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arXiv:1703.06232 · Physical review. B./Physical review. B

Entanglement of condensed magnons via momentum-space fragmentation

Clement H. Wong, Ari Mizel

Published Aug 9, 2017• 3 citations
arXivHTMLPDF

Abstract

A scheme is presented for engineering momentum-space entanglement of fragmented magnon condensates. We consider easy-plane frustrated antiferromagnets in which the magnon dispersion has degenerate minima that represent ``umbrella'' chiral spin textures. We tune the Hamiltonian near a quantum critical point that is signaled by a singularity in the entanglement entropy. The ground state develops momentum-space entanglement of the chiral spin textures. The size of the entangled superposition is accessible experimentally through the magnetic structure factor. Our model is motivated by equilibrium magnon condensates in frustrated antiferromagnets such as ${\mathrm{CsCuCl}}_{3}$, and it can also be simulated in spin-orbit coupled Mott insulators in atomic optical lattices and circuit quantum electrodynamics.

DOI
10.1103/physrevb.96.054412

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A scheme is presented for engineering momentum-space entanglement of fragmented magnon condensates. We consider easy-plane frustrated antiferromagnets in which the magnon dispersion has degenerate minima that represent ``umbrella'' chiral spin textures. We tune the Hamiltonian near a quantum critical point that is signaled by a singularity in the entanglement entropy. The ground state develops momentum-space entanglement of the chiral spin textures. The size of the entangled superposition is accessible experimentally through the magnetic structure factor. Our model is motivated by equilibrium magnon condensates in frustrated antiferromagnets such as CsCuCl3{\mathrm{CsCuCl}}_{3}CsCuCl3​, and it can also be simulated in spin-orbit coupled Mott insulators in atomic optical lattices and circuit quantum electrodynamics.
Quantum phase transition at the saturation field is studied for a class of frustrated quantum antiferromagnets. The considered models include (i) the ${J}_{1}\mathrm{\text{\ensuremath{-}}}{J}_{2}$ frustrated square-lattice antiferromagnet with J2=12J1{J}_{2}=\frac{1}{2}{J}_{1}J2​=21​J1​ and (ii) the nearest-neighbor Heisenberg antiferromagnet on a face centered cubic lattice. In the fully saturated phase the magnon spectra for the two models have lines of degenerate minima. Transition into a partially magnetized state is treated via a mapping to a dilute gas of hard-core bosons and by complementary spin-wave calculations. Momentum dependence of the exact four-point boson vertex removes the degeneracy of the single-particle excitation spectra and selects the ordering wave vectors at $(\ensuremath{\pi},\ensuremath{\pi})$ and $(\ensuremath{\pi},0,0)$ for the two models. We predict a unique form for the magnetization curve $\ensuremath{\Delta}M=S\ensuremath{-}M\ensuremath{\simeq}{\ensuremath{\mu}}^{(d\ensuremath{-}1)/2}(\mathrm{log}\ensuremath{\mu}{)}^{(d\ensuremath{-}1)}$, where $\ensuremath{\mu}$ is a distance from the quantum critical point.
The influence of magnon bands on entanglement in the antiferromagnetic XXZ model on a triangular lattice, which models the bilayer structure consisting of an antiferromagnetic insulator and normal metal, is investigated. This effect was studied in ferromagnetic as well as antiferromagnetic triangular lattices. Quantum entanglement measures given by the entanglement negativity have been studied, where a magnon current is induced in the antiferromagnet due to interfacial exchange coupling between localized spins in the antiferromagnet and itinerant electrons in a normal metal. Moreover, quantum correlations in other frustrated models, namely the metal-insulation antiferromagnetic bilayer model and the Heisenberg model with biquadratic and bicubic interactions, are analyzed.
The chiral Luttinger liquid develops quantum chaos as soon as a—however slight—nonlinear dispersion is introduced for the microscopic electronic degrees of freedom. For this nonlinear version of the model, we identify an infinite family of translation-invariant interaction potentials with corresponding modulated symmetries. These symmetries are highly unconventional: they are modulated in momentum space (and do not seem to have an easy physical interpretation). We develop a systematic understanding of these symmetries and study the resulting blocks in the Hamiltonian. In particular, this approach allows us to predict the analytic Hamiltonian block sizes and derive asymptotic scaling laws in the limit of large total momentum. These blocks are reminiscent of Hilbert space fragmentation in that, even though they are labeled by a symmetry, this symmetry is highly nonlocal and does not have a simple interpretation. We corroborate this result by studying entanglement entropy and level statistics.
