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Scientific Reports

Quantum Process Tomography of an Optically-Controlled Kerr Non-linearity

Connor Kupchak, Samuel Rind, Bertus Jordaan, Eden V. Figueroa

Published Nov 20, 2015• 9 citations
Publisher

Abstract

Any optical quantum information processing machine would be comprised of fully-characterized constituent devices for both single state manipulations and tasks involving the interaction between multiple quantum optical states. Ideally for the latter, would be an apparatus capable of deterministic optical phase shifts that operate on input quantum states with the action mediated solely by auxiliary signal fields. Here we present the complete experimental characterization of a system designed for optically controlled phase shifts acting on single-photon level probe coherent states. Our setup is based on a warm vapor of rubidium atoms under the conditions of electromagnetically induced transparency with its dispersion properties modified through the use of an optically triggered N-type Kerr non-linearity. We fully characterize the performance of our device by sending in a set of input probe states and measuring the corresponding output via time-domain homodyne tomography and subsequently performing the technique of coherent state quantum process tomography. This method provides us with the precise knowledge of how our optical phase shift will modify any arbitrary input quantum state engineered in the mode of the reconstruction.

DOI
10.1038/srep16581

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In third order nonlinear mediums, the intensity of one optical field can modify the phase of another optical field. This is known as cross-phase modulation (XPM) and is important for Quantum Information Processing (QIP) as phase shifts of single-photons that exceed π rad can be used to implement two-qubit quantum logic gates. For a conventional XPM scheme, the Kerr nonlinearity responsible for XPM is too small for appreciable phase shifts to be achieved with low intensity optical fields. However, Electromagnetically Induced Transparency (EIT) can increase this nonlinearity by several orders of magnitude. This thesis discusses the experimental construction of a laser-atomic system capable of EIT modulated XPM. This includes construction of a rubidium magneto-optical trap (RbMOT), characterization of this RbMOT, demonstration of EIT in the RbMOT, and a system capable of detecting optical phase shifts produced by EIT. The talk will conclude with an outlook on further implementations to the experiment that will increase this nonlinearity such that phase shifts at the single-photon level are possible. | 76 pages

