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arXiv:1603.03041 · Physical review. B./Physical review. B

Superconductivity from a confinement transition out of a fractionalized Fermi liquid with Z 2 topological and Ising-nematic orders

Shubhayu Chatterjee, Yang Qi, Subir Sachdev A, Julia Steinberg

Published Jul 5, 2016• 18 citations
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Abstract

A ${\mathbb{Z}}_{2}$ fractionalized Fermi liquid (FL*) is a novel state of strongly correlated quantum matter. Although it is metallic, it violates Luttinger's theorem on the volume enclosed by the Fermi surface obeyed by conventional metals; this is possible due to the presence of emergent gauge excitations. The authors study here the superconducting states that can arise out of instabilities of such a topological metal. In particular, they focus on a FL* topological metal that has favorable energetics on the square lattice with nematic order, relevant to the cuprate superconductors. They find that a Higgs transition out of this FL* results in confinement of the anyonic degrees of freedom, and the resulting state is a superconductor with broken translation symmetry or time-reversal invariance. In the process, they also establish a complete mapping between bosonic and fermionic descriptions of time-reversal invariant gapped insulating ${\mathbb{Z}}_{2}$ spin liquid states on the rectangular lattice, which, on doping with charge carriers, can give rise to FL* phases. They also note a possible connection to the recent observation of pair density waves in the superconducting state of the underdoped cuprates.

DOI
10.1103/physrevb.94.024502

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The Schwinger-boson theory of the frustrated square lattice antiferromagnet yields a stable, gapped $\mathbb{Z}_2$ spin liquid ground state with time-reversal symmetry, incommensurate spin correlations and long-range Ising-nematic order. We obtain an equivalent description of this state using fermionic spinons (the fermionic spinons can be considered to be bound states of the bosonic spinons and the visons). Upon doping, the $\mathbb{Z}_2$ spin liquid can lead to a FL* metal with small Fermi pockets of electron-like quasiparticles, while preserving the $\mathbb{Z}_2$ topological and Ising-nematic orders. We describe a Higgs transition out of this deconfined metallic state into a confining superconducting state which is usually of the Fulde-Ferrell-Larkin-Ovchinnikov type, with spatial modulation of the superconducting order.

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Fractionalized Fermi liquid with bosonic chargons as a candidate for the pseudogap metal

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Doping a Mott-insulating ${\mathbb{Z}}_{2}$ spin liquid can lead to a fractionalized Fermi liquid (FL*). Such a phase has several favorable features that make it a candidate for the pseudogap metal for the underdoped cuprates. We focus on a particular, simple ${\mathbb{Z}}_{2}$-FL* state which can undergo a confinement transition to a spatially uniform superconductor which is smoothly connected to the ``plain vanilla'' BCS superconductor with $d$-wave pairing. Such a transition occurs by the condensation of bosonic particles carrying $+e$ charge but no spin (``chargons''). We show that modifying the dispersion of the bosonic chargons can lead to confinement transitions with charge density waves and pair density waves at the same wave vector $\mathbf{K}$, coexisting with $d$-wave superconductivity. We also compute the evolution of the Hall number in the normal state during the transition from the plain vanilla FL* state to a Fermi liquid, and argue, following Coleman, Marston, and Schofield [Phys. Rev. B 72, 245111 (2005)], that it exhibits a discontinuous jump near optimal doping. We note the distinction between these results and those obtained from models of the pseudogap with fermionic chargons.

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Transport and Symmetry Breaking in Strongly Correlated Systems With Topological Order

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This thesis is devoted to the study of strongly correlated phases of quantum matter in two spatial dimensions. In presence of strong interactions, the electron can split up into separate spin and charge degrees of freedom. The diagnosis of such fractionalized excitations in recent experiments, as well as finding new probes for their detection, comprise the two major themes of this thesis.\nThe first part of the thesis, comprising chapters 2-6, discusses the relevance of fractionalization to the pseudogap phase of the underdoped high Tc cuprate superconductors. This is motivated by transport experiments that show a violation of Luttinger's theorem, possible only in the presence of topological order that can arise naturally as a consequence of fractionalization. Chapters 2 and 3 focus on phenomenological models with bosonic charge carriers and fermionic spin carriers, and investigate transport properties as well as various confinement transitions to symmetry broken phases. Chapters 4, 5 and 6 deal with a different framework of electron fractionalization, where the charge carriers are fermionic and spin carriers are bosonic. We find that these models can better explain the thermal and electrical transport properties in chapter 5. In chapters 6 and 7, we show how such models arise naturally from quantum fluctuations of antiferromagnetism, and can simultaneously intertwine the anti-nodal spectral gap with the discrete broken symmetries that are observed in the cuprates. \nThe second part of the thesis, comprising chapters 7 and 8, proposes new experimental probes to study the behavior of insulating two dimensional quantum magnets. Aided by geometric frustration and strong quantum fluctuations, they may realize a spin liquid ground state which can be extremely difficult to detect via conventional probes. Chapter 7 discusses how novel spin-transport probes from the spintronics community can be used to detect fractionalized excitations in a quantum spin liquid. Chapter 8 studies how the temperature dependent anisotropy of in-plane versus out-of-plane thermal conductivities can serve as an explicit signature of fractionalization in layered two-dimensional materials.

