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arXiv:1807.04915 · Physical Review Letters

Spinor Self-Ordering of a Quantum Gas in a Cavity

Ronen M. Kroeze, Yudan Guo, Varun Vaidya, Jonathan Keeling, Benjamin Lev

Published Oct 16, 2018• 157 citations
arXivHTMLPDF

Abstract

We observe the joint spin-spatial (spinor) self-organization of a two-component Bose-Einstein condensate (BEC) strongly coupled to an optical cavity. This unusual nonequilibrium Hepp-Lieb-Dicke phase transition is driven by an off-resonant Raman transition formed from a classical pump field and the emergent quantum dynamical cavity field. This mediates a spinor-spinor interaction that, above a critical strength, simultaneously organizes opposite spinor states of the BEC on opposite checkerboard configurations of an emergent 2D lattice. The resulting spinor density-wave polariton condensate is observed by directly detecting the atomic spin and momentum state and by holographically reconstructing the phase of the emitted cavity field. The latter provides a direct measure of the spin state, and a spin-spatial domain wall is observed. The photon-mediated spin interactions demonstrated here may be engineered to create dynamical gauge fields and quantum spin glasses.

DOI
10.1103/physrevlett.121.163601

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We observe the joint spin-spatial (spinor) self-organization of a two-component Bose-Einstein condensate (BEC) strongly coupled to an optical cavity. This unusual nonequilibrium Hepp-Lieb-Dicke phase transition is driven by an off-resonant Raman transition formed from a classical pump field and the emergent quantum dynamical cavity field. This mediates a spinor-spinor interaction that, above a critical strength, simultaneously organizes opposite spinor states of the BEC on opposite checkerboard configurations of an emergent 2D lattice. The resulting spinor density-wave polariton condensate is observed by directly detecting the atomic spin and momentum state and by holographically reconstructing the phase of the emitted cavity field. The latter provides a direct measure of the spin state, and a spin-spatial domain wall is observed. The photon-mediated spin interactions demonstrated here may be engineered to create dynamical gauge fields and quantum spin glasses.
We realize the dynamical 1D spin-orbit coupling (SOC) of a Bose-Einstein condensate confined within an optical cavity. The SOC emerges through spin-correlated momentum impulses delivered to the atoms via Raman transitions. These are effected by classical pump fields acting in concert with the quantum dynamical cavity field. Above a critical pump power, the Raman coupling emerges as the atoms superradiantly populate the cavity mode with photons. Concomitantly, these photons cause a backaction onto the atoms, forcing them to order their spin-spatial state. This SOC-inducing superradiant Dicke phase transition results in a spinor-helix polariton condensate. We observe emergent SOC through spin-resolved atomic momentum imaging and temporal heterodyne measurement of the cavity-field emission. Dynamical SOC in quantum gas cavity QED, and the extension to dynamical gauge fields, may enable the creation of Meissner-like effects, topological superfluids, and exotic quantum Hall states in coupled light-matter systems.
The recent experimental observation of spinor self-ordering of ultracold atoms in optical resonators has set the stage for the exploration of emergent magnetic orders in quantum-gas−-−cavity systems. Based on this platform, we introduce a generic scheme for the implementation of quantum spin Hamiltonians composed of various kinds of couplings, including Heisenberg and Dzyaloshinskii-Moriya interactions. These interactions with spatially modulated coupling coefficients are mediated by cavity photons. Specifically, our model is comprised of a two-component Bose-Einstein condensate, driven by two classical pump lasers and coupled to a single dynamic mode of a linear cavity in a double Λ\LambdaΛ scheme. We exemplify the emergence of an achiral antiferromagnetic domain-wall phase and a chiral spin-spiral order beyond critical laser strengths. The transition between these two phases can be observed in a single experimental setup by tuning the reflectivity of a mirror. We also discuss straightforward extensions of our scheme for the implementation of other classes of spin Hamiltonians.
