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arXiv:1612.05411

Macroscopic magnetic field generated in laser atom interaction

Swarupananda Pradhan

Published Dec 16, 2016• 2 citations
arXivHTMLPDF

Abstract

We observe shift in the zero magnetic field resonance as the handedness of resonantly interacting circularly polarized light is changed. The characteristic of the shift resembles with the Zeeman light shift that arises due to interaction of non-resonant circularly polarized light with atom. However many attributes of our observed resonant phenomena like dependence on buffer gas, saturation of the shift with light intensity and involved time constant in evolution of the shift contradicts to the fictitious magnetic field model. We propose collective alignment of atomic magnetic moment giving rise to a real magnetic field as a possible mechanism behind the observed shift. The characteristic changes in the signal profile with respect to the three axis magnetic field have been established that can reveal many subtle issues pertaining to the phenomenon.

DOI
10.48550/arxiv.1612.05411

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We observe shift in the zero magnetic field resonance as the handedness of resonantly interacting circularly polarized light is changed. The characteristic of the shift resembles with the Zeeman light shift that arises due to interaction of non-resonant circularly polarized light with atom. However many attributes of our observed resonant phenomena like dependence on buffer gas, saturation of the shift with light intensity and involved time constant in evolution of the shift contradicts to the fictitious magnetic field model. We propose collective alignment of atomic magnetic moment giving rise to a real magnetic field as a possible mechanism behind the observed shift. The characteristic changes in the signal profile with respect to the three axis magnetic field have been established that can reveal many subtle issues pertaining to the phenomenon.
We report a different type of optical Stern-Gerlach effect, where a magnetic-field gradient is replaced with a light-intensity gradient and a paramagnetic atom is deflected according to its magnetic quantum number. The laser light is detuned between the D1D1D1 and D2D2D2 frequencies, with the size of the detuning from the D2D2D2 resonance being twice that from the D1D1D1 resonance, and it is circularly polarized to produce an ac Stark shift that takes the form of a pure Zeeman shift. Slow rubidium atoms are extracted from a magneto-optical trap and then spin polarized. The atoms traversing the laser-intensity gradient on one side of the Gaussian beam profile show deflections that depend on the atomic spin state and the laser polarization. When the laser-beam axis is aligned with the slit that defines the atomic beam, we observe focusing and defocusing of the atomic beam.
We demonstrate that when laser light is circularly polarized and properly detuned, the ac Stark shift of an alkali-metal atom in its ground state takes the form of a pure Zeeman shift. The condition is satisfied when the laser frequency is between the D1D1D1 and D2D2D2 transition frequencies, with the size of the detuning from the D2D2D2 resonance twice that from the D1D1D1 resonance. The direction of the effective magnetic field is along the laser propagation axis, and its magnitude is proportional to the vector polarizability of the atom and to the laser intensity. We use stimulated Raman spectroscopy on an optically pumped slow atomic beam from a magneto-optical trap to measure the vector polarizability and saturated absorption spectroscopy to show that the scalar polarizability vanishes at the particular detuning.
Results of a fairly straightforward experiment on resonant magneto-optical rotation by rubidium-87 atoms revealed strong time-dependence of the polarization plane of light emerging from atomic vapors following a sudden irradiation with a laser beam. The rotation of the plane appears as a not direct consequence of the influence of the magnetic field on atoms. Reported measurements conducted using a vapor cell without any buffer gas or an anti-relaxation wall coating show that transmitted light has initially the same (linear) polarization as the incident one. Rotation of the polarization plane caused by an axial magnetic field develops in time scales similar to the pace of establishing the optical pumping/relaxation equilibrium in the atomic ensemble. The traditional passive Faraday rotation picture providing working description for the resonant magneto-optical effects in steady-state conditions does not explain the observed sequence of evolution of the polarization. The picture has to be augmented with analysis of time dependence in the spatial distribution of relevant quantum states within the atomic ensemble as well as longitudinal and transversal intensity profiles of the light beam. Isolation of external effects caused by the optical pumping and relaxation processes from consequences of internal atomic coherences should uncover more details of mechanisms of the latter in the presence of magnetic field. Plentitude of data available from time-dependent polarization measurements provides strong incentives for further development and tests of comprehensive models of coherent interactions of atomic ensembles with radiation and possibly a base for additional advance in understanding and applications of these phenomena.
A theoretical analysis is made of the resonant interaction between a traveling monochromatic light wave of arbitrary intensity and polarization and the 1/21/2 and 10 transitions in gas atoms in a magnetic field. An analysis is made of the influence of atomic collisions and coherence of the Zeeman sublevels of the terms on the structure of nonlinear magnetooptic resonances in the amplitude and polarization characteristics of the wave. Some features of nonlinear magnetooptic resonances for laser excitation of atoms from the ground state are noted. A study is made of the Faraday rotation and self-rotation of the polarization ellipse of the radiation as a function of the detuning of the wave frequency, the saturation parameter, and the optical density of the gas. The stability of the polarization of light in the medium is discussed. It is noted that these laws may be used to analyze and control the radiation characteristics of lasers and amplifiers when the level of saturation of a resonant gaseous medium in a magnetic field is high.
The energy shift of an atom due to its interaction with the oscillating electric field of an electromagnetic wave, or a laser light, is called the ac Stark shift. It has been studied both in the field of precision spectroscopy and atom optics. When the laser intensity is not constant spatially, its gradient gives rise to a dipole force. The force was used either to trap atoms in an optical trap or to reflect or guide atoms. We studied the ac Stark effect taking into account the fine structure of an alkali atom. We found that when the laser light is circularly polarized and properly detuned between the D1 and D2 transitions, the ac Stark shift can take the form of a pure Zeeman shift, hence the name analogous Zeeman shift.
According to the quantum theory of the optical-pumping cycle, one can describe the effect of a nonresonant light beam on the different Zeeman sublevels of an atomic ground state by an effective Hamiltonian He{\mathcal{H}}_{e}He​ which depends on the polarization and spectral profile of the incident light. In order to check the structure of He{\mathcal{H}}_{e}He​, we have performed a detailed experimental study of the ground-state energy sublevels of various kinds of atoms perturbed by different types of nonresonant light beams. Attention is paid to the modification of the Zeeman structure due to He{\mathcal{H}}_{e}He​. We have been able to obtain experimentally in the ground state of 199Hg^{199}\mathrm{Hg}199Hg, 201Hg^{201}\mathrm{Hg}201Hg, and 87Rb^{87}\mathrm{Rb}87Rb, Zeeman light shifts that are larger than the width of the levels due to the thermal relaxation. The removal of the Zeeman degeneracy in zero external field, due to a nonresonant light irradiation, is observed by different optical-pumping techniques; the full Zeeman diagram of the perturbed atoms is also determined when a static field ${\stackrel{\ensuremath{\rightarrow}}{\mathrm{H}}}_{0}$ is added. We have checked that the effect of He{\mathcal{H}}_{e}He​ can be described in terms of fictitious static electric or magnetic fields. These fictitious fields can be used to act selectively on a given atomic level.