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arXiv:1705.06382 · Physical Review Letters

Disorder-Driven Density and Spin Self-Ordering of a Bose-Einstein Condensate in a Cavity

Farokh Mivehvar, Francesco Piazza, Helmut Ritsch

Published Aug 9, 2017• 59 citations
arXivHTMLPDF

Abstract

We study spatial spin and density self-ordering of a two-component Bose-Einstein condensate via collective Raman scattering into a linear cavity mode. The onset of the Dicke superradiance phase transition is marked by a simultaneous appearance of a crystalline density order and a spin-wave order. The latter spontaneously breaks the discrete Z_{2} symmetry between even and odd sites of the cavity optical potential. Moreover, in the superradiant state the continuous U(1) symmetry of the relative phase of the two condensate wave functions is explicitly broken by the cavity-induced position-dependent Raman coupling with a zero spatial average. Thus, the spatially averaged relative condensate phase is locked at either π/2 or -π/2. This continuous symmetry breaking and relative condensate phase locking by a zero-average Raman field can be considered as a generic order-by-disorder process similar to the random-field-induced order in the two-dimensional classical ferromagnetic XY spin model. However, the seed of the random field in our model stems from quantum fluctuations in the cavity field and is a dynamical entity affected by self-ordering. The spectra of elementary excitations exhibit the typical mode softening at the superradiance threshold.

DOI
10.1103/physrevlett.119.063602

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We study spatial spin and density self-ordering of a two-component Bose-Einstein condensate via collective Raman scattering into a linear cavity mode. The onset of the Dicke superradiance phase transition is marked by a simultaneous appearance of a crystalline density order and a spin-wave order. The latter spontaneously breaks the discrete Z_{2} symmetry between even and odd sites of the cavity optical potential. Moreover, in the superradiant state the continuous U(1) symmetry of the relative phase of the two condensate wave functions is explicitly broken by the cavity-induced position-dependent Raman coupling with a zero spatial average. Thus, the spatially averaged relative condensate phase is locked at either π/2 or -π/2. This continuous symmetry breaking and relative condensate phase locking by a zero-average Raman field can be considered as a generic order-by-disorder process similar to the random-field-induced order in the two-dimensional classical ferromagnetic XY spin model. However, the seed of the random field in our model stems from quantum fluctuations in the cavity field and is a dynamical entity affected by self-ordering. The spectra of elementary excitations exhibit the typical mode softening at the superradiance threshold.
We report on the first experimental realization of the Dicke quantum phase transition realized in the quantum motion of a Bose–Einstein condensate coupled to an optical cavity. Conceptually, the transition is driven by cavity-mediated long-range interactions, giving rise to the emergence of a self-organized supersolid phase. The Dicke phase transition, predicted in 1973, has not been demonstrated experimentally before this work, both due to fundamental and technological reasons. These challenges have been overcome in the present thesis by employing atomic momentum states of a Bose-Einstein condensate, which are coupled via two-photon Raman transitions involving a cavity photon and a free-space pump photon. This open-system implementation of the Dicke model allows to tune all relevant parameters and offers a unique detection scheme to monitor the manybody system in real time. We demonstrate that the phase transition is accompanied by a macroscopically occupied cavity field and a striking change in the atomic momentum distribution, due to spontaneous self-organization of the atomic density on a checkerboard lattice. The boundary of the transition is mapped out by scanning two parameters of the Dicke model, to reveal a phase diagram in close agreement with the model description. Two different ordered configurations are allowed in the superradiant phase, giving rise to the concept of spontaneous symmetry breaking at the phase transition. We experimentally distinguish the symmetry-broken states and study the origin of the symmetry-breaking process. The finite spatial extension of our system induces a small symmetry-breaking field which changes randomly on each experimental realization. The influence of this field is studied and shown to diminish upon dynamically crossing the transition point with increasing transition rates.
We theoretically examine collective excitations of an optically driven atomic Bose-Einstein condensate, coupled to a high-finesse optical cavity. This open system has been recently used for the experimental demonstration of the Dicke superradiance of cavity photons, which is simultaneously and mutually triggered by spontaneous breaking of translational symmetry of the condensate into a crystalline order. We first develop a Hartree-Fock mean field dynamical model of the physical system. Using this model, we compute the dynamics of the cavity photons, the condensate density profile and the Dicke phase transition diagram. Both the imaginary-time and real-time evolution methods are used in the calculations. Collective excitations are determined by the solving Bogoliubov-de Gennes equations. The spectrum, softening of the modes and energetic hierarchy of excitations are determined.
We observe the joint spin-spatial (spinor) self-organization of a two-component Bose-Einstein condensate (BEC) strongly coupled to an optical cavity. This unusual nonequilibrium Hepp-Lieb-Dicke phase transition is driven by an off-resonant Raman transition formed from a classical pump field and the emergent quantum dynamical cavity field. This mediates a spinor-spinor interaction that, above a critical strength, simultaneously organizes opposite spinor states of the BEC on opposite checkerboard configurations of an emergent 2D lattice. The resulting spinor density-wave polariton condensate is observed by directly detecting the atomic spin and momentum state and by holographically reconstructing the phase of the emitted cavity field. The latter provides a direct measure of the spin state, and a spin-spatial domain wall is observed. The photon-mediated spin interactions demonstrated here may be engineered to create dynamical gauge fields and quantum spin glasses.
We explore the density and spin self-ordering of driven spin-1/2 collisionless fermionic atoms coupled to the electromagnetic fields of a ring resonator. The two spin states are two-photon Raman-coupled via a pair of degenerate counterpropagating cavity modes and two transverse pump fields. In this one-dimensional configuration the coupled atom-field system possesses a continuous U (1) translational symmetry and a discrete Z 2 spin inversion symmetry. At half filling for sufficiently strong pump strengths, the combined U (1) × Z 2 symmetry is spontaneously broken at the onset of a superradiant phase transition to a state with self-ordered density and spin structures. We predominately find an antiferromagnetic lattice order at the cavity wavelength. The self-ordered states exhibit unexpected positive momentum pair correlations between fermions with opposite spin. These strong cavity-mediated correlations vanish at higher pump strength.
We investigate the interplay between cavity-induced density-wave ordering and controllable disorder in a trapped two-dimensional gas of ultracold fermions. The atoms are dispersively coupled to an optical cavity and transversely driven by a pump beam, while an additional speckle beam spatially modulates the atom-light coupling through an AC-Stark shift of the atomic transition. In momentum space, this disorder converts the usual coupling between the cavity mode and a discrete set of density-wave Fourier components into a coupling to a continuum of fermionic density modes, weighted by the spectrum of the speckle pattern. Using linear response theory, we derive the superradiant threshold and show that the disordered interaction renormalizes the effective light-matter coupling, lowering the critical pump strength on average, with the threshold becoming self-averaging for short speckle correlation lengths. We complement this analysis with a numerical mean-field treatment that gives access to the intracavity photon number and to the real-space fermion density across the transition. These results confirm that the disorder shifts the photonic phase boundary and, above threshold, distorts the density-wave crystal by populating Fourier components beyond those selected by the clean cavity geometry. Our findings identify both the emitted cavity light and in situ density images as probes of engineered disorder in fermionic matter coupled to optical cavities.