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Any optical quantum information processing machine would be comprised of fully-characterized constituent devices for both single state manipulations and tasks involving the interaction between multiple quantum optical states. Ideally for the latter, would be an apparatus capable of deterministic optical phase shifts that operate on input quantum states with the action mediated solely by auxiliary signal fields. Here we present the complete experimental characterization of a system designed for optically controlled phase shifts acting on single-photon level probe coherent states. Our setup is based on a warm vapor of rubidium atoms under the conditions of electromagnetically induced transparency with its dispersion properties modified through the use of an optically triggered N-type Kerr non-linearity. We fully characterize the performance of our device by sending in a set of input probe states and measuring the corresponding output via time-domain homodyne tomography and subsequently performing the technique of coherent state quantum process tomography. This method provides us with the precise knowledge of how our optical phase shift will modify any arbitrary input quantum state engineered in the mode of the reconstruction.
Any optical quantum information processing machine would be comprised of fully-characterized constituent devices for both single state manipulations and tasks involving the interaction between multiple quantum optical states. Ideally for the latter, would be an apparatus capable of deterministic optical phase shifts that operate on input quantum states with the action mediated solely by auxiliary signal fields. Here we present the complete experimental characterization of a system designed for optically controlled phase shifts acting on single-photon level probe coherent states. Our setup is based on a warm vapor of rubidium atoms under the conditions of electromagnetically induced transparency with its dispersion properties modified through the use of an optically triggered N-type Kerr non-linearity. We fully characterize the performance of our device by sending in a set of input probe states and measuring the corresponding output via balanced homodyne tomography and subsequently performing the technique of coherent state quantum process tomography. This method provides us with the precise knowledge of how our optical phase shift will modify any arbitrary input quantum state engineered in the mode of the reconstruction.
Conditional quantum optical processes enable a wide range of technologies from generation of highly non-classical states to implementation of quantum logic operations. The process fidelity that can be achieved in a realistic implementation depends on a number of system parameters. Here we experimentally examine Fock state filtration, a canonical example of a broad class of conditional quantum operations acting on a single optical field mode. This operation is based upon interference of the mode to be manipulated with an auxiliary single-photon state at a beam splitter, resulting in the entanglement of the two output modes. A conditional projective measurement onto a single photon state at one output mode heralds the success of the process. This operation, which implements a measurement-induced nonlinearity, is capable of suppressing particular photon-number probability amplitudes of an arbitrary quantum state. We employ coherent-state process tomography to determine the precise operation realized in our experiment, which is mathematically represented by a process tensor. To identify the key sources of experimental imperfection, we develop a realistic model of the process and identify three main contributions that significantly hamper its efficacy. The experimentally reconstructed process tensor is compared with the model, yielding a fidelity better than 0.95. This enables us to identify three key challenges to overcome in realizing a filter with optimal performance—namely the single-photon nature of the auxiliary state, high mode overlap of the optical fields involved, and the need for photon-number-resolving detection when heralding. The results show that the filter does indeed exhibit a non-linear response as a function of input photon number and preserves the phase relation between Fock layers of the output state, providing promise for future applications.
This thesis introduces and implements a characterization procedure called coherent state quantum process tomography and applies it to a selection of quantum operations. The procedure holds advantages over previous quantum process tomography methods, a pri- mary one is that a process can be characterized by measuring its effect on a set of coherent states which are readily available from a laser source. After introduction of the characterization procedure, the method is tested on a simple process of an electro-optical modulator and polarizing beam splitter. The accuracy of the characterization is verified by comparison of the predicted action of the reconstructed process tensor versus the actual experiment involving a squeezed vacuum state. The algorithm is then implemented and verified on a quantum memory system based on electromagnetically induced transparency, a system that was previously shown capable of storing a squeezed vacuum state. Lastly, a new optical storage system based on a gradient echo memory scheme is con- structed and optimized to achieve memory retrieval efficiencies of >80%. To characterize this system, a modified coherent state quantum process tomography algorithm based on the method of maximum likelihood estimation is employed. Despite the high efficiency values, the presence of excess noise resulted in the degradation of the storage device per- formance to be below the benchmarks of a quantum memory system. This estimation algorithm is also successfully implemented on the non-deterministic processes of photon creation and annihilation.
This thesis is concerned with the generation of non-classical quantum states of light, the photon-level manipulation of quantum states and the accurate tomography of both quantum states and quantum processes. In optics, quantum information can be encoded and processed in both discrete and continuous variables. Hybrid approaches combining for example homodyne detection with conditional state preparation and manipulation are gaining increasing prominence. The development and characterization of a time-domain balanced homodyne detector (BHD) is presented. The detector has a bandwidth of 80 MHz, a signal-to-noise ratio of 14.5 dB and an efficiency of 86% making it well-suited to pulse-to-pulse measurement of quantum optical states. The BHD is employed to perform quantum state tomography (QST) of non-classical multi-photon Fock states generated by spontaneous parametric down-conversion. A detailed investigation of the mode-matching between the local oscillator used for homodyne detection and the generated Fock states is presented. The one-, two- and three-photon Fock states are reconstructed with a combined preparation and detection efficiency exceeding 50%. Fock states have a number of applications in quantum state engineering, where non-classical ancilla states and conditional measurements enable photon-level manipulation of quantum states. Fock state filtration (FSF) is investigated - an example of a post-selected beam splitter which is a basic building block for many quantum state engineering protocols. A model is developed incorporating the effect of experimental imperfections. An experimental implementation of a Fock state filter is fully characterized by means of coherent-state quantum process tomography (QPT). The reconstructed process is found to be consistent with the model. The filter preferentially removes the single-photon component from an arbitrary input quantum state. Calibration of optical detectors in the quantum regime is discussed. Quantum detector tomography (QDT) is reviewed and contrasted with a new technique for performing QST with a calibrated detector known as the fitting of data patterns (FDP). The first experimental characterization of a BHD is performed by probing the detector with phase-averaged coherent states. The FDP method is shown to be applicable to the estimation of quantum processes, where a detector response is not assumed - thus demonstrating the versatility of the FDP approach as a new method in the quantum tomography toolbox.
We review the method for characterizing, with arbitrarily high accuracy, any quantum optical process, which our group has developed over the past few years. Our protocol recovers complete knowledge of the process by studying, via homodyne tomography, its effect on a set of coherent states, that is, classical fields produced by common laser sources. We present a simple scheme for calculating the process matrix from this information. We demonstrate the capability of our protocol by demonstrating complete characterization of an optical memory based on electromagnetically induced transparency.
In third order nonlinear mediums, the intensity of one optical field can modify the phase of another optical field. This is known as cross-phase modulation (XPM) and is important for Quantum Information Processing (QIP) as phase shifts of single-photons that exceed π rad can be used to implement two-qubit quantum logic gates. For a conventional XPM scheme, the Kerr nonlinearity responsible for XPM is too small for appreciable phase shifts to be achieved with low intensity optical fields. However, Electromagnetically Induced Transparency (EIT) can increase this nonlinearity by several orders of magnitude. This thesis discusses the experimental construction of a laser-atomic system capable of EIT modulated XPM. This includes construction of a rubidium magneto-optical trap (RbMOT), characterization of this RbMOT, demonstration of EIT in the RbMOT, and a system capable of detecting optical phase shifts produced by EIT. The talk will conclude with an outlook on further implementations to the experiment that will increase this nonlinearity such that phase shifts at the single-photon level are possible. | 76 pages