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A Z2{\mathbb{Z}}_{2}Z2​ fractionalized Fermi liquid (FL*) is a novel state of strongly correlated quantum matter. Although it is metallic, it violates Luttinger's theorem on the volume enclosed by the Fermi surface obeyed by conventional metals; this is possible due to the presence of emergent gauge excitations. The authors study here the superconducting states that can arise out of instabilities of such a topological metal. In particular, they focus on a FL* topological metal that has favorable energetics on the square lattice with nematic order, relevant to the cuprate superconductors. They find that a Higgs transition out of this FL* results in confinement of the anyonic degrees of freedom, and the resulting state is a superconductor with broken translation symmetry or time-reversal invariance. In the process, they also establish a complete mapping between bosonic and fermionic descriptions of time-reversal invariant gapped insulating Z2{\mathbb{Z}}_{2}Z2​ spin liquid states on the rectangular lattice, which, on doping with charge carriers, can give rise to FL* phases. They also note a possible connection to the recent observation of pair density waves in the superconducting state of the underdoped cuprates.
Superconductivity from a confinement transition out of a FL* metal with Z2\mathbb{Z}_2Z2​ topological and Ising-nematic orders
The Schwinger-boson theory of the frustrated square lattice antiferromagnet yields a stable, gapped Z2\mathbb{Z}_2Z2​ spin liquid ground state with time-reversal symmetry, incommensurate spin correlations and long-range Ising-nematic order. We obtain an equivalent description of this state using fermionic spinons (the fermionic spinons can be considered to be bound states of the bosonic spinons and the visons). Upon doping, the Z2\mathbb{Z}_2Z2​ spin liquid can lead to a FL* metal with small Fermi pockets of electron-like quasiparticles, while preserving the Z2\mathbb{Z}_2Z2​ topological and Ising-nematic orders. We describe a Higgs transition out of this deconfined metallic state into a confining superconducting state which is usually of the Fulde-Ferrell-Larkin-Ovchinnikov type, with spatial modulation of the superconducting order.
Doping a Mott-insulating Z2{\mathbb{Z}}_{2}Z2​ spin liquid can lead to a fractionalized Fermi liquid (FL*). Such a phase has several favorable features that make it a candidate for the pseudogap metal for the underdoped cuprates. We focus on a particular, simple Z2{\mathbb{Z}}_{2}Z2​-FL* state which can undergo a confinement transition to a spatially uniform superconductor which is smoothly connected to the ``plain vanilla'' BCS superconductor with ddd-wave pairing. Such a transition occurs by the condensation of bosonic particles carrying +e+e+e charge but no spin (``chargons''). We show that modifying the dispersion of the bosonic chargons can lead to confinement transitions with charge density waves and pair density waves at the same wave vector K\mathbf{K}K, coexisting with ddd-wave superconductivity. We also compute the evolution of the Hall number in the normal state during the transition from the plain vanilla FL* state to a Fermi liquid, and argue, following Coleman, Marston, and Schofield [Phys. Rev. B 72, 245111 (2005)], that it exhibits a discontinuous jump near optimal doping. We note the distinction between these results and those obtained from models of the pseudogap with fermionic chargons.
This article is based on a talk by S.S. at the Nambu Memorial Symposium at the University of Chicago. We review ideas on the nature of the metallic states of the hole-doped cuprate high temperature superconductors, with an emphasis on the connections between the Luttinger theorem for the size of the Fermi surface, topological quantum field theories (TQFTs), and critical theories involving changes in the size of the Fermi surface. We begin with the derivation of the Luttinger theorem for a Fermi liquid, using momentum balance during a process of flux-insertion in a lattice electronic model with toroidal boundary conditions. We then review the TQFT of the Z2 spin liquid, and demonstrate its compatibility with the toroidal momentum balance argument. This discussion leads naturally to a simple construction of `topological' Fermi liquid states: the fractionalized Fermi liquid (FL*) and the algebraic charge liquid (ACL). We present arguments for a description of the pseudogap metal of the cuprates using Z2-FL* or Z2-ACL states with Ising-nematic order. These pseudogap metal states are also described as Higgs phases of a SU(2) gauge theory. The Higgs field represents local antiferromagnetism, but the Higgs-condensed phase does not have long-range antiferromagnetic order: the magnitude of the Higgs field determines the pseudogap, the reconstruction of the Fermi surface, and the Ising-nematic order. Finally, we discuss the route to the large Fermi surface Fermi liquid via the critical point where the Higgs condensate and Ising nematic order vanish, and the application of Higgs criticality to the strange metal.
Insulating quantum spin liquids can undergo a confinement transition to a valence bond solid via the condensation of topological excitations of the associated gauge theory. We extend the theory of such transitions to fractionalized Fermi liquids (FL*): These are metallic doped spin liquids in which the Fermi surfaces only have gauge neutral quasiparticles. Using insights from a duality transform on a doped quantum dimer model for the U(1)-FL* state, we show that projective symmetry group of the theory of the topological excitations remains unmodified, but the Fermi surfaces can lead to additional frustrating interactions. We propose a theory for the confinement transition of Z2{\mathbb{Z}}_{2}Z2​-FL* states via the condensation of visons. A variety of confining, incommensurate density wave states are possible, including some that are similar to the incommensurate ddd-form factor density wave order observed in several recent experiments on the cuprate superconductors.
