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arXiv:1701.04709 · Physical Review Letters

Ultrastrong Coupling Few-Photon Scattering Theory

Tao Shi, Yue Chang, Juan José García‐Ripoll

Published Apr 12, 2018• 59 citations
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Abstract

We study the scattering of individual photons by a two-level system ultrastrongly coupled to a waveguide. The scattering is elastic for a broad range of couplings and can be described with an effective U(1)-symmetric Hamiltonian. This simple model allows the prediction of scattering resonance line shapes, validated up to α=0.3, and close to the Toulouse point α=1/2, where inelastic scattering becomes relevant. Our predictions model experiments with superconducting circuits [P. Forn-Díaz et al., Nat. Phys. 13, 39 (2017)NPAHAX1745-247310.1038/nphys3905] and can be extended to study multiphoton scattering.

DOI
10.1103/physrevlett.120.153602

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We study the scattering of individual photons by a two-level system ultrastrongly coupled to a waveguide. The scattering is elastic for a broad range of couplings and can be described with an effective U(1)-symmetric Hamiltonian. This simple model allows the prediction of scattering resonance line shapes, validated up to α=0.3, and close to the Toulouse point α=1/2, where inelastic scattering becomes relevant. Our predictions model experiments with superconducting circuits [P. Forn-Díaz et al., Nat. Phys. 13, 39 (2017)NPAHAX1745-247310.1038/nphys3905] and can be extended to study multiphoton scattering.
The scattering of a flying photon by a two-level system ultrastrongly coupled to a one-dimensional photonic waveguide is studied numerically. The photonic medium is modeled as an array of coupled cavities and the whole system is analyzed beyond the rotating wave approximation using matrix product states. It is found that the scattering is strongly influenced by the single- and multiphoton dressed bound states present in the system. In the ultrastrong coupling regime a new channel for inelastic scattering appears, where an incident photon deposits energy into the qubit, exciting a photon-bound state, and escaping with a lower frequency. This single-photon nonlinear frequency conversion process can reach up to 50% efficiency. Other remarkable features in the scattering induced by counterrotating terms are a blueshift of the reflection resonance and a Fano resonance due to long-lived excited states.
In this work we study the scattering of pairs of photons by a two-level system ultrastrongly coupled to a one-dimensional waveguide. We describe this problem using a spin-boson model with an Ohmic environment J(ω)=παω1.J(ω)=παω^1.J(ω)=παω1. We show that when coupling strength lays is about α≤1,α\leq 1,α≤1, the dynamics is well approximated by a polaron Hamiltonian, under the approximation of a conserved number of excitations. In this regime, we develop analytical predictions for the single- and two-photon scattering matrix computed with a Green's function method.
Understanding large-scale interacting quantum matter requires dealing with the huge number of quanta that are produced by scattering even a few particles against a complex quantum object. Prominent examples are found from high-energy cosmic ray showers, to the optical or electrical driving of degenerate Fermi gases. We tackle this challenge in the context of many-body quantum optics, as motivated by the recent developments of circuit quantum electrodynamics at ultrastrong coupling. The issue of particle production is addressed quantitatively with a simple yet powerful concept rooted in the quantum superposition principle of multimode coherent states. This key idea is illustrated by the study of multiphoton emission from a single two-level artificial atom coupled to a high impedance waveguide, driven by a nearly monochromatic coherent tone. We find surprisingly that the off-resonant inelastic emission line shape is dominated by broadband particle production, due to the large phase space associated with contributions that do not conserve the number of excitations. Such frequency conversion processes produce striking signatures in time correlation measurements, which can be tested experimentally in quantum waveguides. These ideas open new directions for the simulation of a variety of physical systems, from polaron dynamics in solids to complex superconducting quantum architectures.
In recent studies on ultrastrong coupling between matter and light in cavities, the significance of gauge choice when employing the widely used two-level approximation has been highlighted. Expanding upon these investigations, we extend the analysis to waveguide QED, where we demonstrate that truncations performed in the dipole gauge also yield accurate results. To illustrate this point, we consider the case of a dipole coupled to a cavity array. Various numerical and analytical techniques have been employed to investigate the low-energy dynamics of the system. Leveraging these theoretical tools, we argue that single-photon scattering is an ideal method for investigating gauge-related issues. Our findings reveal two effects in the scattering spectra, which cannot be reproduced in a truncated model using the Coulomb gauge. First, the primary resonance is modified due to a Lamb shift contribution. Second, we observe asymmetric transmission amplitudes surrounding this resonance, reflecting the asymmetry of the spectral density in this model. Additionally, we explore other features in the scattering spectra resulting from ultrastrong couplings, such as the emergence of Fano resonances and inelastic channels. Finally, we propose an experimental test of our ideas in the context of circuit QED.
