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arXiv:1704.03250 · Physical review. B./Physical review. B

Spectral functions of a time-periodically driven Falicov-Kimball model: Real-space Floquet dynamical mean-field theory study

Tao Qin, Walter Hofstetter

Published Aug 16, 2017• 24 citations
arXivHTMLPDF

Abstract

We present a systematic study of the spectral functions of a time-periodically driven Falicov-Kimball Hamiltonian. In the high-frequency limit, this system can be effectively described as a Harper-Hofstadter-Falicov-Kimball model. Using real-space Floquet dynamical mean-field theory (DMFT), we take into account the interaction effects and contributions from higher Floquet bands in a nonperturbative way. Our calculations show a high degree of similarity between the interacting driven system and its effective static counterpart with respect to spectral properties. However, as also illustrated by our results, one should bear in mind that Floquet DMFT describes a nonequilibrium steady state, while an effective static Hamiltonian describes an equilibrium state. We further demonstrate the possibility of using real-space Floquet DMFT to study edge states on a cylinder geometry.

DOI
10.1103/physrevb.96.075134

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We present a systematic study of the spectral functions of a time-periodically driven Falicov-Kimball Hamiltonian. In the high-frequency limit, this system can be effectively described as a Harper-Hofstadter-Falicov-Kimball model. Using real-space Floquet dynamical mean-field theory (DMFT), we take into account the interaction effects and contributions from higher Floquet bands in a nonperturbative way. Our calculations show a high degree of similarity between the interacting driven system and its effective static counterpart with respect to spectral properties. However, as also illustrated by our results, one should bear in mind that Floquet DMFT describes a nonequilibrium steady state, while an effective static Hamiltonian describes an equilibrium state. We further demonstrate the possibility of using real-space Floquet DMFT to study edge states on a cylinder geometry.
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We give a general overview of the high-frequency regime in periodically driven systems and identify three distinct classes of driving protocols in which the infinite-frequency Floquet Hamiltonian is not equal to the time-averaged Hamiltonian. These classes cover systems, such as the Kapitza pendulum, the Harper–Hofstadter model of neutral atoms in a magnetic field, the Haldane Floquet Chern insulator and others. In all setups considered, we discuss both the infinite-frequency limit and the leading finite-frequency corrections to the Floquet Hamiltonian. We provide a short overview of Floquet theory focusing on the gauge structure associated with the choice of stroboscopic frame and the differences between stroboscopic and non-stroboscopic dynamics. In the latter case, one has to work with dressed operators representing observables and a dressed density matrix. We also comment on the application of Floquet Theory to systems described by static Hamiltonians with well-separated energy scales and, in particular, discuss parallels between the inverse-frequency expansion and the Schrieffer–Wolff transformation extending the latter to driven systems.
In order to investigate photoinduced insulator-metal transitions observed in correlated electron systems, we propose a new theoretical method, where we combine a Floquet-matrix method for AC-driven systems with the dynamical mean-field theory. The method can treat nonequilibrium steady states exactly beyond the linear-response regime. We have applied the method to the Falicov-Kimball model coupled to AC electric fields, and numerically obtained the spectral function, the nonequilibrium distribution function and the current-voltage characteristic. The results show that intense AC fields indeed drive Mott-like insulating states into photoinduced metallic states in a nonlinear way.
Time-periodically driven systems are a versatile toolbox for realizing interesting effective Hamiltonians. Heating, caused by excitations to high-energy states, is a challenge for experiments. While most setups so far address the relatively weakly interacting regime, it is of general interest to study heating in strongly correlated systems. Using Floquet dynamical mean-field theory, we study nonequilibrium steady states (NESS) in the Falicov-Kimball model, with time-periodically driven kinetic energy or interaction. We systematically investigate the nonequilibrium properties of the NESS. For a driven kinetic energy, we show that resonant tunneling, where the interaction is an integer multiple of the driving frequency, plays an important role in the heating. In the strongly correlated regime, we show that this can be well understood using Fermi's golden rule and the Schrieffer-Wolff transformation for a time-periodically driven system. We furthermore demonstrate that resonant tunneling can be used to control the population of Floquet states to achieve ``photodoping.'' For driven interactions introduced by an oscillating magnetic field near a widely adopted Feshbach resonance, we find that the double occupancy is strongly modulated. Our calculations apply to shaken ultracold-atom systems and to solid-state systems in a spatially uniform but time-dependent electric field. They are also closely related to lattice modulation spectroscopy. Our calculations are helpful to understand the latest experiments on strongly correlated Floquet systems.
In this paper, we investigate periodically driven open quantum systems within the framework of Floquet-Lindblad master equations. Specifically, we discuss Lindblad master equations in the presence of a coherent, time-periodic driving and establish their general spectral features. We also clarify the notions of transient and nondecaying solutions from this spectral perspective, and then prove that any physical system described by a Floquet-Lindblad equation must have at least one physical nonequilibrium steady state (NESS), corresponding to an eigenoperator of the Floquet-Lindblad evolution superoperator UF{\mathcal{U}}_{F}UF​ with unit eigenvalue. Since the Floquet-Lindblad formalism encapsulates the entire information regarding the NESS, it in principle enables us to obtain nonlinear effects to all orders at once. The Floquet-Lindblad formalism thus provides a powerful tool for studying driven-dissipative solid-state systems, which we illustrate by deriving the nonlinear optical response of a simple two-band model of an insulating solid and comparing it with prior results established through Keldysh techniques.
We study the circularly driven Falicov-Kimball model on a honeycomb lattice within real space Floquet dynamical mean field theory (DMFT). The noninteracting version of this model has been realized experimentally. The noninteracting system hosts an effective Haldane phase at large driving frequencies, while at intermediate frequencies it hosts an anomalous topological phase. We study the effect of two-body interactions UUU on the stability of these phases. We find that charge pumping does not remain quantized upon increasing UUU, despite the presence of edge modes in the spectrum. This can be attributed to the broadening of the edge modes due to interaction. We also calculate the rate of energy dissipation into the bath and find remarkably different behaviour in the two regimes.