This thesis investigates quantum magnetism in two-dimensional synthetic systems, where strong correlations, geometric frustration, and enhanced quantum fluctuations produce unconventional magnetic phases. I focus on two major classes of engineered platforms: moiré materials and quantum simulators, which offer precise control over lattice geometry, interaction strengths, and dynamics, enabling access to regimes beyond conventional condensed-matter approaches. The first project studies moiré magnetism in strained multilayers of CrBr₃, where strain generates a spatial modulation of the interlayer exchange alternating between ferromagnetic and antiferromagnetic. With S=3/2 moments, the system admits a classical bilayer description with competing interactions. I develop a theoretical framework capturing the resulting non-collinear orders and reproducing experimental signatures, demonstrating how moiré engineering stabilizes non-trivial magnetic textures. The second project examines quantum magnetism in a WSe₂/WS₂ heterobilayer at three-quarters filling, where electrons form an effective kagome lattice. From the underlying Hubbard model, I derive a frustrated Heisenberg Hamiltonian with competing exchanges. Using Schwinger-boson mean-field theory, I map a phase diagram of non-collinear orders and spin-liquid phases. For realistic parameters, the ground state is a chiral spin liquid, highlighting transition-metal dichalcogenide moiré materials as platforms for topological and strongly correlated magnetism. The third project investigates quantum phase-transition dynamics with superconducting circuit quantum simulators, focusing on Hamiltonian ramps in the 2D XY model. An analogue-digital protocol drives the system from a gapped staggered state to the gapless XY phase. Analysis of correlations reveals scaling of the correlation length with ramp rate, broadly consistent with Kibble–Zurek predictions, with deviations reflecting finite-size, dimensionality, and experimental constraints. The fourth project develops a Holstein–Primakoff spin-wave description for the same XY ramps. Adapting the quantization axis to the instantaneous magnetization, this solvable quadratic theory provides magnon dispersions, time- and space-dependent correlations, and single-magnon dynamics, including decay and scattering. This framework offers a detailed picture of non-equilibrium quasiparticle behavior in a 2D magnet under time-dependent fields. Together, these projects show how moiré materials and quantum simulators enable controlled studies of frustrated and strongly correlated magnetism in two dimensions. By combining analytical modeling with experimentally relevant conditions, this thesis advances understanding of how frustration, topology, and non-equilibrium dynamics shape quantum magnetic phenomena in low-dimensional systems.
This thesis investigates quantum magnetism in two-dimensional synthetic systems, where strong correlations, geometric frustration, and enhanced quantum fluctuations produce unconventional magnetic phases. I focus on two major classes of engineered platforms: moiré materials and quantum simulators, which offer precise control over lattice geometry, interaction strengths, and dynamics, enabling access to regimes beyond conventional condensed-matter approaches. The first project studies moiré magnetism in strained multilayers of CrBr₃, where strain generates a spatial modulation of the interlayer exchange alternating between ferromagnetic and antiferromagnetic. With S=3/2 moments, the system admits a classical bilayer description with competing interactions. I develop a theoretical framework capturing the resulting non-collinear orders and reproducing experimental signatures, demonstrating how moiré engineering stabilizes non-trivial magnetic textures. The second project examines quantum magnetism in a WSe₂/WS₂ heterobilayer at three-quarters filling, where electrons form an effective kagome lattice. From the underlying Hubbard model, I derive a frustrated Heisenberg Hamiltonian with competing exchanges. Using Schwinger-boson mean-field theory, I map a phase diagram of non-collinear orders and spin-liquid phases. For realistic parameters, the ground state is a chiral spin liquid, highlighting transition-metal dichalcogenide moiré materials as platforms for topological and strongly correlated magnetism. The third project investigates quantum phase-transition dynamics with superconducting circuit quantum simulators, focusing on Hamiltonian ramps in the 2D XY model. An analogue-digital protocol drives the system from a gapped staggered state to the gapless XY phase. Analysis of correlations reveals scaling of the correlation length with ramp rate, broadly consistent with Kibble–Zurek predictions, with deviations reflecting finite-size, dimensionality, and experimental constraints. The fourth project develops a Holstein–Primakoff spin-wave description for the same XY ramps. Adapting the quantization axis to the instantaneous magnetization, this solvable quadratic theory provides magnon dispersions, time- and space-dependent correlations, and single-magnon dynamics, including decay and scattering. This framework offers a detailed picture of non-equilibrium quasiparticle behavior in a 2D magnet under time-dependent fields. Together, these projects show how moiré materials and quantum simulators enable controlled studies of frustrated and strongly correlated magnetism in two dimensions. By combining analytical modeling with experimentally relevant conditions, this thesis advances understanding of how frustration, topology, and non-equilibrium dynamics shape quantum magnetic phenomena in low-dimensional systems.