This thesis investigates quantum magnetism in two-dimensional synthetic systems, where strong correlations, geometric frustration, and enhanced quantum fluctuations produce unconventional magnetic phases. I focus on two major classes of engineered platforms: moiré materials and quantum simulators, which offer precise control over lattice geometry, interaction strengths, and dynamics, enabling access to regimes beyond conventional condensed-matter approaches. The first project studies moiré magnetism in strained multilayers of CrBr₃, where strain generates a spatial modulation of the interlayer exchange alternating between ferromagnetic and antiferromagnetic. With S=3/2 moments, the system admits a classical bilayer description with competing interactions. I develop a theoretical framework capturing the resulting non-collinear orders and reproducing experimental signatures, demonstrating how moiré engineering stabilizes non-trivial magnetic textures. The second project examines quantum magnetism in a WSe₂/WS₂ heterobilayer at three-quarters filling, where electrons form an effective kagome lattice. From the underlying Hubbard model, I derive a frustrated Heisenberg Hamiltonian with competing exchanges. Using Schwinger-boson mean-field theory, I map a phase diagram of non-collinear orders and spin-liquid phases. For realistic parameters, the ground state is a chiral spin liquid, highlighting transition-metal dichalcogenide moiré materials as platforms for topological and strongly correlated magnetism. The third project investigates quantum phase-transition dynamics with superconducting circuit quantum simulators, focusing on Hamiltonian ramps in the 2D XY model. An analogue-digital protocol drives the system from a gapped staggered state to the gapless XY phase. Analysis of correlations reveals scaling of the correlation length with ramp rate, broadly consistent with Kibble–Zurek predictions, with deviations reflecting finite-size, dimensionality, and experimental constraints. The fourth project develops a Holstein–Primakoff spin-wave description for the same XY ramps. Adapting the quantization axis to the instantaneous magnetization, this solvable quadratic theory provides magnon dispersions, time- and space-dependent correlations, and single-magnon dynamics, including decay and scattering. This framework offers a detailed picture of non-equilibrium quasiparticle behavior in a 2D magnet under time-dependent fields. Together, these projects show how moiré materials and quantum simulators enable controlled studies of frustrated and strongly correlated magnetism in two dimensions. By combining analytical modeling with experimentally relevant conditions, this thesis advances understanding of how frustration, topology, and non-equilibrium dynamics shape quantum magnetic phenomena in low-dimensional systems.
We study momentum-space entanglement in quantum spin-half ladders consisting of two coupled critical XXZXXZXXZ spin-half chains, using field theoretical methods developed by Lundgren et al. [Phys. Rev. B 88, 245137 (2013)] and exact diagonalization. When the system is gapped, we analytically find that the momentum-space entanglement Hamiltonian is described by a chiral conformal field theory with a central charge of 2. This is in contrast to entanglement Hamiltonians of various real-space partitions of gapped-spin ladders that have a central charge of 1. When the system is gapless, the entanglement Hamiltonian consists of one gapless mode that is linear in subsystem momentum and one mode with a flat dispersion relation. In the gapless region, we extend the work of Lundgren et al. to include the effect of a certain irrelevant term on the entanglement spectrum. In both the gapless and gapped phases, the momentum-space entanglement entropy obeys a volume law. In the gapless region, we find a subleading constant term in the entanglement entropy which contains information about the underlying field theory of the system. The analytical predictions for the entanglement spectrum are consistent with results from exact diagonalization.
Fractionalized excitations develop in many unusual many-body states such as quantum spin liquids, disordered phases that cannot be described using any local order parameter. Because these exotic excitations correspond to emergent degrees of freedom, how to probe them and establish their existence is a long-standing challenge. We present a general procedure to reveal the fractionalized excitations using real-space entanglement entropy in critical spin liquids that are particularly relevant to experiments. Moreover, we show how to use the entanglement entropy to construct the corresponding spinon Fermi surface. Our work defines a new pathway to establish and characterize exotic excitations in novel quantum phases of matter.