasiparticles (electrons or holes) tunneling at the small junction add coherently to produce a ″1+cosφ″ term. As a result, when Φext= Φ0/2, dissipation caused by quasiparticle tunneling is suppressed and the energy relaxation time (T1) increases drastically. C-shunt flux qubit (CSFQ) decreases α and EJ to suppress flux noise in the qubit. While the charge noise becomes the dominant noise source, a large shunt capacitor is added to suppress the charge noise, similar to that in a transmon qubit. It is worth to notice that in CSFQ, the α decreases to below but near 1/2. As a result, the double-well potential no longer exists. The energy structure become similar to transmon, with the anharmonicity be opposite. CSFQ can get a much improved coherence time, while its anharmonicity can be larger than that of transmon. Those new superconducting qubit structures provide different solutions to improve the coherence time. Although it looks much different in circuit models and parameters, they have ideas in common, and may act as guides to other novel designs with longer coherence time. We can summarize as below. (1) The qubit circuit should be free of small superconducting islands. Charge fluctuation in small islands is a major source of decoherence. As a result, increase the area of the islands, that is, increase the capacitance becomes a straight forward way to suppress the charge noise. In Fluxonium, the small junction is connected with a large series of large junctions that there is also no small islands in the whole loop. (2) Remove superconducting loops in the qubit circuit, or minimize the loop size and loop current to suppress flux noise. (3) Bias the phase difference of the small junction to π, where dissipation caused by quasiparticle tunneling can be suppressed coherently. (4) Decrease the coupling bandwidth of qubit to the environment. In a circuit-QED readout scheme, a high-Q readout resonator that dispersively coupled to the qubit protects the qubit from exposed to the electromagnetic environment of the readout circuit. A ″Purcell filter″ can also be added to suppress such decoherence further. In conclusion, we overviewed some qubit engineering techniques or ideas to improve the coherence time, which is a very important figure for building practical quantum computer/simulator. We hope that someone can combine and optimize these ideas, while interact with developments in materials and micro-fabrication technologies, to develop novel new generation superconducting qubit structures in the near future.
Superconductor qubits typically use aluminum–aluminum oxide tunnel junctions to provide the nonlinear inductance. Junctions with semiconductor barriers make it possible to vary the superconductor material and explore beyond aluminum. We use InAs semiconductor nanowires coated with thin superconducting shells of β-Sn to realize transmon qubits. By tuning the Josephson energy with a gate voltage, we adjust the qubit frequency over a range of 3 GHz. The longest energy relaxation time, T 1 = 27 μs, is obtained at the lowest qubit frequencies, while the longest echo dephasing time, T 2 = 1.8 μs, is achieved at higher frequencies. We assess the possible factors limiting coherence times in these devices and discuss steps to enhance performance through improvements in materials fabrication and circuit design.