Frustrated magnetism provides a rich platform for realizing exotic quantum phases in condensed matter systems. Among these, quantum spin liquids (QSLs) are a particularly intriguing class of states that exhibit no magnetic ordering and preserve all symmetries down to zero temperature. Just as conventional magnets can be thought of as spin crystals,QSLs represent their liquid analogs. This thesis explores two broad types of QSLs in two-dimensional magnets, with a focus on their dynamic properties and the nature of transitions from conventional magnetic states into QSL phases. QSLs are topological phases that host fractionalized excitations known as spinons. In these states, mobile spinons are coupled to an emergent gauge field, forming a highly entangled phase of matter. The first part of this thesis focuses on Dirac spin liquids (DSLs), a class of QSLs where spinons exhibit a gapless Dirac dispersion. To study the dynamicsof these spin liquids beyond leading-order mean-field theory, we develop a novel large-N fermionic limit of gapless spinons. In this limit, all gauge excitations are suppressed, and the leading-order corrections instead arise from order parameter fluctuations, which may condense and drive transitions into symmetry-broken phases from the parent DSL. Incorporating random phase approximation (RPA) corrections to the spin susceptibility, we find that sharp, spin-wave–like modes are recovered in the excitation spectrum. This methodology successfully captures characteristic features of the dynamics near phase transitions and in weakly symmetry-broken phases proximate to a DSL. We apply this approach to microscopic models, including the J1-J2 XXZ model on the triangular lattice and the J1-J3 XXZ model on the honeycomb lattice. These models closely represent a wide range of frustrated materials, such as triangular and honeycomb cobaltates and triangular ytterbium compounds. Our theoretical predictions show excellent agreement with experimentally measured inelastic neutron scattering spectra from these materials. Gapless spinons can also sometimes become gapped through chiral symmetry breaking, leading to the formation of a chiral spin liquid (CSL). The CSL is an archetypal bosonic realization of a fractional quantum Hall (FQH) state at half-filling, and has been proposed as a time-reversal–breaking ground state in a variety of frustrated spin models. The second part of this thesis addresses the intriguing possibility of realizing a CSL through the "melting" of a chiral spin crystal—a conventional magnet with non-coplanar ordering. Such a transition offers a physically appealing analogue to the melting of a Wigner crystal into a fermionic FQH liquid. Focusing on the kagome lattice, where chiral interactions are knownto stabilize a CSL ground state, we study the effects of additional long-range Heisenberg interactions and demonstrate a phase transition into a non-coplanar octahedral magnetic order. To describe the universal class of transition between a CSL and a non-coplanar anti-ferromagnetic order, we then develop a novel Chern-Simons–matter field theory framework, constrained by symmetry principles and symmetry fractionalization patterns. This thesis thus provides new insights into the dynamical signatures and phase transitions of quantum spin liquids, offering a bridge between theoretical models and experimental observations in frustrated magnetic systems.
