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arXiv:1806.06322 · Physical Review A

Exotic dynamical evolution in a secant-pulse-driven quantum system

Pengju Zhao, Wei Li, Hong Cao, Shao-Wu Yao, Li-Xiang Cen

Published Aug 28, 2018• 7 citations
arXivHTMLPDF

Abstract

We investigate an explicitly time-dependent quantum system driven by a secant-pulse external field. By solving the Schr\"odinger equation exactly, we elucidate exotic properties of the system with respect to its dynamical evolution: On the one hand, the system is shown to be essentially nonadiabatic, which prohibits an adiabatic approximation for its dynamics; on the other hand, the loop evolution of the model can induce a geometric phase which, analogous to the Berry phase of the cyclic adiabatic evolution, is in direct proportion to the solid angle subtended by the path of the state vector. Moreover, we extend the model and show that the described properties coincide in a special family of secant-pulse-driven models.

DOI
10.1103/physreva.98.022136

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We investigate an explicitly time-dependent quantum system driven by a secant-pulse external field. By solving the Schr"odinger equation exactly, we elucidate exotic properties of the system with respect to its dynamical evolution: On the one hand, the system is shown to be essentially nonadiabatic, which prohibits an adiabatic approximation for its dynamics; on the other hand, the loop evolution of the model can induce a geometric phase which, analogous to the Berry phase of the cyclic adiabatic evolution, is in direct proportion to the solid angle subtended by the path of the state vector. Moreover, we extend the model and show that the described properties coincide in a special family of secant-pulse-driven models.
In this work we present a simple and elegant approach to study the adiabatic and nonadiabatic evolution of a generalized damped harmonic oscillator which is described by the generalized Caldirola–Kanai Hamiltonian, in both classical and quantum contexts. Based on time-dependent dynamical invariants, we find that the geometric phase acquired when the damped oscillator evolves adiabatically in time provides a direct connection between the classical Hannay’s angle and the quantum Berry’s phase. In addition, we solve the time-dependent Schrödinger equation for this system and calculate various quantum properties of the damped generalized harmonic one, such as coherent states, expectation values of the position and momentum operators, their quantum fluctuations and the associated uncertainty product.
Exact solution to the driven quantum system with an explicitly time-dependent Hamiltonian is not only an issue of fundamental importance to quantum mechanics itself, but also a ubiquitous problem in the design for quantum control. In particular, the nonadiabatic transition induced by the time-dependent external field is often involved in order to target the quantum state for the atomic and molecular systems. In this paper we investigate the exact dynamics and the associated nonadiabatic transition in a typical driven model, the Rosen-Zener model and its multi-level extension, by virtue of the algebraic dynamical method. Previously, this kind of driven models, especially of the two-level case, were solved by converting the corresponding Schrödinger equation to a hypergeometric equation. The property of the dynamical transition of the system was then achieved by the asymptotic behavior of the yielded hypergeometric function. A critical drawback related to such methods is that they are very hard to be developed so as to treat the multi-level extension of the driven model. Differing from the above mentioned method, we demonstrate that the particular kind of the Rosen-Zener model introduced here could be solved analytically via a canonical transformation or a gauge transformation approach. In comparison, we show that the present method at least has two aspects of advantages. Firstly, the method enables one to describe the evolution of the wavefunction of the system analytically over any time interval of the pulse duration. Moreover, we show that the method could be exploited to deal with the multi-level extensions of the model. The explicit expression of the dynamical basis states, including the three-level system and the four-level system, is presented and the transition probabilities induced by the nonadiabatic evolution among different levels are then characterized for the model during the time evolution. In addition, our study reveals further that the dual model of the driven system can be constructed. Since the dynamical invariant of a solvable system can always be obtained within the framework of the algebraic dynamical method, the general connection between the dual model and the original one, including the solvability and their dynamical invariants, are established and characterized distinctly.
We decompose the quantum adiabatic evolution as the products of gauge invariant unitary operators and obtain the exact nonadiabatic correction in the adiabatic approximation. A necessary and sufficient condition that leads to adiabatic evolution with geometric phases is provided and we determine that in the adiabatic evolution, while the eigenstates are slowly varying, the eigenenergies and degeneracy of the Hamiltonian can change rapidly. We exemplify this result by the example of the adiabatic evolution driven by parametrized pulse sequences. For driving fields that are rotating slowly with the same average energy and evolution path, fast modulation fields can have smaller nonadiabatic errors than obtained under the traditional approach with a constant amplitude.
If the time evolution of a quantum state leads back to the initial state, a geometric phase is accumulated that is known as the Berry phase for adiabatic evolution or as the Aharonov-Anandan (AA) phase for nonadiabatic evolution. We evaluate these geometric phases using Floquet theory for systems in time-dependent external fields with a focus on paths leading through a degeneracy of the eigenenergies. Contrary to expectations, the low-frequency limits of the two phases do not always coincide. This happens as the degeneracy leads to a slow convergence of the quantum states to adiabaticity, resulting in a nonzero finite or divergent contribution to the AA phase. Steering the system adiabatically through a degeneracy provides control over the geometric phase as it can cause a π shift of the Berry phase. On the other hand, we revisit an example of degeneracy crossing proposed by AA. We find that, at suitable driving frequencies, both geometric-phase definitions give the same result and the dynamical phase is zero due to the symmetry of time evolution about the point of degeneracy, providing an advantageous setup for manipulation of quantum states.
We decompose the quantum adiabatic evolution as the products of gauge invariant unitary operators and obtain the exact nonadiabatic correction in the adiabatic approximation. A necessary and sufficient condition that leads to adiabatic evolution with geometric phases is provided, and we determine that in the adiabatic evolution, while the eigenstates are slowly varying, the eigenenergies and degeneracy of the Hamiltonian can change rapidly. We exemplify this result by the example of the adiabatic evolution driven by parametrized pulse sequences. For driving fields that are rotating slowly with the same average energy and evolution path, fast modulation fields can have smaller nonadiabatic errors than obtained under the traditional approach with a constant amplitude.