We study spatial spin and density self-ordering of a two-component Bose-Einstein condensate via collective Raman scattering into a linear cavity mode. The onset of the Dicke superradiance phase transition is marked by a simultaneous appearance of a crystalline density order and a spin-wave order. The latter spontaneously breaks the discrete Z_{2} symmetry between even and odd sites of the cavity optical potential. Moreover, in the superradiant state the continuous U(1) symmetry of the relative phase of the two condensate wave functions is explicitly broken by the cavity-induced position-dependent Raman coupling with a zero spatial average. Thus, the spatially averaged relative condensate phase is locked at either π/2 or -π/2. This continuous symmetry breaking and relative condensate phase locking by a zero-average Raman field can be considered as a generic order-by-disorder process similar to the random-field-induced order in the two-dimensional classical ferromagnetic XY spin model. However, the seed of the random field in our model stems from quantum fluctuations in the cavity field and is a dynamical entity affected by self-ordering. The spectra of elementary excitations exhibit the typical mode softening at the superradiance threshold.
We report on the first experimental realization of the Dicke quantum phase transition realized in the quantum motion of a Bose–Einstein condensate coupled to an optical cavity. Conceptually, the transition is driven by cavity-mediated long-range interactions, giving rise to the emergence of a self-organized supersolid phase. The Dicke phase transition, predicted in 1973, has not been demonstrated experimentally before this work, both due to fundamental and technological reasons. These challenges have been overcome in the present thesis by employing atomic momentum states of a Bose-Einstein condensate, which are coupled via two-photon Raman transitions involving a cavity photon and a free-space pump photon. This open-system implementation of the Dicke model allows to tune all relevant parameters and offers a unique detection scheme to monitor the manybody system in real time. We demonstrate that the phase transition is accompanied by a macroscopically occupied cavity field and a striking change in the atomic momentum distribution, due to spontaneous self-organization of the atomic density on a checkerboard lattice. The boundary of the transition is mapped out by scanning two parameters of the Dicke model, to reveal a phase diagram in close agreement with the model description. Two different ordered configurations are allowed in the superradiant phase, giving rise to the concept of spontaneous symmetry breaking at the phase transition. We experimentally distinguish the symmetry-broken states and study the origin of the symmetry-breaking process. The finite spatial extension of our system induces a small symmetry-breaking field which changes randomly on each experimental realization. The influence of this field is studied and shown to diminish upon dynamically crossing the transition point with increasing transition rates.
We explore the many-body phases of a two-dimensional Bose-Einstein condensate with cavity-mediated dynamic spin-orbit coupling. With the help of two transverse noninterfering, counterpropagating pump lasers and a single standing-wave cavity mode, two degenerate Zeeman sub-levels of the quantum gas are Raman coupled in a double-$\mathrm{\ensuremath{\Lambda}}$-configuration. Beyond a critical pump strength the cavity mode is populated via coherent superradiant Raman scattering from the two pump lasers, leading to the appearance of a dynamical spin-orbit coupling for the atoms. We identify three quantum phases with distinct atomic and photonic properties: the normal ``homogeneous'' phase, the superradiant ``spin-helix'' phase, and the superradiant ``supersolid spin-density-wave'' phase. The last exhibits an emergent periodic atomic density distribution with an orthorhombic centered rectangular-lattice structure due to the interplay between the coherent photon scattering into the resonator and the collision-induced momentum coupling. The transverse lattice spacing of the emergent crystal is set by the dynamic spin-orbit coupling.
The recent experimental observation of spinor self-ordering of ultracold atoms in optical resonators has set the stage for the exploration of emergent magnetic orders in quantum-gas-cavity systems. Based on this platform, we introduce a generic scheme for the implementation of long-range quantum spin Hamiltonians composed of various types of couplings, including Heisenberg and Dzyaloshinskii-Moriya interactions. Our model is composed of an effective two-component Bose-Einstein condensate, driven by two classical pump lasers and coupled to a single dynamic mode of a linear cavity in a double Λ scheme. Cavity photons mediate the long-range spin-spin interactions with spatially modulated coupling coefficients, where the latter ones can be tuned by modifying spatial profiles of the pump lasers. As experimentally relevant examples, we demonstrate that by properly choosing the spatial profiles of the pump lasers achiral domain-wall antiferromagnetic and chiral spin-spiral orders emerge beyond critical laser strengths. The transition between these two phases can be observed in a single experimental setup by tuning the reflectivity of a mirror. We also discuss extensions of our scheme for the implementation of other classes of spin Hamiltonians.