The quantum nature of electrons emerges in various exotic ways when they are put together with quantum many-body interactions. In Mott insulating systems with strong electron correlation, frustration and strong quantum fluctuations promote localized electron spins to form nontrivial quantum paramagnetic phases such as quantum spin liquid and valence bond solid preventing the development of conventional magnetic orders. In this thesis, we study such exotic quantum phases in various different frustrated quantum magnets. First, encouraged by the spin liquid phenomenology observed in Ba3XSb2O9 (X=Cu, Ni), we investigate Z2 spin liquids on a three dimensional triangular lattice by employing the Schwinger boson mean-field theory with projective symmetry group analysis. It is found that a nematic spin liquid is energetically favorable on this lattice structure rather than symmetric spin liquids. Next, we study various valence bond solid phases that can appear in kagome lattice antiferromagnets by generalizing the recently proposed phenomenological Z2 gauge theory for the topological Z2 spin liquid state found in the nearest-neighbor kagome lattice Heisenberg model. This work provides a bridge between the topological spin liquid and valence bond solid phases previously proposed for kagome lattice antiferromagnets via vison condensation in the gauge theory. Then, we consider optical conductivity in Mott insulators as an experimental probe to detect quantum paramagnetic phases like valence bond solid. Applying this idea to deformed kagome lattice antiferromagnet Rb2Cu3SnF12 with a 12-site valence bond solid state, we estimate the size of optical conductivity in this quantum magnet. After this, another quantum paramagnet BiCu2PO6 is carefully investigated to clarify its puzzling ground state nature and quasiparticle excitations. Utilizing recent high resolution neutron scattering data, we construct a microscopic spin model and also an effective theory for the low energy spin excitations in the compound. We find significant influences of magnetic anisotropies on the ground state and quasiparticle dynamics. Lastly, we investigate emergent quantum phases in the thin film geometries of the pyrochlore iridates, where a number of exotic quantum ground states are proposed to occur in bulk materials as a result of the interplay between electron correlation and strong spin-orbit coupling. The fate of these bulk phases, as well as the novel quantum states that may arise only in a thin film setting, are studied via a theoretical model that allows layer-dependent magnetic structures.
This thesis makes three contributions to the understanding, control, and design of strongly correlated quantum matter. First, motivated by recent experiments reporting light-induced superconductivity, magnetism, and charge order, this thesis develops a unified description of photoexcited quantum materials. We show that seemingly disparate nonequilibrium phenomena can often be interpreted in terms of emergent order parameters and their collective dynamical fluctuations, providing a framework for modeling complex driven many-body systems with competing equilibrium phases. We propose experimental tests of this framework, several of which have already been realized, and highlight the role of programmable quantum simulators as platforms for studying driven many-body physics and probing emergent nonequilibrium order. Second, the thesis investigates atomically thin materials, with a primary focus on transition metal dichalcogenides (TMDs), as a platform for exploring strongly interacting quantum matter and for designing electro-optical quantum devices. In addition to electrical tunability, TMDs are direct band-gap semiconductors exhibiting sharp excitonic resonances in the optical frequency range, enabling optical manipulation of these materials. At relevant carrier densities, interactions dominate, leading to rich and unconventional behavior. To this end, we report the observation of Wigner crystallization, interlayer electron coherence, magnon hydrodynamics, and excitonic superradiance. Finally, motivated by rapid progress in programmable neutral-atom quantum simulation and computation, this thesis introduces a general algorithmic framework for {\it inverse quantum simulation} aimed at quantum material design. Target material characteristics are encoded as a cost function, which is minimized on quantum hardware to prepare a many-body state with the desired properties in quantum memory. Hamiltonian learning is then used to reconstruct a low-energy Hamiltonian for which this state is an approximate ground state, yielding a physically interpretable model that can guide experimental realization. This framework extends the scope of quantum simulators from exploring quantum many-body systems to designing and discovering new quantum materials.
