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arXiv:1706.07018 · Physical Review Letters

Measurement-Induced Strong Kerr Nonlinearity for Weak Quantum States of Light

Luca S. Costanzo, A. S. Coelho, Nicola Biagi, Jaromı́r Fiurášek, Marco Bellini, Alessandro Zavatta

Published Jul 5, 2017• 50 citations
arXivHTMLPDF

Abstract

Strong nonlinearity at the single photon level represents a crucial enabling tool for optical quantum technologies. Here we report on experimental implementation of a strong Kerr nonlinearity by measurement-induced quantum operations on weak quantum states of light. Our scheme coherently combines two sequences of single photon addition and subtraction to induce a nonlinear phase shift at the single photon level. We probe the induced nonlinearity with weak coherent states and characterize the output non-Gaussian states with quantum state tomography. The strong nonlinearity is clearly witnessed as a change of sign of specific off-diagonal density matrix elements in the Fock basis.

DOI
10.1103/physrevlett.119.013601

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Any optical quantum information processing machine would be comprised of fully-characterized constituent devices for both single state manipulations and tasks involving the interaction between multiple quantum optical states. Ideally for the latter, would be an apparatus capable of deterministic optical phase shifts that operate on input quantum states with the action mediated solely by auxiliary signal fields. Here we present the complete experimental characterization of a system designed for optically controlled phase shifts acting on single-photon level probe coherent states. Our setup is based on a warm vapor of rubidium atoms under the conditions of electromagnetically induced transparency with its dispersion properties modified through the use of an optically triggered N-type Kerr non-linearity. We fully characterize the performance of our device by sending in a set of input probe states and measuring the corresponding output via time-domain homodyne tomography and subsequently performing the technique of coherent state quantum process tomography. This method provides us with the precise knowledge of how our optical phase shift will modify any arbitrary input quantum state engineered in the mode of the reconstruction.
Any optical quantum information processing machine would be comprised of fully-characterized constituent devices for both single state manipulations and tasks involving the interaction between multiple quantum optical states. Ideally for the latter, would be an apparatus capable of deterministic optical phase shifts that operate on input quantum states with the action mediated solely by auxiliary signal fields. Here we present the complete experimental characterization of a system designed for optically controlled phase shifts acting on single-photon level probe coherent states. Our setup is based on a warm vapor of rubidium atoms under the conditions of electromagnetically induced transparency with its dispersion properties modified through the use of an optically triggered N-type Kerr non-linearity. We fully characterize the performance of our device by sending in a set of input probe states and measuring the corresponding output via balanced homodyne tomography and subsequently performing the technique of coherent state quantum process tomography. This method provides us with the precise knowledge of how our optical phase shift will modify any arbitrary input quantum state engineered in the mode of the reconstruction.
Non-Gaussian states of light are a critical resource for fault-tolerant quantum computing and enhanced metrology, but are typically faint and often obtained via post-selection. Here, we demonstrate the deterministic generation of a bright non-Gaussian state by introducing a Kerr nonlinearity to a macroscopic state of light called bright squeezed vacuum (BSV). To characterize the resulting state, we use a single-shot f-2f interferometer to sample its Husimi function. We observe a clear transformation from a 2D Gaussian distribution to an 'S'-shaped non-Gaussian profile, which is the direct statistical evidence of the intensity-dependent nonlinear phase. The negativity of the Wigner function, which is an intrinsic property of any pure non-Gaussian state, cannot be observed because BSV is a mixed state even under minute optical loss. However, we show that BSV can be considered as a mixture of pure squeezed coherent states, for some of which Kerr-induced Wigner-function negativity is quite tolerant to loss. This work bridges the gap between quantum optics and ultrafast nonlinear optics, opening a path to quantum applications that require high photon flux.
We study the entanglement generated by a weak cross-Kerr nonlinearity between two initial coherent states, one of which has an amplitude close to the single-photon level, while the other one is macroscopic. We show that strong micro-macro entanglement is possible for weak phase shifts by choosing the amplitude of the macroscopic beam sufficiently large. We analyze the effects of loss and discuss possible experimental demonstrations of the micro-macro entanglement based on homodyne tomography and an entanglement witness. We also discuss the macroscopicity of the generated entanglement from the point of view of a recently proposed measure.
Conditional addition of photons represents a crucial tool for optical quantum state engineering and it forms a fundamental building block of advanced quantum photonic devices. Here we report on experimental implementation of the conditional addition of several photons. We demonstrate the addition of one, two, and three photons to input coherent states with various amplitudes. The resulting highly nonclassical photon-added states are completely characterized with time-domain homodyne tomography, and the nonclassicality of the prepared states is witnessed by the negativity of their Wigner functions. We experimentally demonstrate that the conditional addition of photons realizes approximate noiseless quantum amplification of coherent states with sufficiently large amplitude. We also investigate certification of the stellar rank of the generated multiphoton-added coherent states, which quantifies the non-Gaussian resources required for their preparation. Our results pave the way towards the experimental realization of complex optical quantum operations based on combination of multiple photon additions and subtractions.