Abstract There are two standard ways of classifying transport behavior of systems. The first is via time scaling of spread of correlations in the isolated system in thermodynamic limit. The second is via system size scaling of conductance in the steady state of the open system. We show here that these correspond to taking the thermodynamic limit and the long time limit of the integrated equilibrium current–current correlations of the open system in different order. In general, the limits may not commute leading to a conflict between the two standard ways of transport classification. Nevertheless, the full information is contained in the equilibrium current–current correlations of the open system. We show this analytically by rigorously deriving the open-system current fluctuation dissipation relations starting from an extremely general open quantum set-up and then carefully taking the proper limits. We test our theory numerically on the non-trivial example of the critical Aubry–André–Harper model, where, it has been recently shown that, the two standard classifications indeed give different results. We find that both the total current autocorrelation and the long-range local current correlations of the open system in equilibrium show signatures of diffusive transport up to a time scale. This time scale grows as square of system size. Beyond this time scale a steady state value is reached. The steady state value is conductance, which shows sub-diffusive scaling with system size.
Abstract There are two standard ways of classifying transport behavior of systems. The first is via time scaling of spread of correlations in the isolated system in thermodynamic limit. The second is via system size scaling of conductance in the steady state of the open system. We show here that these correspond to taking the thermodynamic limit and the long time limit of the integrated equilibrium current–current correlations of the open system in different order. In general, the limits may not commute leading to a conflict between the two standard ways of transport classification. Nevertheless, the full information is contained in the equilibrium current–current correlations of the open system. We show this analytically by rigorously deriving the open-system current fluctuation dissipation relations starting from an extremely general open quantum set-up and then carefully taking the proper limits. We test our theory numerically on the non-trivial example of the critical Aubry–André–Harper model, where, it has been recently shown that, the two standard classifications indeed give different results. We find that both the total current autocorrelation and the long-range local current correlations of the open system in equilibrium show signatures of diffusive transport up to a time scale. This time scale grows as square of system size. Beyond this time scale a steady state value is reached. The steady state value is conductance, which shows sub-diffusive scaling with system size.
There are two well-established ways of characterizing transport properties. The first is via the spread of correlations in an isolated system. The second is through the system-size dependence of the current, when a potential bias is applied by connecting the two ends of the system to reservoirs. These are two different experiments, but usually the result of one experiment can be inferred from that of the other. This work presents a surprising counterexample. The authors show that, at the critical point of the Aubry-Andr\'e-Harper model, transport in the presence of reservoirs is drastically different from transport in the isolated system. The scaling of current with system size shows clear subdiffusive behavior, while the spread of correlations does not show any subdiffusive behavior. It actually hints at superdiffusion. This implies that the understanding of the relation between transport in open and in isolated systems needs to be reexamined.
Understanding the transport properties of quantum many-body systems is a central challenge in condensed matter and statistical physics. Theoretical studies usually rely on two main approaches: Dynamics of linear-response functions in closed systems and boundary-driven dynamics governed by Markovian master equations for open systems. While the equivalence of their dynamical behavior has been explored in recent studies, a systematic comparison of the transport coefficients obtained from these two classes of approaches remains a largely open question. Here, we address this gap by comparing and contrasting the dc diffusion constant Ddc according to the two approaches, focusing on the specific example of magnetization transport in the spin-1/2 XXZ chain. Using exact numerical simulations for finite system sizes, we find (i) a clear mismatch between the two Ddc and (ii) a strong dependence of Ddc on the system-bath coupling strength for the open system, where neither (i) nor (ii) tend to vanish in the thermodynamic limit. These findings suggest limitations of the open-system approach to transport coefficients. To gain insight into the origin of (i) and (ii), we go beyond Ddc and analyze the full time dependence of the diffusion coefficient D(t) in the open system. In this way, we find that both (i) and (ii) vanish up to a finite time scale. While this time scale gradually increases with system size and tends to be macroscopic in the thermodynamic limit, this increase is still slow compared to the increase of the time to reach the steady state, where (i) and (ii) do not vanish. This observation can be seen as a wrong, yet unavoidable order of limits of long times first and large system sizes afterwards.
Non-equilibrium steady-states are characterized by the existence of macroscopic heat currents flowing between two or more reservoirs. However, the existence of these currents also implies that information is constantly being transmitted from one reservoir to the other. In this letter we address the transport of information in the context of quantum non-equilibrium steady states. We first show how the ability of the excitations to transfer information can be quantified by the conditional mutual information (CMI), a more general measure of tripartite correlations. We then apply this to an exactly soluble model allowing for both ballistic and diffusive behavior. Our approach allows us to compute the CMI for arbitrary sizes and thus find the scaling rules connecting information transport and diffusivity. Finally, we discuss how this new perspective in the characterization of non-equilibrium systems may be applied to understand the issue of local equilibration in non-equilibrium states.