Abstract We review a theoretical framework for the cuprate superconductors, rooted in a fractionalized Fermi liquid (FL*) description of the intermediate-temperature pseudogap phase at low doping. The FL* theory predicted hole pockets each of fractional area p / 8 at hole doping p , in contrast to the area p / 4 in spin density wave theory. Magnetotransport measurements, including observation of the Yamaji angle, show clear evidence of hole pocket quasiparticles which can tunnel coherently between square lattice layers, and are consistent with the FL* description. The FL* phase of a single-band model is described using a layer construction with a pair of ancilla qubits on each site: the Ancilla layer model (ALM). Its mean field theory yields hole pockets of area p / 8 , and matches the gapped photoemission spectrum in the anti-nodal region of the Brillouin zone. Fluctuations are described by the SU(2) gauge theory of a background spin liquid with critical Dirac spinons. A Monte Carlo study of the thermal SU(2) gauge theory transforms the hole pockets into Fermi arcs in photoemission. One route to confinement of FL* upon lowering temperature yields a d -wave superconductor via a Kosterlitz–Thouless transition of h / ( 2 e ) vortices, with nodal Bogoliubov quasiparticles featuring anisotropic velocities and vortices surrounded by charge order halos. An alternative route yields a charge-ordered metallic state that has quantum oscillations consistent with observations. These confinement transitions are driven by the condensation of a SU(2) fundamental Higgs field, which also provides a fractionalized description of intertwined orders. Increasing doping from the FL* phase in the ALM drives a transition to a conventional FL at large doping, passing through an intermediate strange metal regime. We formulate a theory of the FL*-FL metal-metal transition without a symmetry-breaking order parameter, using a critical quantum ‘charge’ liquid of mobile electrons in the presence of disorder, developed via an extension of the Sachdev–Ye–Kitaev model to two spatial dimensions. At low temperatures, and across optimal and over doping, we address the regimes of extended non-FL behavior by Griffiths effects near quantum phase transitions in disordered metals. Partly based on lectures by S S at Boulder School 2025, Dynamics of Strongly Correlated Electrons , 14–18 July. Lecture videos . Joint ICTP-WE Heraeus School and Workshop on Advances in Quantum Matter: Pushing the Boundaries , ICTP, Trieste, 4, 6 August 2025. Lecture videos . School on Quantum Dynamics of Matter, Light and Information , ICTP, Trieste, 18, 19 August 2025. Lecture videos . Croucher Advanced Study Institute for Fractional Chern Insulators , University of Hong Kong, 4, 5 September 2025. Lecture slides . Advanced School and Conference on Quantum Matter , ICTP Trieste, 1–12 December 2025. Lecture Notes . Lecture videos .
This thesis is devoted to the study of strongly correlated phases of quantum matter in two spatial dimensions. In presence of strong interactions, the electron can split up into separate spin and charge degrees of freedom. The diagnosis of such fractionalized excitations in recent experiments, as well as finding new probes for their detection, comprise the two major themes of this thesis.\nThe first part of the thesis, comprising chapters 2-6, discusses the relevance of fractionalization to the pseudogap phase of the underdoped high Tc cuprate superconductors. This is motivated by transport experiments that show a violation of Luttinger's theorem, possible only in the presence of topological order that can arise naturally as a consequence of fractionalization. Chapters 2 and 3 focus on phenomenological models with bosonic charge carriers and fermionic spin carriers, and investigate transport properties as well as various confinement transitions to symmetry broken phases. Chapters 4, 5 and 6 deal with a different framework of electron fractionalization, where the charge carriers are fermionic and spin carriers are bosonic. We find that these models can better explain the thermal and electrical transport properties in chapter 5. In chapters 6 and 7, we show how such models arise naturally from quantum fluctuations of antiferromagnetism, and can simultaneously intertwine the anti-nodal spectral gap with the discrete broken symmetries that are observed in the cuprates. \nThe second part of the thesis, comprising chapters 7 and 8, proposes new experimental probes to study the behavior of insulating two dimensional quantum magnets. Aided by geometric frustration and strong quantum fluctuations, they may realize a spin liquid ground state which can be extremely difficult to detect via conventional probes. Chapter 7 discusses how novel spin-transport probes from the spintronics community can be used to detect fractionalized excitations in a quantum spin liquid. Chapter 8 studies how the temperature dependent anisotropy of in-plane versus out-of-plane thermal conductivities can serve as an explicit signature of fractionalization in layered two-dimensional materials.