The study of topological magnetic excitations have attracted widespread attention in the past few years.The wide variety of ground state phases realized in different two-dimensional magnets have emerged as versatile platforms for realizing magnetic analogues of topological phases uncovered in electronic systems over the past two decades.Dzyaloshinskii-Moriya(DM) interactions, that are ubiquitous in many quantum magnets, and has been demonstrated to induce a non-trivial topology in the magnetic excitations in many quantum magnets.In particular, signatures of DM-interaction induced topological features observed in the dispersion of magnetic excitations in the geometrically frustrated Shastry-Sutherland compound SrCu 2 (BO 3 ) 2 and honeycomb ferromagnet CrI 3 have provided the motivation behind the bulk of the research presented in this thesis.In the first chapter we introduce the background and motivation of our study.We showed that the vastly available materials with a possibility of nonzero symmetry allowed DM-interaction motivate us to study the minimal models of interacting spins related to the materials.In the second chapter we have described the methods that is used to study the spin systems.To describe the spin excitations in the long-range ordered system and dimerized system, we use Holstein-Primakoff transformation and bond-operator formalism respectively.The Schwinger Boson mean field theory is applicable for any generic magnetic ground state and useful to study the system at high temperatures compared with Holstein-Primakoff transformation.After transforming the Hamiltonian into a quadratic bosonic Hamiltonian, it is diagonalized by using Bogoliubov-Valatin transformation.Different observables like Berry-curvature, Chern-number, Dynamical Spin structure factor etc. are cal-vii culated by using the single particle wave-function obtained from Bogoliubov-Valatin transformation.A non-zero Berry curvature is a signature of topologically protected edge states in a stripe geometry of a lattice and a systematic way of calculating edge states is also explained in the second chapter.Moreover in the second chapter the usefulness of symmetry in obtaining band degeneracies and the allowed spin-spin interaction terms are also described.The past theoretical studies show the presence of topological magnons in honeycomb ferromagnetic models due to presence of DM-interaction on a next-nearest neighbour bonds.Recently this kind of DM-interaction is detected in the honeycomb ferromagnet CrI 3 .This type of DM-interaction induces chiral edge states of magnon in the system and so we named it as chiral DM-interaction.In the third chapter we show that breaking of inversion symmetry at the center of honeycomb structure gives rise to a extra DM-interaction which we named as anti-chiral DM-interaction.We studied the system by using Schwinger Boson mean field theory and Holstein-Primakoff transformation and show that when the antichiral DM-interaction dominates over the chiral DM-interaction, the direction of velocity of the edge states become in the same direction (antichiral edge states).Due to conservation of total number of spins in the system a bulk current flows in the opposite direction relative to the antichiral edge current.In this study we suggested the way to break the inversion symmetries in the materials CrSrTe 3 , CrGrTe 3 , AFe 2 (PO 4 ) 2 (A=Ba, Cs, K, La) to achieve antichiral DM-interaction.The presence of antichiral edge states can be detected by using inelastic neutron scattering by detecting the band tilting at K and K points of magnon bands.Moreover we showed that spin noise spectroscopy at the edges is useful measurements to detect the presence of antichiral edge modes.Magnetic force microscopy is also a promising tool to detect the antichiral magnons at edges.The underlying spin-Hamiltonian of the antiferromagnetic systems in the materials like rare-earth tetraborides(RB 4 , R=Er,Tm) and U 2 Pd 2 In can be described by using extended Shastry-Sutherland models.In previous theoretical studies it is shown that there is a non-collinear spin-state known as flux state exists in the Shastry-Sutherland model in presence of out of plane DM-interaction.Although the presence of perpendicular component of DM-interactions in the rare-earth materials are not known, it can be induced artificially by using circularly polarized light or using heavy-metal alloys.In the fourth chapter, we studied the magnetic excitations in the flux state on Shastry-Sutherland lattice in-First of all, I would like to thank my research supervisor Prof. Pinaki Sengupta for his continuous support and guidance throughout my Ph.D. study on and off the field.whenever I went to his office with a problem he always welcomed me and assisted me.He has encouraged and inspired me to become an independent researcher and developed my critical thinking.I am really grateful to him as a person who introduced me the field of research.Moreover my scientific writing and presentation skills also improved due to his suggestions.I am really very thankful for being so flexible and allowing me to choose the work and project which interests me most.
