Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1805.06029 · Physical Review A

ac Stark shifts of dark resonances probed with Ramsey spectroscopy

J. W. Pollock, Valeriy I. Yudin, M. Shuker, M. Yu. Basalaev, А. В. Тайченачев, Xiaochi Liu, John E. Kitching, Elizabeth A. Donley

Published Nov 16, 2018• 29 citations
arXivHTMLPDF

Abstract

The off-resonant ac Stark shift for coherent population trapping (CPT) resonances probed with Ramsey spectroscopy is investigated experimentally and theoretically. Measurements with laser-cooled $^{87}\mathrm{Rb}$ atoms show excellent quantitative agreement with a simple theory. The shift depends on the relative intensity of the two CPT light fields, but depends only weakly on the total intensity. Since the origin of the shift is through couplings of the interrogation light to off-resonant excited-state hyperfine levels, the size and sign of the shift depend on the specific interrogation scheme. The theory also shows that for several commonly used interrogation schemes it is possible to minimize the off-resonant light shift or its dependence on the CPT intensity ratio by properly selecting the system parameters.

DOI
10.1103/physreva.98.053424

Related papers

Line shape and light shift of coherent population trapping resonance under Ramsey interrogation in ‘hot’ atoms in an optically dense medium

Г. В. Волошин, К. А. Баранцев, A.N. Litvinov

Abstract A theory is developed for the effect of coherent population trapping (CPT) in ‘hot’ atoms under pulsed pumping in an optically dense medium with a buffer gas. The case is considered when the excited level is not degenerate. Based on an analysis of the shape of Ramsey resonances, we show that with increasing optical density of the medium, the dependence of the light shifts of the CPT resonance becomes more and more nontrivial. The dependence of the light shifts of the CPT resonance on the magnitude of the hyperfine splitting of the excited level, concentration of active atoms, temperature, and duration of the dark pause is constructed.

Quantum Electronics•Feb 1, 2022•7 citations

Investigation on light shift in CPT-Ramsey resonance for compact atomic clocks

Yuichiro Yano, Wujie Gao, Shigeyoshi Goka +1 more

This paper presents a theoretical and experimental investigation on the light shift (AC Stark shift) of the 62S1/2(F = 3 ↔ 4) transition in133Cs, as observed through coherent population trapping (CPT) under a pulsed excitation. The calculated results are good agreement in the experimental results on various parameters and show that the light shift under pulsed excitation is 20∼30 times less than that under continuous excitation. In addition, this paper also presents a two-step pulse method for suppressing the light shift.

Joint Conference of the European Frequency and Time Forum and IEEE International Frequency Control Symposium (EFTF/IFCS)•May 1, 2014•0 citations

ac Stark shift in double resonance and coherent population trapping in a wall-coated cell for compact Rb atomic clocks

D. Miletic, Thejesh Bandi, C. Affolderbach +1 more

We present a comparative study of the light-shifts (ac Stark shift) in a Rb vapour cell using two possible schemes for Rb atomic clocks: double resonance (DR) and coherent population trapping (CPT). For both schemes, the same wall-coated cell in a compact atomic resonator was used. The light-shift resulting from a monochromatic (DR) or a non-monochromatic (CPT) optical excitation was measured as a function of the laser intensity and the laser frequency and compared with existing theoretical results.

Physica Scripta•Apr 27, 2012•5 citations

The Effect of the Hyperfine Structure of an Excited Level on the Shape of the Coherent Population Trapping Resonance under Ramsey Interrogation in an Optically Dense Medium

Г. В. Волошин, К. А. Баранцев, Е. Н. Попов +1 more

Abstract The effect of the hyperfine structure of an excited level on the shape of the coherent population trapping (CPT) resonance under Ramsey interrogation is investigated in media with different optical thicknesses. The shape of the CPT resonance is constructed for optically thin and dense media, and the results are compared. The dependence of the light shift on the optical density of a medium is analyzed. The parameters of the field phases are determined for which the light shift remains constant under fluctuations of the optical thickness of the medium.

Journal of Experimental and Theoretical Physics•Jul 1, 2019•4 citations

Light shift of Double Resonance and Coherent Population Trapping in wall-coated cells for compact Rb clocks

D. Miletic, Thejesh Bandi, C. Affolderbach +1 more

We report on a comparative study on the light shift in two possible clock schemes for vapor-cell standards, Double Resonance (DR) and Coherent Population Trapping (CPT), by using the same wall coated cell and compact atomic resonator. Our experimental setup allowed us to measure and study the AC Stark shift, resulting from a mono-chromatic or a non monochromatic optical excitation. The light-shift was investigated as function of the laser intensity and the laser frequency.

