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arXiv:1607.05727 · Physical review. B./Physical review. B

Fractionalized Fermi liquid with bosonic chargons as a candidate for the pseudogap metal

Shubhayu Chatterjee, Subir Sachdev A

Published Nov 10, 2016• 37 citations
arXivHTMLPDF

Abstract

Doping a Mott-insulating ${\mathbb{Z}}_{2}$ spin liquid can lead to a fractionalized Fermi liquid (FL*). Such a phase has several favorable features that make it a candidate for the pseudogap metal for the underdoped cuprates. We focus on a particular, simple ${\mathbb{Z}}_{2}$-FL* state which can undergo a confinement transition to a spatially uniform superconductor which is smoothly connected to the ``plain vanilla'' BCS superconductor with $d$-wave pairing. Such a transition occurs by the condensation of bosonic particles carrying $+e$ charge but no spin (``chargons''). We show that modifying the dispersion of the bosonic chargons can lead to confinement transitions with charge density waves and pair density waves at the same wave vector $\mathbf{K}$, coexisting with $d$-wave superconductivity. We also compute the evolution of the Hall number in the normal state during the transition from the plain vanilla FL* state to a Fermi liquid, and argue, following Coleman, Marston, and Schofield [Phys. Rev. B 72, 245111 (2005)], that it exhibits a discontinuous jump near optimal doping. We note the distinction between these results and those obtained from models of the pseudogap with fermionic chargons.

