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arXiv:1708.03362

Quantum Lubricity

Tommaso Zanca, Franco Pellegrini, Giuseppe E. Santoro, Erio Tosatti

Published Aug 10, 2017• 0 citations
arXivHTMLPDF

Abstract

The quantum motion of nuclei, generally ignored in sliding friction, can become important for an atom, ion, or light molecule sliding in an optical lattice. The density-matrix-calculated evolution of a quantum Prandtl-Tomlinson model, describing the frictional dragging by an external force of a quantum particle, shows that classical predictions can be very wrong. The strongest quantum effect occurs not for weak, but for strong periodic potentials, where barriers are high but energy levels in each well are discrete, and resonant tunnelling to excited states in the nearest well can preempt classical stick-slip with great efficiency. The resulting permeation of otherwise impassable barriers is predicted to cause quantum lubricity

DOI
10.48550/arxiv.1708.03362

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The quantum motion of nuclei, generally ignored in sliding friction, can become important for an atom, ion, or light molecule sliding in an optical lattice. The density-matrix-calculated evolution of a quantum Prandtl-Tomlinson model, describing the frictional dragging by an external force of a quantum particle, shows that classical predictions can be very wrong. The strongest quantum effect occurs not for weak, but for strong periodic potentials, where barriers are high but energy levels in each well are discrete, and resonant tunnelling to excited states in the nearest well can preempt classical stick-slip with great efficiency. The resulting permeation of otherwise impassable barriers is predicted to cause quantum lubricity
The quantum motion of nuclei, generally ignored in the physics of sliding friction, can affect in an important manner the frictional dissipation of a light particle forced to slide in an optical lattice. The density matrix-calculated evolution of the quantum version of the basic Prandtl-Tomlinson model, describing the dragging by an external force of a point particle in a periodic potential, shows that purely classical friction predictions can be very wrong. The strongest quantum effect occurs not for weak but for strong periodic potentials, where barriers are high but energy levels in each well are discrete, and resonant Rabi or Landau-Zener tunneling to states in the nearest well can preempt classical stick-slip with nonnegligible efficiency, depending on the forcing speed. The resulting permeation of otherwise unsurmountable barriers is predicted to cause quantum lubricity, a phenomenon which we expect should be observable in the recently implemented sliding cold ion experiments.
Friction in atomistic systems is usually described by the classical Prandtl-Tomlinson model suitable for capturing the dragging force of a nanoparticle in a periodic potential. Here we consider the quantum mechanical version of this model in which the dissipation is facilitated by releasing heat to an external bath reservoir. The time evolution of the system is captured with the Liouville-von Neumann equation through the density matrix of the system in the Markov approximation. We examine several kinetic and dissipative properties of the nanoparticle by delineating classical vs quantum mechanical effects. We find that the Landau-Zener tunneling is a key factor in the overall reduction of the frictional dissipation when compared to the classical motion in which such tunneling is absent. Other regimes of motion, controlled by the corrugation parameter and other properties, are also found. This in-depth study analyzes the interplay between velocity, strength of interaction, and temperature to control the frictional force and provide useful guidelines for experimental data interpretation.
Nanoscaled friction is a fundamental tribological phenomenon with complex behavior of its dynamical force. Here, we utilize the Prandtl-Tomlinson framework to investigate systematically the different means of control of the frictional force at the quantum and classical levels. It is found that the frictional dynamics can be controlled by the corrugation and characteristic length ratio parameters dependent upon properties of the nanoparticle-chain system. In addition to the stick-slip regime, other types of motion are uncovered, highlighting the richness of the frictional dynamics. The importance of Landau-Zener tunneling for the quantum motion is also analyzed. These findings provide valuable insights for interpreting experimental observations and controlling quantum frictional behavior in nanoscale systems.