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Proceedings of the National Academy of Sciences

Frictional lubricity enhanced by quantum mechanics

Tommaso Zanca, Franco Pellegrini, Giuseppe E. Santoro, Erio Tosatti

Published Mar 19, 2018• 21 citations
Publisher

Abstract

The quantum motion of nuclei, generally ignored in the physics of sliding friction, can affect in an important manner the frictional dissipation of a light particle forced to slide in an optical lattice. The density matrix-calculated evolution of the quantum version of the basic Prandtl-Tomlinson model, describing the dragging by an external force of a point particle in a periodic potential, shows that purely classical friction predictions can be very wrong. The strongest quantum effect occurs not for weak but for strong periodic potentials, where barriers are high but energy levels in each well are discrete, and resonant Rabi or Landau-Zener tunneling to states in the nearest well can preempt classical stick-slip with nonnegligible efficiency, depending on the forcing speed. The resulting permeation of otherwise unsurmountable barriers is predicted to cause quantum lubricity, a phenomenon which we expect should be observable in the recently implemented sliding cold ion experiments.

DOI
10.1073/pnas.1801144115

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The quantum motion of nuclei, generally ignored in the physics of sliding friction, can affect in an important manner the frictional dissipation of a light particle forced to slide in an optical lattice. The density matrix-calculated evolution of the quantum version of the basic Prandtl-Tomlinson model, describing the dragging by an external force of a point particle in a periodic potential, shows that purely classical friction predictions can be very wrong. The strongest quantum effect occurs not for weak but for strong periodic potentials, where barriers are high but energy levels in each well are discrete, and resonant Rabi or Landau-Zener tunneling to states in the nearest well can preempt classical stick-slip with nonnegligible efficiency, depending on the forcing speed. The resulting permeation of otherwise unsurmountable barriers is predicted to cause quantum lubricity, a phenomenon which we expect should be observable in the recently implemented sliding cold ion experiments.
The quantum motion of nuclei, generally ignored in sliding friction, can become important for an atom, ion, or light molecule sliding in an optical lattice. The density-matrix-calculated evolution of a quantum Prandtl-Tomlinson model, describing the frictional dragging by an external force of a quantum particle, shows that classical predictions can be very wrong. The strongest quantum effect occurs not for weak, but for strong periodic potentials, where barriers are high but energy levels in each well are discrete, and resonant tunnelling to excited states in the nearest well can preempt classical stick-slip with great efficiency. The resulting permeation of otherwise impassable barriers is predicted to cause quantum lubricity
Nanoscaled friction is a fundamental tribological phenomenon with complex behavior of its dynamical force. Here, we utilize the Prandtl-Tomlinson framework to investigate systematically the different means of control of the frictional force at the quantum and classical levels. It is found that the frictional dynamics can be controlled by the corrugation and characteristic length ratio parameters dependent upon properties of the nanoparticle-chain system. In addition to the stick-slip regime, other types of motion are uncovered, highlighting the richness of the frictional dynamics. The importance of Landau-Zener tunneling for the quantum motion is also analyzed. These findings provide valuable insights for interpreting experimental observations and controlling quantum frictional behavior in nanoscale systems.
Friction in atomistic systems is usually described by the classical Prandtl-Tomlinson model suitable for capturing the dragging force of a nanoparticle in a periodic potential. Here we consider the quantum mechanical version of this model in which the dissipation is facilitated by releasing heat to an external bath reservoir. The time evolution of the system is captured with the Liouville-von Neumann equation through the density matrix of the system in the Markov approximation. We examine several kinetic and dissipative properties of the nanoparticle by delineating classical vs quantum mechanical effects. We find that the Landau-Zener tunneling is a key factor in the overall reduction of the frictional dissipation when compared to the classical motion in which such tunneling is absent. Other regimes of motion, controlled by the corrugation parameter and other properties, are also found. This in-depth study analyzes the interplay between velocity, strength of interaction, and temperature to control the frictional force and provide useful guidelines for experimental data interpretation.
The Landau criterion, a cornerstone of quantum fluid dynamics, dictates that dissipation is forbidden for uniform motion below a critical velocity. Yet, the fundamental question of how acceleration reshapes the principles of quantum friction has remained open since Landau and Pitaevskii's seminal works. Here, we establish a theoretical framework for the quantum tribology of non-inertial motion, describing a probe particle undergoing composite translation and rotation within a weakly interacting Bose condensate. Using the nonlinear Gross-Pitaevskii equation, we show that centripetal acceleration fundamentally modifies the energy-momentum constraints on elementary excitations. This leads to a finite drag force in the subsonic regime of the probe particle motion, and a characteristic quantum stick-slip behaviour in the deeply supersonic regime -- a direct generalization of the classical Landau-Pitaevskii picture. Beyond this dissipative response, we uncover a fundamentally distinct mechanism: the nonlinearity of the quantum fluid, combined with the broken symmetry of the trajectory, gives rise to a non-dissipative anomalous transverse force. This quantum Magnus-like response, emerging from the second-order density perturbation, performs no work and is rooted in the geometric asymmetry of the dynamically induced flow. Our findings lay the foundation for a universal program in quantum tribology of accelerated motion, establishing a direct and experimentally testable connection among non-inertial dynamics, nonlinear response, and topological symmetry breaking across platforms ranging from ultracold atoms and exciton-polariton condensates to cosmological analog systems.
Bodies in relative motion, spatially separated in vacuum, experience a tiny friction force known as quantum friction. This force has eluded experimental detection so far due to its small magnitude and short range. Herein, we give quantitative details so as to track traces of the quantum friction by measuring coherences in the atom. We notice that the environmentally induced decoherence can be decomposed into contributions of different signature: corrections induced by the electromagnetic vacuum in the presence of the dielectric sheet and those induced by the motion of the particle. In this direction, we show that noncontact friction enhances the decoherence of the moving atom. Further, its effect can be enlarged by a thorough selection of the two-level particle and the Drude-Lorentz parameters of the material. In this context, we suggest that measuring decoherence times through velocity dependence of coherences could indirectly demonstrate the existence of quantum friction.
Quantum decay rates for barrier potentials driven by external stochastic and periodic forces in the strong damping regime are studied. Based on the quantum Smoluchowski equation derived recently by Ankerhold, Pechukas, and Grabert [Phys. Rev. Lett. 87, 086802 (2001)] explicit analytical and numerical results are presented for the case of the resonant activation phenomenon in a bistable potential and the escape from a metastable well with oscillating barrier, respectively. The significant impact of quantum fluctuations is revealed.