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arXiv:1804.08526 · Physical Review Letters

Strong Purcell Effect on a Neutral Atom Trapped in an Open Fiber Cavity

J. Gallego, Wolfgang Alt, Tobias Macha, Miguel Martinez-Dorantes, Deepak Pandey, Dieter Meschede

Published Oct 23, 2018• 75 citations
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Abstract

We observe a sixfold Purcell broadening of the D_{2} line of an optically trapped ^{87}Rb atom strongly coupled to a fiber cavity. Under external illumination by a near-resonant laser, up to 90% of the atom's fluorescence is emitted into the resonant cavity mode. The sub-Poissonian statistics of the cavity output and the Purcell enhancement of the atomic decay rate are confirmed by the observation of a strongly narrowed antibunching dip in the photon autocorrelation function. The photon leakage through the higher-transmission mirror of the single-sided resonator is the dominant contribution to the field decay (κ≈2π×50 MHz), thus offering a high-bandwidth, fiber-coupled channel for photonic interfaces such as quantum memories and single-photon sources.

DOI
10.1103/physrevlett.121.173603

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We observe a sixfold Purcell broadening of the D_{2} line of an optically trapped ^{87}Rb atom strongly coupled to a fiber cavity. Under external illumination by a near-resonant laser, up to 90% of the atom's fluorescence is emitted into the resonant cavity mode. The sub-Poissonian statistics of the cavity output and the Purcell enhancement of the atomic decay rate are confirmed by the observation of a strongly narrowed antibunching dip in the photon autocorrelation function. The photon leakage through the higher-transmission mirror of the single-sided resonator is the dominant contribution to the field decay (κ≈2π×50 MHz), thus offering a high-bandwidth, fiber-coupled channel for photonic interfaces such as quantum memories and single-photon sources.
We demonstrate efficient interfacing of individually trapped single atoms to a nanofiber cavity. The cavity is formed by fabricating photonic crystal structures directly on the nanofiber using femtosecond laser ablation. The single atoms are interfaced to the nanofiber cavity using an optical tweezer based side-illumination trapping scheme. We show that the fluorescence of individual single atoms trapped on the nanofiber cavity can be readily observed in real-time through the fiber guided modes. From the photon statistics measured for different cavity decay rates, the effective coupling rate of the atom-cavity interface is estimated to be 34±2 MHz. This yields a cooperativity of 5.4±0.6 (Purcell factor=6.4±0.6) and a cavity enhanced channeling efficiency as high as 85±2% for a cavity mode with a finesse of 140. The trap lifetime is measured to be 52±5 ms. These results may open new possibilities for deterministic preparation of single atom events for quantum photonics applications on an all-fiber platform.
High-bandwidth, fiber-based optical cavities are a promising building block for future quantum networks. They are used to resonantly couple stationary qubits such as single or multiple atoms with photons routing quantum information into a fiber network at high rates. In high-bandwidth cavities, standard fluorescence imaging on the atom-cavity resonance line for controlling atom positions is impaired since the Purcell effect strongly suppresses all-directional fluorescence. Here, we restore imaging of 87Rb^{87}\mathrm{Rb}87Rb atoms strongly coupled to such a fiber Fabry-P\'erot cavity by detecting the repumper fluorescence which is generated by continuous and three-dimensional Raman sideband cooling. We have carried out a detailed spectroscopic investigation of the repumper-induced differential light shifts affecting the Raman resonance, dependent on intensity and detuning. Our analysis identifies a compromise regime between imaging signal-to-noise ratio and survival rate, where physical insight into the role of dipole-force fluctuations in the heating dynamics of trapped atoms is gained.
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The radiative properties of atoms inside an optical cavity can be dramatically changed with respect to those in free space. In the strong-coupling limit, the reversible dipole interaction between an atom and the cavity field dominates the irreversible decay resulting from spontaneous emission and cavity damping. In this limit the atom and field can no longer be regarded as separate quantities but instead form a composite dynamic system. To enhance the dipole coupling constant and increase the photon storage time, our experiments are performed with a small cavity 1 mm long, with a finesse of 8 × 104. On average, 0.4 photons are sufficient to saturate the resonance transition at 852 nm for the cesium atoms used, while the cooperativity parameter for a single atom is 2. Optical bistability is studied in this system over the range 3 < N < 65 atoms inside the cavity, with the semiclassical theory predicting bistability for N > 5. We report observations of manifestly quantum effects in this regime, including photon antibunching and sub-Poissonian photon statistics, with the magnitude of these nonclassical effects observed to be largely independent of the number of intracavity atoms.
We study the behavior of a single laser-driven trapped ion inside a microscopic optical Fabry-Perot cavity. In particular, we demonstrate a fiber Fabry-Perot cavity operating on the principal ${S}_{1/2}\ensuremath{\rightarrow}{P}_{1/2}$ electric dipole transition of an Yb+{\mathrm{Yb}}^{+}Yb+ ion at 369 nm with an ion-cavity coupling strength of $g=2\ensuremath{\pi}\ifmmode\times\else\texttimes\fi{}67(1)$ MHz. We employ the cavity to study the generation of single photons and observe cavity-induced backaction in the Purcell-enhanced emission of photons. Tuning of the amplitude and phase between the driving field and the cavity field built up from photons scattered into the cavity mode by the ion allows us to enhance or suppress the total rate of photon emission from the ion-cavity system.