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arXiv:1709.07921 · Physical Review Letters

Spin Order and Phase Transitions in Chains of Polariton Condensates

Hamid Ohadi, A. J. Ramsay, Helgi Sigurðsson, Yago del Valle‐Inclan Redondo, S. I. Tsintzos, Z. Hatzopoulos, T. C. H. Liew, Ivan Andreevich Shelykh, Yuri G. Rubo, Pavlos G. Savvidis, Jeremy J. Baumberg

Published Aug 8, 2017• 83 citations
arXivHTMLPDF

Abstract

We demonstrate that multiply coupled spinor polariton condensates can be optically tuned through a sequence of spin-ordered phases by changing the coupling strength between nearest neighbors. For closed four-condensate chains these phases span from ferromagnetic (FM) to antiferromagnetic (AFM), separated by an unexpected crossover phase. This crossover phase is composed of alternating FM-AFM bonds. For larger eight-condensate chains, we show the critical role of spatial inhomogeneities and demonstrate a scheme to overcome them and prepare any desired spin state. Our observations thus demonstrate a fully controllable nonequilibrium spin lattice.

DOI
10.1103/physrevlett.119.067401

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We demonstrate that multiply coupled spinor polariton condensates can be optically tuned through a sequence of spin-ordered phases by changing the coupling strength between nearest neighbors. For closed four-condensate chains these phases span from ferromagnetic (FM) to antiferromagnetic (AFM), separated by an unexpected crossover phase. This crossover phase is composed of alternating FM-AFM bonds. For larger eight-condensate chains, we show the critical role of spatial inhomogeneities and demonstrate a scheme to overcome them and prepare any desired spin state. Our observations thus demonstrate a fully controllable nonequilibrium spin lattice.
Tunable spin correlations are found to arise between two neighboring trapped exciton-polariton condensates which spin polarize spontaneously. We observe a crossover from an antiferromagnetic to a ferromagnetic pair state by reducing the coupling barrier in real time using control of the imprinted pattern of pump light. Fast optical switching of both condensates is then achieved by resonantly but weakly triggering only a single condensate. These effects can be explained as the competition between spin bifurcations and spin-preserving Josephson coupling between the two condensates, and open the way to polariton Bose-Hubbard ladders.
There is a growing interest in investigating new states of matter using out-of-equilibrium lattice spin models in two dimensions. However, a control of pairwise interactions in such systems has been elusive as due to their nonequilibrium nature they maintain nontrivial particle fluxes even at the steady state. Here we suggest how to overcome this problem and formulate a method for engineering reconfigurable networks of nonequilibrium condensates with control of individual pairwise interactions. Representing spin by condensate phase, the effective two spin interactions are created with nonresonant pumping, are directed with dissipative channels, and are further controlled with dissipative gates. The dissipative barriers are used to block unwanted interactions between condensates. Together, spatial anisotropy of dissipation and pump profiles allow an effective control of sign and intensity of the coupling strength between any two neighboring sites independent of the rest of the spins, which we demonstrate with a two dimensional square lattice of polariton condensates. Experimental realisation of such fully-controllable networks offers great potential for an efficient analog Hamiltonian optimizer and for reservoir computing.
We observe the joint spin-spatial (spinor) self-organization of a two-component Bose-Einstein condensate (BEC) strongly coupled to an optical cavity. This unusual nonequilibrium Hepp-Lieb-Dicke phase transition is driven by an off-resonant Raman transition formed from a classical pump field and the emergent quantum dynamical cavity field. This mediates a spinor-spinor interaction that, above a critical strength, simultaneously organizes opposite spinor states of the BEC on opposite checkerboard configurations of an emergent 2D lattice. The resulting spinor density-wave polariton condensate is observed by directly detecting the atomic spin and momentum state and by holographically reconstructing the phase of the emitted cavity field. The latter provides a direct measure of the spin state, and a spin-spatial domain wall is observed. The photon-mediated spin interactions demonstrated here may be engineered to create dynamical gauge fields and quantum spin glasses.
We investigate the formation of mutual coherence and deterministic phase control in a multimode exciton-polariton system realized in two optically induced traps with tunable intertrap coupling. As the coupling channel between the traps is progressively opened, the mutual first-order coherence rises sharply from nearly zero to values close to unity, revealing a threshold-like crossover from weakly correlated to highly coherent dynamics. We demonstrate deterministic multimode phase control with a short spatially localized nonresonant pulse, which allows the phase relations between selected polariton condensate modes to be set while keeping their amplitudes nearly unchanged. The induced phase transformation is read out directly from time-resolved interferograms and realized for different sets of modes in both intermediate- and high-coherence regimes. Within a reduced four-mode description, the control pulse implements an effective phase operator on the coherent multimode field with a fidelity exceeding 0.995. The same approach can be extended to larger networks of coupled traps, offering a route to optical control over phase relations in increasingly complex multimode polariton states.
Phase transitions in spinor Bose gases with ferromagnetic (FM) couplings are studied via mean-field theory. We show that an infinitesimal value of the coupling can induce a FM phase transition at a finite temperature always above the critical temperature of Bose-Einstein condensation. This contrasts sharply with the case of Fermi gases, in which the Stoner coupling Is{I}_{s}Is​ cannot lead to a FM phase transition unless it is larger than a threshold value I0.{I}_{0}.I0​. The FM coupling also increases the critical temperatures of both the ferromagnetic transition and the Bose-Einstein condensation.
Ground state properties, dispersion relations and scaling behaviour of spin gap of a bond alternating spin-1 2 anisotropic Heisenberg chain have been studied where the exchange interactions on alternate bonds are ferromagnetic (FM) and antiferromagnetic (AFM) in two separate cases.The resulting models separately represent nearest neighbour (NN) AFM-AFM and AFM-FM bond alternating chains.Ground state energy has been estimated analytically by using both bond operator and Jordan-Wigner representations and numerically by using exact diagonalization.Dispersion relations, spin gap and several ground state orders have been obtained.Dimer order and string orders are found to coexist in the ground state.Spin gap is found to develop as soon as the non-uniformity in alternating bond strength is introduced in the AFM-AFM chain which further remains non-zero for the AFM-FM chain.This spin gap along with the string orders attribute to the Haldane phase.The Haldane phase is found to exist in most of the anisotropic region similar to the isotropic point.