The study of electrical currents in a regime where a description as a continuous flow fails and the particle nature becomes important, but where notions such as particle density or currents continue to be meaningful, will be at the heart of the present dissertation. Given such a mesoscopic system through which electrons flow, either actively through quantum pumping or passively due to a potential difference, we investigate quantities such as transferred charge, noise, current fluctuations, and relations between them. More generally we shall examine the statistics of particle transport. All discussions will concentrate on compact devices transferring charge between two one-dimensional reservoirs (the leads) of independent electrons. Firstly, we consider the generating function of the moments of transferred charge and we prove that it is given by the determinant of a single-particle operator. It is formally equivalent to a formula of Lesovik and Levitov, but is shown to be well-defined in the situations under consideration, whereas the former is not, in general. The mechanism leading to regularization is typical for mesoscopic systems: we consider a limiting case that reveals the fundamental structure of the problem. In fact, as suited for an open system, the leads contain an infinite number of charges. It follows mathematically that the second quantization ought to be carried out upon the Fermi sea and not upon the vacuum, a procedure known as the GNS construction. We shall rely heavily on operator algebraic techniques. The set of observables, the C*-algebra of canonical anticommutation relations, admits different representations for systems in the thermodynamic limit, which are described by their reduced one-particle density matrix. An important question will be the existence of operators such as the charge or the time evolution in a given representation, which induce so-called Bogoliubov transformations. These prerequisites at hand, we shall pose the problem of counting statistics clearly, prove that the regularized determinant emerges naturally, and show that it describes the transport of integer charges with non-negative probabilities. Secondly, we introduce a model of instantaneous scattering in which various examples can be computed explicitely. In particular, we show that the above theorem applies for scattering through a smoothly operating pump over a finite time interval. We also exhibit situations where the propagator does exist but the generating function is ambiguous. In a more computational approach, we then turn to the relation of individual moments of transferred charge to current correlators. It turns out that the former can indeed be expressed as integrals of the latter over time, provided the current operators are ordered according to Matthews’ T∗ ordering. It is given by first arranging the charge operators according to their time indices, and only then taking the time derivatives, which induce contact terms whose singular support lies along time coincidences. We shall give two derivations of this result, because the first one is transparent, and the second one is related to contradictory computations in the literature where the system is considered to be measured by an external spin. In the model of constant instantaneous scattering, we then argue from the Lesovik-Levitov determinant that the transport can be interpreted in terms of a binomial process in the long time limit. In a parallel computation, we concentrate on the third cumulant as defined by integration of current correlators and show how the contact terms of the T∗ ordering play an essential role in providing the expected binomial result, too. To close this thesis, we suggest an algebraic framework that lays the foundations for a rigorous discussion of the Casimir effect. The problem of infinites arising in the comparison of two physical situations for a bosonic field is interpreted as the non-equivalence of states on the algebra of canonical commutation relations. We exhibit sufficient conditions on the one-particle Hamiltonians which ensure that the Casimir energy is finite and give an expression for it. We discuss its formal equivalence with the result obtained from the standard mode summing method.
Based on the references [P1–P6], we investigate in this cumulative PhD thesis the dynamics and transport in closed and open interacting spin chain models. We focus on (i) the connection between the open and the closed system dynamics [P1, P2], (ii) the influence of various system parameters on the transport behavior in closed and open systems [P3, P5], and in addtion (iii) the dynamics and transport in closed models [P4, P6]. As for (i), we explore the connection of the dynamics in open systems, modeled by the Lindblad equation, and the correlation functions in the closed system [P1]. Building on this connection for magnetization transport, we study whether the time evolution of the open quantum system can be described in terms of classical correlation functions generated by the Hamiltonian equations of motion for real vectors [P2]. Second, we study in (ii) the influence of different parameters on the diffusion constants in closed and open systems [P3, P5]. In Ref. [P3], we study the impact of integrability-breaking perturbations in both closed and open spin chain systems. While we find a continuous change of the diffusion constant with perturbation strength in the closed system, in the open system, in the weak-perturbation limit, we indicate the possibility of a diverging diffusion constant. Also, we investigate the influence of the system-bath coupling on the transport behavior in boundary-driven open systems [P5]. We observe that the diffusion constants depend on the system-bath coupling and that in the nonequilibrium steady state, they inevitably retain finite-size effects, limiting the computation of long-time transport coefficients. Additional for (iii), in Ref. [P4], we first examine the impact of perturbations on the dynamics in closed spin chain models. We employ projector-operator techniques to understand, on perturbative grounds, the nontrivial damping of the standard correlation function. Second, we also discuss a dynamical quantum typicality approach for studying the energy transport in bipartite systems at low temperatures [P6].
Full understanding of the relaxation mechanisms and far-from-equilibrium transport in modern mesoscopic structures requires that such systems be treated as open. We therefore generalize some of the core elements of the Kadanoff-Baym-Keldysh nonequilibrium Green's function formalism, inherently formulated for closed systems, to treatment of an open system, coupled with its environment. We define the two-time correlation functions and analyze the influence of the memory effects on the open-system transport. In the transient regime, the two-time correlation functions clearly show four distinct terms: a closed-system-like term, an entanglement term, and two memory terms that depend explicitly on the initial state of the environment. We show that it is not possible to completely eliminate the influence of the environment by a fortunate choice of the initial state, and approximating the system as closed is valid only in the limit of negligible system-environment coupling, which is never the case in the transient regime. We derive the transport equations for transients that properly account for the system-environment coupling. On the other hand, we address the important issue of transport in a far-from-equilibrium steady state. We show that, once a steady state is reached, the balance between the driving and relaxation forces implies that the two-time correlation functions regain a closed-system-like form, but with an effective, modified system Hamiltonian, and with the system statistical operator unrelated to that of the initial state. We emphasize that the difference between the transient and the far-from-equilibrium steady-state regimes, crucial for theoretical investigation of nonequilibrium quasiparticle transport, effectively lies within the different relative magnitude of the combined entanglement and memory terms with respect to the closed-system-like term in two-time correlation functions.