Exotic phases and associated phase transitions in low
dimensions have been a fascinating frontier and a driving force in
modern condensed matter physics since the 80s. Due to strong
correlation effect, they are beyond the description of mean-field
theory based on a single-particle picture and Landau's
symmetry-breaking theory of phase transitions. These new phases of
matter require new physical quantities to characterize them and new
languages to describe them. This thesis is devoted to the study on
exotic phases of correlated electrons in two spatial dimensions. We
present the following efforts in understanding two-dimensional
exotic phases: (1) Using Zn vertex algebra, we give a complete
classification and characterization of different one-component
fractional quantum Hall (FQH) states, including their ground state
properties and quasiparticles. (2) In terms of a non-unitary
transformation, we obtain the exact form of statistical
interactions between composite fermions in the lowest Landau level
(LLL) with v=1/(2m), m=1,2... By studying the pairing instability
of composite fermions we theoretically explains recently observed
FQHE in LLL with v=1/2,1/4. (3) We classify different Z2 spin
liquids (SLs) on kagome lattice in Schwinger-fermion representation
using projective symmetry group (PSG). We propose one most
promising candidate for the numerically discovered SL state in
nearest-neighbor Heisenberg model on kagome lattice}. (4) By
analyzing different Z2 spin liquids on honeycomb lattice within PSG
classification, we find out the nature of the gapped SL phase in
honeycomb lattice Hubbard model, labeled sublattice pairing state
(SPS) in Schwinger-fermion representation. We also identify the
neighboring magnetic phase of SPS as a chiral-antiferromagnetic
(CAF) phase and analyze the continuous phase transition between SPS
and CAF phase. For the first time we identify a SL called 0-flux
state in Schwinger-boson representation with one (SPS) in
Schwinger-fermion representation by a duality transformation. (5)
We show that when certain non-collinear magnetic order coexists in
a singlet nodal superconductor, there will be Majorana bound states
in vortex cores/on the edges of the superconductor. This proposal
opens a window for discovering Majorana fermions in strongly
correlated electrons. (6) Motivated by recent numerical discovery
of fractionalized phases in topological flat bands, we construct
wavefunctions for spin-polarized fractional Chern insulators (FCI)
and time reversal symmetric fractional topological insulators (FTI)
by parton approach. We show that lattice symmetries give rise to
different FCI/FTI states even with the same filling fraction. For
the first time we construct FTI wavefunctions in the absence of
spin conservation which preserve all lattice symmetries. The
constructed wavefunctions also set up the framework for future
variational Monte Carlo simulations.
The strong interest in strongly correlated systems in condensed matter physics has continued unabated for the past few decades. In recent years, the number of novel, exotic quantum phases found in theoretical studies has seen a phenomenal rise. Among those interesting quantum states are bose liquids and spin liquids, where strong quantum fluctuations have prevented the systems from developing a long range order. Our work in this thesis seeks to further the understanding of frustrated systems. In the study of a hard-core boson model with ring-only exchange interactions on a square lattice, we obtain concrete numerical realization of the unconventional Exciton Bose Liquid (EBL) phase, which possesses interesting properties such as a "Bose surface" which resembles the Fermi surface in a metal, as well as unusual thermodynamic properties such as a T Log T dependence for specific heat. An equally important result from this work is the demonstration that the widely used Gutzwiller projection on slave-particle wave functions may generally fail to capture the correct long wavelength physics in the respective systems. For the Heisenberg antiferromagnet on the kagome lattice, which is a promising candidate for realizing a spin-disordered ground state, our variational study shows that the projected Schwinger boson wave function is energetically better than the Dirac spin liquid wave function when a small antiferromagnetic second-neighbor spin coupling is added to the nearest-neighbor model. We also study the anisotropic triangular Heisenberg antiferromagnetic in magnetic field, and find simple, yet accurate wave functions for various regions of the surprisingly rich phase diagram, thus providing insights into the energetics of the competing phases in this interesting model. Finally, our work also highlights permanent-type wave functions as potentially useful constructions in variational studies of systems with short-ranged correlations, e.g., a Mott insulator and a gapped spin liquid.