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arXiv:1708.06920 · New Journal of Physics

A high repetition deterministic single ion source

C Sahin, Philipp Geppert, A. Müllers, Herwig Ott

Published Oct 18, 2017• 13 citations
arXivHTMLPDF

Abstract

We report on a deterministic single ion source with high repetition rate and high fidelity. The source employs a magneto-optical trap, where ultracold rubidium atoms are photoionized. The electrons herald the creation of a corresponding ion, whose timing information is used to manipulate its trajectory in flight. We demonstrate an ion rate of up to and achieve a fidelity for single ion operation of 98%. The technique can be used for all atomic species, which can be laser-cooled, and opens up new applications in ion microscopy, ion implantation and surface spectroscopy.

DOI
10.1088/1367-2630/aa9461

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This Week in Science

The manipulation of single-quantum objects is a key requirement for the engineering of microscopic quantum systems. Applications such as single-atom micromasers (microwave lasers), triggered single-photon sources, or deterministic entanglement of atoms all require the ability to deliver single atoms on demand to a desired location. The trapping and manipulation of atoms as neutral species is more challenging than for charged ions because of the weak interaction of neutral species with electromagnetic fields. Kuhr et al. (p. 278) have overcome these difficulties by combining magneto-optical trapping and optical-trapping techniques. They demonstrate the precision transport of single neutral cesium atoms over distances of 1 centimeter and the ejection of single atoms into free flight.

Science•Jul 13, 2001•1 citation
We report on a deterministic single ion source with high repetition rate and high fidelity. The source employs a magneto-optical trap, where ultracold rubidium atoms are photoionized. The electrons herald the creation of a corresponding ion, whose timing information is used to manipulate its trajectory in flight. We demonstrate an ion rate of up to and achieve a fidelity for single ion operation of 98%. The technique can be used for all atomic species, which can be laser-cooled, and opens up new applications in ion microscopy, ion implantation and surface spectroscopy.
Using a segmented ion trap with mK laser-cooled ions we have realised a novel single ion source which can deterministically deliver a wide range of ion species, isotopes or ionic molecules [Schnitzler et al. Phys. Rev. Lett. 2009, 102, 070501]. Experimental data is discussed in detail and compared with numerical simulations of ion trajectories. For the novel ion source we numerically investigate the influence of various extraction parameters on fluctuations in velocity and position of the beam. We present specialised ion optics and show from numerical simulations that a nm spatial resolution is achievable. The Paul trap, which is used as a single ion source, together with the presented ion optics, constitutes a promising candidate for a deterministic ion implantation method for applications in solid state quantum computing or classical nano-electronic devices.
We report on the demonstration of a low emittance, high brightness ion source based on magneto-optically trapped neutral atoms. Our source has ion optical properties comparable to or better than those of the commonly used liquid metal ion source. In addition, it has several advantages that offer new possibilities, including high resolution ion microscopy with ion species tailored for specific applications, contamination-free ion milling, and nanoscale implantation of a variety of elements, either in large quantities, or one at a time, deterministically. Using laser-cooled Cr atoms, we create an ion beam with a normalized rms (root-mean-square) emittance of 6.0 x 10 (-7) mm mrad M e V and approximately 0.25 pA of current, yielding a brightness as high as 2.25 A cm (-2) sr (-1) eV (-1). These values of emittance and brightness show that, with suitable ion optics, an ion beam with a useful amount of current can be produced and focused to spot sizes of less than 1 nm.
The major challenge in improving deterministic single-ion sources is to control the position and momentum of each ion. Based on the extra information given by the electron created in a photoionization process, the trajectory of the correlated ion can be controlled, using a real-time feedback system. This versatile single-ion feedback control can be applied to different kinds of ion sources. This approach improves the spatial and temporal manipulation of charged particles (ions and electrons), and thus boosts applications in quantum technology and materials science, especially deterministic implantation.
The authors describe a new method for creating a high quality focused ion beam using laser-cooled neutral atoms in a magneto-optical trap as an ion source. They show that this new technique can provide spot resolutions and brightness values that are better than the state of the art in focused ion beams. The source can be used with a range of different ionic species and can be combined with laser cooling techniques to exert unprecedented control over the ion emission, for example, producing single ions “on demand.” The beam quality is a result of a high brightness and a narrow energy distribution, both of which stem from the cold temperature (≈100μK) of the atoms. The ions are produced by subjecting the cold neutral atoms to a photoionization laser, after which they become a compact source of nearly monoenergetic ions. With the application of a potential gradient, the ions form a beam that can be focused via standard ion optical techniques. They discuss estimations based on the initial size of the ion cloud and the energy distribution and show that the resulting beam has a low emittance.
Deterministic ion implantation and color-center creation methods at the nanometer scale provide a route towards scalable quantum information processing. For this purpose, we have developed an inherently deterministic single-ion implantation method based on a linear Paul trap (LPT) as a single-ion source since the laser-cooling technique can be applied to the trap system to obtain ultralow-emittance ions and manipulate single ions one by one . Doubly charged nitrogen ions (N2+) produced in a sputter ion source is introduced into the LPT and sympathetically cooled with laser-cooled calcium ions (Ca+). Both the sputter ion source and the LPT chamber are elevated to +50kV for the 100keV-implantation of doubly charged single ions into a grounded diamond crystal.
The manipulation of single-quantum objects is a key requirement for the engineering of microscopic quantum systems. Applications such as single-atom micromasers (microwave lasers), triggered single-photon sources, or deterministic entanglement of atoms all require the ability to deliver single atoms on demand to a desired location. The trapping and manipulation of atoms as neutral species is more challenging than for charged ions because of the weak interaction of neutral species with electromagnetic fields. Kuhr et al. (p. 278) have overcome these difficulties by combining magneto-optical trapping and optical-trapping techniques. They demonstrate the precision transport of single neutral cesium atoms over distances of 1 centimeter and the ejection of single atoms into free flight.