DOI
10.1103/physrevb.94.205117

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Doping a Mott-insulating Z2{\mathbb{Z}}_{2}Z2​ spin liquid can lead to a fractionalized Fermi liquid (FL*). Such a phase has several favorable features that make it a candidate for the pseudogap metal for the underdoped cuprates. We focus on a particular, simple Z2{\mathbb{Z}}_{2}Z2​-FL* state which can undergo a confinement transition to a spatially uniform superconductor which is smoothly connected to the plain vanilla'' BCS superconductor with $d$-wave pairing. Such a transition occurs by the condensation of bosonic particles carrying $+e$ charge but no spin (chargons''). We show that modifying the dispersion of the bosonic chargons can lead to confinement transitions with charge density waves and pair density waves at the same wave vector K\mathbf{K}K, coexisting with ddd-wave superconductivity. We also compute the evolution of the Hall number in the normal state during the transition from the plain vanilla FL* state to a Fermi liquid, and argue, following Coleman, Marston, and Schofield [Phys. Rev. B 72, 245111 (2005)], that it exhibits a discontinuous jump near optimal doping. We note the distinction between these results and those obtained from models of the pseudogap with fermionic chargons.
A Z2{\mathbb{Z}}_{2}Z2​ fractionalized Fermi liquid (FL*) is a novel state of strongly correlated quantum matter. Although it is metallic, it violates Luttinger's theorem on the volume enclosed by the Fermi surface obeyed by conventional metals; this is possible due to the presence of emergent gauge excitations. The authors study here the superconducting states that can arise out of instabilities of such a topological metal. In particular, they focus on a FL* topological metal that has favorable energetics on the square lattice with nematic order, relevant to the cuprate superconductors. They find that a Higgs transition out of this FL* results in confinement of the anyonic degrees of freedom, and the resulting state is a superconductor with broken translation symmetry or time-reversal invariance. In the process, they also establish a complete mapping between bosonic and fermionic descriptions of time-reversal invariant gapped insulating Z2{\mathbb{Z}}_{2}Z2​ spin liquid states on the rectangular lattice, which, on doping with charge carriers, can give rise to FL* phases. They also note a possible connection to the recent observation of pair density waves in the superconducting state of the underdoped cuprates.
Insulating quantum spin liquids can undergo a confinement transition to a valence bond solid via the condensation of topological excitations of the associated gauge theory. We extend the theory of such transitions to fractionalized Fermi liquids (FL*): These are metallic doped spin liquids in which the Fermi surfaces only have gauge neutral quasiparticles. Using insights from a duality transform on a doped quantum dimer model for the U(1)-FL* state, we show that projective symmetry group of the theory of the topological excitations remains unmodified, but the Fermi surfaces can lead to additional frustrating interactions. We propose a theory for the confinement transition of Z2{\mathbb{Z}}_{2}Z2​-FL* states via the condensation of visons. A variety of confining, incommensurate density wave states are possible, including some that are similar to the incommensurate ddd-form factor density wave order observed in several recent experiments on the cuprate superconductors.
Two of the iconic phases of the hole-doped cuprate materials are the intermediate temperature pseudogap metal and the lower temperature ddd-wave superconductor. Following the suggestion of P. W. Anderson, there were early theories of these phases as doped quantum spin liquids. However, these theories have had difficulties with two prominent observations: (i) angle-dependent magnetoresistance measurements (ADMR) in the pseudogap metal, including observation of the Yamaji effect, present convincing evidence of small hole pockets which can tunnel coherently between square lattice layers (Fang et al., Nature Physics 18, 558 (2022); Chan et al., Nature Physics 21, 1753 (2025)) and (ii) the velocities of the nodal Bogoliubov quasiparticles in the ddd-wave superconductor are highly anisotropic, with vF≫vΔv_F \gg v_ΔvF​≫vΔ​ (Chiao et al., Phys. Rev. B 62, 3554 (2000)). These notes review how the fractionalized Fermi Liquid (FL*) state, which dopes quantum spin liquids with gauge-neutral electron-like quasiparticles, resolves both difficulties. Theories of insulating quantum spin liquids employing fractionalization of the electron spin into bosonic or fermionic partons are discussed. Doping the bosonic parton theory leads to a holon metal theory: while not appropriate for the cuprate pseudogap, this theory is argued to apply to ultracold atom experiments on the Lieb lattice. Doping the fermionic parton theory leads to a ddd-wave superconductor with nearly isotropic quasiparticle velocities. The construction of the FL* state in a single band Hubbard-type model is described using a quantum dimer model, followed by a more realistic description using the Ancilla Layer Model (ALM), which is then used to obtain the theory of the pseudogap and the ddd-wave superconductor. The ALM also leads to a wavefunction for the FL* state of the Hubbard model, which agrees with ultracold atom observations.
Abstract We review a theoretical framework for the cuprate superconductors, rooted in a fractionalized Fermi liquid (FL*) description of the intermediate-temperature pseudogap phase at low doping. The FL* theory predicted hole pockets each of fractional area p / 8 at hole doping p , in contrast to the area p / 4 in spin density wave theory. Magnetotransport measurements, including observation of the Yamaji angle, show clear evidence of hole pocket quasiparticles which can tunnel coherently between square lattice layers, and are consistent with the FL* description. The FL* phase of a single-band model is described using a layer construction with a pair of ancilla qubits on each site: the Ancilla layer model (ALM). Its mean field theory yields hole pockets of area p / 8 , and matches the gapped photoemission spectrum in the anti-nodal region of the Brillouin zone. Fluctuations are described by the SU(2) gauge theory of a background spin liquid with critical Dirac spinons. A Monte Carlo study of the thermal SU(2) gauge theory transforms the hole pockets into Fermi arcs in photoemission. One route to confinement of FL* upon lowering temperature yields a d -wave superconductor via a Kosterlitz–Thouless transition of h / ( 2 e ) vortices, with nodal Bogoliubov quasiparticles featuring anisotropic velocities and vortices surrounded by charge order halos. An alternative route yields a charge-ordered metallic state that has quantum oscillations consistent with observations. These confinement transitions are driven by the condensation of a SU(2) fundamental Higgs field, which also provides a fractionalized description of intertwined orders. Increasing doping from the FL* phase in the ALM drives a transition to a conventional FL at large doping, passing through an intermediate strange metal regime. We formulate a theory of the FL*-FL metal-metal transition without a symmetry-breaking order parameter, using a critical quantum ‘charge’ liquid of mobile electrons in the presence of disorder, developed via an extension of the Sachdev–Ye–Kitaev model to two spatial dimensions. At low temperatures, and across optimal and over doping, we address the regimes of extended non-FL behavior by Griffiths effects near quantum phase transitions in disordered metals. Partly based on lectures by S S at Boulder School 2025, Dynamics of Strongly Correlated Electrons , 14–18 July. Lecture videos . Joint ICTP-WE Heraeus School and Workshop on Advances in Quantum Matter: Pushing the Boundaries , ICTP, Trieste, 4, 6 August 2025. Lecture videos . School on Quantum Dynamics of Matter, Light and Information , ICTP, Trieste, 18, 19 August 2025. Lecture videos . Croucher Advanced Study Institute for Fractional Chern Insulators , University of Hong Kong, 4, 5 September 2025. Lecture slides . Advanced School and Conference on Quantum Matter , ICTP Trieste, 1–12 December 2025. Lecture Notes . Lecture videos .
Fractionalized Fermi liquids (FL ⁣∗\mathrm{FL}^{\!*}FL∗), elusive metallic states characterized by fractionalized quasiparticles alongside conventional ones and defying Luttinger's theorem, are prime candidates for the pseudogap regime of underdoped cuprates. We show that a FL ⁣∗\mathrm{FL}^{\!*}FL∗ phase emerges in the single-band ttt-JJJ model through a simple ghost-Gutzwiller Ansatz, optimized at the cost of a mean-field calculation. The resulting temperature-doping phase diagram encompasses a low-doping FL ⁣∗\mathrm{FL}^{\!*}FL∗, a ddd-wave superconducting dome, and an overdoped conventional Fermi liquid, thereby reproducing key qualitative features of cuprate phenomenology.
Recent experiments in the underdoped regime of the hole-doped cuprates have found evidence for an incommensurate charge density-wave state. We present an analysis of the charge ordering instabilities in a metal with antiferromagnetic correlations, where the electronic excitations are coupled to the fractionalized excitations of a quantum fluctuating antiferromagnet on the square lattice. The resulting charge density-wave state emerging out of such a fractionalized Fermi liquid (FL*) has wave vectors of the form $(\ifmmode\pm\else\textpm\fi{}{Q}_{0},0),(0,\ifmmode\pm\else\textpm\fi{}{Q}_{0})$, with a predominantly ddd-form factor, in agreement with experiments on a number of different families of the cuprates. In contrast, as previously shown, the charge density-wave instability of a nearly antiferromagnetic metal with a large Fermi surface, interacting via short-range interactions, has wave vectors of the type $(\ifmmode\pm\else\textpm\fi{}{Q}_{0},\ifmmode\pm\else\textpm\fi{}{Q}_{0})$. Our results show that the observed charge density-wave appears as a low-energy instability of a fractionalized metallic state linked to the proximity to an antiferromagnetic insulator, and the pseudogap regime can be described by such a metal at least over intermediate length and energy scales.