Joint Conference of the European Frequency and Time Forum and IEEE International Frequency Control Symposium (EFTF/IFCS)•May 1, 2011•0 citations

An effective model for describing coherent population trapping resonances, which correctly takes into account the off-resonant frequency components in periodically modulated laser field

Valeriy I. Yudin, M. Yu. Basalaev, A. V. Taichenachev +1 more

We have developed an effective mathematical model to calculate the coherent population trapping (CPT) resonance in periodically modulated light, when the modulation frequency $f$ varies near the fractional part of hyperfine splitting in the ground state $Δ_{\rm hfs}/N$ (where $N=1,2,...$). In such polychromatic field, only two frequency components that are most resonant with atomic optical transitions are taken into account accurately, while all other off-resonant components are taken into account using the second-order perturbation theory in the field. Within the presented concept, equation for atomic density matrix is obtained, in which the contribution of all off-resonant components is reduced to the appearance of two new operators (non-diagonal, in general case): the shift operator and relaxation operators. In the case of three-level $Λ$-system, the adequacy of presented effective model was verified by numerical calculations of various dependencies, in which we did not find visual differences from the exact calculations. In addition to a significant mathematical simplification, our model provides a clear physical picture of various features of CPT spectroscopy in a periodically modulated laser field, including effects that have not been discussed in the scientific literature before. In particular, we show that the widespread viewpoint that the CPT resonance shift is determined by usual ac Stark shifts of the lower levels is, in general, fundamentally incorrect, since the contribution to the light shift due to beats at the frequency $Δ_{\rm hfs}$ between different off-resonant frequency components can be comparable (or even dominate) with the standard ac Stark shift. Therefore, even if we have detailed information on the modulated field spectrum (e.g. using a spectrum analyzer), this is, in general, absolutely insufficient to determine the light shift of CPT resonance.

arXiv:2505.01924•May 3, 2025•0 citations
The off-resonant ac Stark shift for coherent population trapping (CPT) resonances probed with Ramsey spectroscopy is investigated experimentally and theoretically. Measurements with laser-cooled 87Rb^{87}\mathrm{Rb}87Rb atoms show excellent quantitative agreement with a simple theory. The shift depends on the relative intensity of the two CPT light fields, but depends only weakly on the total intensity. Since the origin of the shift is through couplings of the interrogation light to off-resonant excited-state hyperfine levels, the size and sign of the shift depend on the specific interrogation scheme. The theory also shows that for several commonly used interrogation schemes it is possible to minimize the off-resonant light shift or its dependence on the CPT intensity ratio by properly selecting the system parameters.
Abstract A theory is developed for the effect of coherent population trapping (CPT) in ‘hot’ atoms under pulsed pumping in an optically dense medium with a buffer gas. The case is considered when the excited level is not degenerate. Based on an analysis of the shape of Ramsey resonances, we show that with increasing optical density of the medium, the dependence of the light shifts of the CPT resonance becomes more and more nontrivial. The dependence of the light shifts of the CPT resonance on the magnitude of the hyperfine splitting of the excited level, concentration of active atoms, temperature, and duration of the dark pause is constructed.
This paper presents a theoretical and experimental investigation on the light shift (AC Stark shift) of the 62S1/2(F = 3 ↔ 4) transition in133Cs, as observed through coherent population trapping (CPT) under a pulsed excitation. The calculated results are good agreement in the experimental results on various parameters and show that the light shift under pulsed excitation is 20∼30 times less than that under continuous excitation. In addition, this paper also presents a two-step pulse method for suppressing the light shift.
We present a comparative study of the light-shifts (ac Stark shift) in a Rb vapour cell using two possible schemes for Rb atomic clocks: double resonance (DR) and coherent population trapping (CPT). For both schemes, the same wall-coated cell in a compact atomic resonator was used. The light-shift resulting from a monochromatic (DR) or a non-monochromatic (CPT) optical excitation was measured as a function of the laser intensity and the laser frequency and compared with existing theoretical results.
Abstract The effect of the hyperfine structure of an excited level on the shape of the coherent population trapping (CPT) resonance under Ramsey interrogation is investigated in media with different optical thicknesses. The shape of the CPT resonance is constructed for optically thin and dense media, and the results are compared. The dependence of the light shift on the optical density of a medium is analyzed. The parameters of the field phases are determined for which the light shift remains constant under fluctuations of the optical thickness of the medium.
We have developed an effective mathematical model to calculate the coherent population trapping (CPT) resonance in periodically modulated light, when the modulation frequency fff varies near the fractional part of hyperfine splitting in the ground state Δhfs/NΔ_{\rm hfs}/NΔhfs​/N (where N=1,2,...N=1,2,...N=1,2,...). In such polychromatic field, only two frequency components that are most resonant with atomic optical transitions are taken into account accurately, while all other off-resonant components are taken into account using the second-order perturbation theory in the field. Within the presented concept, equation for atomic density matrix is obtained, in which the contribution of all off-resonant components is reduced to the appearance of two new operators (non-diagonal, in general case): the shift operator and relaxation operators. In the case of three-level ΛΛΛ-system, the adequacy of presented effective model was verified by numerical calculations of various dependencies, in which we did not find visual differences from the exact calculations. In addition to a significant mathematical simplification, our model provides a clear physical picture of various features of CPT spectroscopy in a periodically modulated laser field, including effects that have not been discussed in the scientific literature before. In particular, we show that the widespread viewpoint that the CPT resonance shift is determined by usual ac Stark shifts of the lower levels is, in general, fundamentally incorrect, since the contribution to the light shift due to beats at the frequency ΔhfsΔ_{\rm hfs}Δhfs​ between different off-resonant frequency components can be comparable (or even dominate) with the standard ac Stark shift. Therefore, even if we have detailed information on the modulated field spectrum (e.g. using a spectrum analyzer), this is, in general, absolutely insufficient to determine the light shift of CPT resonance.