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arXiv:1607.00818 · Physical Review Letters

Large Cross-Phase Modulations at the Few-Photon Level

Ziyu Liu, Yi‐Hsin Chen, Yen-Chun Chen, Hsiang-Yu Lo, Pin-Ju Tsai, Ite A. Yu, Ying-Cheng Chen, Yong‐Fan Chen

Published Nov 7, 2016• 75 citations
arXivHTMLPDF

Abstract

We demonstrate an efficient cross-phase modulation (XPM) based on a closed-loop double-Λ system. The property of the double-Λ medium can be controlled by changing the phases of the applied optical fields. This phase-dependent XPM scheme can achieve large phase modulations at low-light intensities without requiring cavities or tightly focusing laser beams. With this scheme, we observe a π-level phase shift with two pulses, both consisting of eight photons in cold rubidium atoms. Such a novel scheme provides a simple route to generate strong interactions between photons and may have potential applications in all-optical quantum signal processing.

DOI
10.1103/physrevlett.117.203601

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We demonstrate an efficient cross-phase modulation (XPM) based on a closed-loop double-Λ system. The property of the double-Λ medium can be controlled by changing the phases of the applied optical fields. This phase-dependent XPM scheme can achieve large phase modulations at low-light intensities without requiring cavities or tightly focusing laser beams. With this scheme, we observe a π-level phase shift with two pulses, both consisting of eight photons in cold rubidium atoms. Such a novel scheme provides a simple route to generate strong interactions between photons and may have potential applications in all-optical quantum signal processing.
We propose an efficient all-optical phase modulation based on a double-Λ system and demonstrate a π phase shift of a few-photon pulse induced by another few-photon pulse in cold rubidium atoms with this scheme. By changing the phases of the applied laser fields, one can control the property of the double-Λ medium. This phase-dependent mechanism makes the double-Λ system different form the conventional cross-Kerr-based system which only depends on the applied laser intensities. The proposed scheme provides a new route to generate strong nonlinear interactions between photons, and may have potential for applications in quantum information technologies.
We experimentally demonstrate a low-light-level cross-phase-modulation (XPM) scheme based on the light-storage technique in laser-cooled 87Rb atoms. The proposed scheme can achieve a similar phase shift and has the same figure of merit as one using static electromagnetically induced transparency under the constant coupling field. Nevertheless, the phase shift and the energy loss of a probe pulse induced by a signal pulse are neither influenced by the coupling intensity nor by the atomic optical density in the light-storage XPM scheme. This scheme enhances the flexibility of the experiment and makes possible conditional phase shifts on the order of pi with single photons.
We investigate a four-level double-Λ atomic scheme interacting with four laser fields, a weak probe field, a weak signal field and two driven fields, in a closed-loop configuration. We study the Kerr nonlinearity associated with cross-phase modulation based on electromagnetically induced transparency. Our results show, in this closed-loop system, that the strength of cross-phase modulation and two-photon absorption are dependent critically on the relative phase between the excitation paths. By choosing the parameters appropriately, large cross-phase modulation can be achieved within a wide transparency window, while two-photon absorption is cancelled completely. The strength of cross-phase modulation can be enhanced much more by decreasing the intensities of two driven fields.
We investigate a four-level double-Lambda atomic scheme interacting with four laser fields, a weak probe field, a weak signal field and two driven fields, in a closed-loop configuration. We study the Kerr nonlinearity associated with cross-phase modulation based on electromagnetically induced transparency. Our results show, in this closed-loop system, that the strength of cross-phase modulation and two-photon absorption are dependent critically on the relative phase between the excitation paths. By choosing the parameters appropriately, large cross-phase modulation can be achieved within a wide transparency window, while two-photon absorption is cancelled completely. The strength of cross-phase modulation can be enhanced much more by decreasing the intensities of two driven fields.
This thesis explores the theoretical foundations of cross-phase modulation (XPM) between optical fields in the N-configuration atom. This is the process by which the refractive index experienced by one field can be modulated by controlling the intensity of another. The electro-optical version of this effect was first discovered by John Kerr in 1875 and found applications in photonics as a means of very rapidly modulating the phase and intensity of electromagnetic fields. Due to recent advances in experimental techniques there has been growing interest in generating nonlinear optical interactions in coherently prepared atomic ensembles. \n \nThe use of coherently prepared media brings the possibility of achieving a much larger cross-phase modulation than is possible using classical materials. This is particularly useful when trying to create large optical nonlinearities between low-intensity electromagnetic fields. Much of the current research into cross-phase modulation is directed towards realising potential applications in the emerging field of quantum information processing. Above all, the possibility of constructing an all-optical quantum computer has been at the heart of much research and controversy in the field. \n \nIn this thesis the theory of steady-state, transient and pulsed cross-phase modulation is developed. Moreover, care has been taken to relate all research back to experimentally feasible situations. As such, the relevance of the theory is justified by consideration of the situation present in rubidium-87. Due to the close relationship between XPM in the N-configuration atom and electromagnetically induced transparency in the Lambda-atom, many similarities and insights act as link between these two fields. Indeed, it is frequently demonstrated that the key to understanding the various properties of XPM in the N-configuration atom is by comparison with the situation in the corresponding Lambda-atom equivalent.
Large nonlinearity at the single-photon level can pave the way for the implementation of universal quantum gates. However, realizing large and noiseless nonlinearity at such low light levels has been a great challenge for scientists in the past decade. Here, we propose a scheme that enables substantial nonlinear interaction between two light fields that are both stored in an atomic memory. Semiclassical and quantum simulations demonstrate the feasibility of achieving large cross-phase modulation (XPM) down to the single-photon level. The proposed scheme can be used to implement parity gates from which CNOT gates can be constructed. Furthermore, we present a proof of principle experimental demonstration of XPM between two optical pulses: one stored and one freely propagating through the memory medium. Researchers have developed a new technique that shows promise for constructing optical quantum logic gates. Theoretical simulations performed by Mahdi Hosseini and co-workers from the Australian National University and Macquarie University in Australia show that inducing cross-phase modulation between two single-photon light fields stored in a rubidium atomic memory should provide large phase shifts and thus allow the realization of parity gates and CNOT gates, both of which are needed for quantum computing. The researchers estimate that using cold atoms confined in a dipole trap and short-duration single-photon wavepackets should make it possible to realize phase shifts of the order of 10 mrad — orders of magnitude larger than schemes that employ electromagnetically induced transparency.