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arXiv:1603.02830 · Physical Review Letters

Tunable Magnetic Alignment between Trapped Exciton-Polariton Condensates

Hamid Ohadi, Yago del Valle‐Inclan Redondo, Alexander Dreismann, Yuri G. Rubo, Florian Pinsker, S. I. Tsintzos, Z. Hatzopoulos, Pavlos G. Savvidis, Jeremy J. Baumberg

Published Mar 8, 2016• 29 citations
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Abstract

Tunable spin correlations are found to arise between two neighboring trapped exciton-polariton condensates which spin polarize spontaneously. We observe a crossover from an antiferromagnetic to a ferromagnetic pair state by reducing the coupling barrier in real time using control of the imprinted pattern of pump light. Fast optical switching of both condensates is then achieved by resonantly but weakly triggering only a single condensate. These effects can be explained as the competition between spin bifurcations and spin-preserving Josephson coupling between the two condensates, and open the way to polariton Bose-Hubbard ladders.

DOI
10.1103/physrevlett.116.106403

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Tunable spin correlations are found to arise between two neighboring trapped exciton-polariton condensates which spin polarize spontaneously. We observe a crossover from an antiferromagnetic to a ferromagnetic pair state by reducing the coupling barrier in real time using control of the imprinted pattern of pump light. Fast optical switching of both condensates is then achieved by resonantly but weakly triggering only a single condensate. These effects can be explained as the competition between spin bifurcations and spin-preserving Josephson coupling between the two condensates, and open the way to polariton Bose-Hubbard ladders.
We develop the many-body theory of dipolar exciton-polaritons in an optical microcavity in crossed out-of-plane electric and in-plane magnetic fields. Even for relatively weak fields, we reveal the existence of two minima in the bare lower-polariton dispersion, which give rise to the tunable transition between the polariton Bose-Einstein condensate and that of excitons, produced by the competition between these minima. We predict that such dipolar condensate exhibits a roton-maxon character of the excitation spectrum, never before observed for polaritons. We show that upon the transition between the two condensation regimes, the weak correlations in the polariton gas give way to the intermediate interparticle correlations characteristic for excitons, and that the transition is accompanied by a sharp quenching of photoluminescence as the lifetime is increased by several orders of magnitude. While in the polariton regime, the luminescence peak corresponding to the condensate is shifted to a nonzero angle. The angular dependence of the two-photon decay time in the Hanbury Brown and Twiss experiment is calculated and used as a tool to evidence the formation of the macroscopically coherent state. Our proposal opens opportunities towards manipulating the superfluid properties and extended-range dipole-dipole correlations of exciton-polariton condensates.
We demonstrate a linear to circular polarization conversion mechanism of a confined polariton condensate created by an optical potential trap. This system features a high degree of circular polarization under linear polarization pumping and is favorable for the development of spin logic operations. The physical mechanism behind this process is explained by the spin precession in the exciton reservoir that results in a condensate of a preferred spin state. Application of a non-resonant below threshold femtosecond pulse on the spinor condensate results in an ultrafast reversal of the spin state.
We investigate the formation of mutual coherence and deterministic phase control in a multimode exciton-polariton system realized in two optically induced traps with tunable intertrap coupling. As the coupling channel between the traps is progressively opened, the mutual first-order coherence rises sharply from nearly zero to values close to unity, revealing a threshold-like crossover from weakly correlated to highly coherent dynamics. We demonstrate deterministic multimode phase control with a short spatially localized nonresonant pulse, which allows the phase relations between selected polariton condensate modes to be set while keeping their amplitudes nearly unchanged. The induced phase transformation is read out directly from time-resolved interferograms and realized for different sets of modes in both intermediate- and high-coherence regimes. Within a reduced four-mode description, the control pulse implements an effective phase operator on the coherent multimode field with a fidelity exceeding 0.995. The same approach can be extended to larger networks of coupled traps, offering a route to optical control over phase relations in increasingly complex multimode polariton states.
We analyze theoretically the phenomena related to the Josephson effect for exciton and polariton condensates, taking into account their specific spin degrees of freedom. We distinguish between two types of Josephson effects: the extrinsic effect, related to the coherent tunneling of particles with the same spin between two spatially separated potential traps, and the intrinsic effect, related to the ``tunneling'' between different spinor components of the condensate within the same trap. We show that the Josephson effect in the nonlinear regime can lead to nontrivial polarization dynamics and produce spontaneous separation of the condensates with opposite polarization in real space.
The effect of a magnetic field on a spinor exciton-polariton condensate has been investigated. A quenching of a polariton Zeeman splitting and an elliptical polarization of the condensate have been observed at low magnetic fields B<2 T. The effects are attributed to a competition between the magnetic field induced circular polarization buildup and the spin-anisotropic polariton-polariton interaction which favors a linear polarization. The sign of the circular polarization of the condensate emission at B<3 T is negative, suggesting that a dynamic condensation in the excited spin state rather than the ground spin state takes place in this magnetic field range. From about 2T on, the Zeeman splitting opens and from then on the slope of the circular polarization degree changes its sign. For magnetic fields larger than the 3 T, the upper spin state occupation is energetically suppressed and circularly polarized condensation takes place in the ground state.
We demonstrate that multiply coupled spinor polariton condensates can be optically tuned through a sequence of spin-ordered phases by changing the coupling strength between nearest neighbors. For closed four-condensate chains these phases span from ferromagnetic (FM) to antiferromagnetic (AFM), separated by an unexpected crossover phase. This crossover phase is composed of alternating FM-AFM bonds. For larger eight-condensate chains, we show the critical role of spatial inhomogeneities and demonstrate a scheme to overcome them and prepare any desired spin state. Our observations thus demonstrate a fully controllable nonequilibrium spin lattice.