Waveguide quantum electrodynamics (waveguide QED) describes the interaction between an electromagnetic field confined to a one-dimensional waveguide with atom-like quantum emitters close by. The characteristics of these kinds of systems are the possibility for strong and even ultrastrong interactions between the photonic and atom-like systems, and practically infinite range interactions between the emitters. These properties are valuable for a wide range of quantum optical applications, like quantum communication, quantum networks and quantum metrology. In this thesis we focus on two challenges in quantum optics, namely the generation and scattering of multiphoton states. In the first part of this thesis we demonstrate how waveguide QED systems can be exploited for the generation of multiphoton states, in particular of single-mode Fock states and superpositions thereof as well as multi-mode photonic states with metrological applications. The basic setup for this goal is an ensemble of quantum emitters coupled to a waveguide. In the so-called atomic mirror configuration symmetric Dicke states (or a superposition thereof) decay superradiantly to the ground state and emit the desired multiphoton state, which can be efficiently collected at the ends of the waveguide. We propose various protocols for the preparation of these Dicke states in waveguide QED systems and characterize the emitted photonic state. It turns out that in the low excitation regime, that is, if the number of photons is much lower than the ensemble size, the photonic state is emitted into a single mode. This single-mode structure is fundamental to current proposals for applications in quantum metrology with optical interferometers. Outside the low excitation regime, a multi-mode photonic state is generated, for which the metrological capabilities were unknown. We were able to show that these states still lead to quantum-enhanced optical interferometry. In the second part of this thesis we demonstrate how the scattering of multiphoton states on a single quantum emitter coupled to the waveguide can be used for testing the limits of the light-matter interaction strength. In particular, we investigate systems in the so-called ultrastrong coupling regime, where the coupling strength between the photonic and atom-like system is of the order of the emitter's transition energy. In this regime, many methods and approximations used in quantum optics, especially the Rotating Wave Approximation, break down and one needs to develop new analytical and numerical methods to study these systems. One approach is the so-called polaron Transformation. We show how this transformation can be applied for predicting the scattering amplitude of few photons scattering on the emitter. The comparison of these results with numerical simulations using matrix product states shows a good agreement for moderate coupling strengths. Both parts together show that waveguide QED systems are promising candidates for the generation of multiphoton states as well as for the investigation of fundamental limits probed through the scattering of multiphoton states. The latter also finds application in the implementation of photon-photon nonlinearities induced by the interaction with the quantum emitters. Apart from these and many other theoretical predictions, waveguide QED systems are also undergoing rapid progress in experiments. Therefore, we expect these kinds of systems to bring forth several advances in the field of quantum optics.
Engineering strong photon–photon interactions at the quantum level have been crucial in various areas of research, notably in quantum information processing and quantum simulation. It is often done by coupling matter strongly to light. A promising way to achieve this is via waveguide quantum electrodynamics (QED). Motivated by these advancements, we study few-photon transport in waveguide QED setups. First, we present a diagrammatic technique to systematically study multiphoton scattering based on the scattering formalism and Green’s function approach. We demonstrate our proposal through physically relevant examples involving scattering of few-photon states from two-level emitters as well as from arrays of correlated Kerr nonlinear resonators described by the Bose–Hubbard model. In the second part, we apply the diagrammatic technique that was developed to perform a comprehensive study on a Bose–Hubbard lattice with a quasi-periodic potential. This model exhibits many-body localisation. We compute the two-photon transmission probability and show that it carries signatures of the underlying localisation transition with close agreement to the participation ratio of the eigenstates. The systematic scattering approach provided in this paper provides a foundation for future works at the interface between quantum optics and condensed matter.