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arXiv:1606.07697 · Physical review. B./Physical review. B

Non-Fermi-liquid behavior in quantum impurity models with superconducting channels

Rok Žitko, Michele Fabrizio

Published Feb 16, 2017• 13 citations
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Abstract

We study how the non-Fermi-liquid nature of the overscreened multichannel Kondo impurity model affects the response to a BCS pairing term that, in the absence of the impurity, opens a gap $\mathrm{\ensuremath{\Delta}}$. We find that the low-energy spectrum in the limit $\mathrm{\ensuremath{\Delta}}\ensuremath{\rightarrow}0$ actually does not correspond to the spectrum strictly at $\mathrm{\ensuremath{\Delta}}=0$. In particular, in the two-channel Kondo model, the $\mathrm{\ensuremath{\Delta}}\ensuremath{\rightarrow}0$ ground state is an orbitally degenerate spin singlet, while it is an orbital singlet with a residual spin degeneracy at $\mathrm{\ensuremath{\Delta}}=0$. In addition, there are fractionalized spin-1/2 subgap excitations whose energy in units of $\mathrm{\ensuremath{\Delta}}$ tends toward a finite and universal value when $\mathrm{\ensuremath{\Delta}}\ensuremath{\rightarrow}0$, as if the universality of the anomalous power-law exponents that characterize the overscreened Kondo effect turned into universal energy ratios when the scale invariance is broken by $\mathrm{\ensuremath{\Delta}}\ensuremath{\ne}0$. This intriguing phenomenon can be explained by the renormalization flow toward the overscreened fixed point and the gap cutting off the orthogonality catastrophe singularities. We also find other non-Fermi-liquid features at finite $\mathrm{\ensuremath{\Delta}}$: the local density of states lacks coherence peaks, the states in the continuum above the gap are unconventional, and the boundary entropy is a nonmonotonic function of temperature. The persistent subgap excitations are characteristic of the non-Fermi-liquid fixed point of the model, and thus depend on the impurity spin and the number of screening channels.

DOI
10.1103/physrevb.95.085121

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We study how the non-Fermi-liquid nature of the overscreened multichannel Kondo impurity model affects the response to a BCS pairing term that, in the absence of the impurity, opens a gap \ensuremathΔ\mathrm{\ensuremath{\Delta}}\ensuremathΔ. We find that the low-energy spectrum in the limit \ensuremathΔ\ensuremath→0\mathrm{\ensuremath{\Delta}}\ensuremath{\rightarrow}0\ensuremathΔ\ensuremath→0 actually does not correspond to the spectrum strictly at \ensuremathΔ=0\mathrm{\ensuremath{\Delta}}=0\ensuremathΔ=0. In particular, in the two-channel Kondo model, the \ensuremathΔ\ensuremath→0\mathrm{\ensuremath{\Delta}}\ensuremath{\rightarrow}0\ensuremathΔ\ensuremath→0 ground state is an orbitally degenerate spin singlet, while it is an orbital singlet with a residual spin degeneracy at \ensuremathΔ=0\mathrm{\ensuremath{\Delta}}=0\ensuremathΔ=0. In addition, there are fractionalized spin-1/2 subgap excitations whose energy in units of \ensuremathΔ\mathrm{\ensuremath{\Delta}}\ensuremathΔ tends toward a finite and universal value when \ensuremathΔ\ensuremath→0\mathrm{\ensuremath{\Delta}}\ensuremath{\rightarrow}0\ensuremathΔ\ensuremath→0, as if the universality of the anomalous power-law exponents that characterize the overscreened Kondo effect turned into universal energy ratios when the scale invariance is broken by \ensuremathΔ\ensuremath≠0\mathrm{\ensuremath{\Delta}}\ensuremath{\ne}0\ensuremathΔ\ensuremath=0. This intriguing phenomenon can be explained by the renormalization flow toward the overscreened fixed point and the gap cutting off the orthogonality catastrophe singularities. We also find other non-Fermi-liquid features at finite \ensuremathΔ\mathrm{\ensuremath{\Delta}}\ensuremathΔ: the local density of states lacks coherence peaks, the states in the continuum above the gap are unconventional, and the boundary entropy is a nonmonotonic function of temperature. The persistent subgap excitations are characteristic of the non-Fermi-liquid fixed point of the model, and thus depend on the impurity spin and the number of screening channels.
The traditional multichannel Kondo effect takes place when several gapless metallic electronic channels interact with a localized spin-SSS impurity, with the number of channels nnn exceeding the size of the impurity spin, n>2Sn>2Sn>2S, leading to the emergence of non-Fermi liquid impurity behavior at low temperatures. Here, we show that the effect can be realized even when the electronic degrees of freedom are strongly correlated and gapped. The system under consideration consists of a single spin-12\frac{1}{2}21​ impurity coupled isotropically to nnn spin singlet superconducting channels realized by one-dimensional leads with quasi-long-range superconducting order. The competition between the Kondo and superconducting fluctuations induces multiple distinct ground states and boundary phases depending on the relative strengths of the bulk and boundary interactions. Using the Bethe Ansatz technique, we identify four regimes: an overscreened Kondo phase, a zero-mode phase, a Yu-Shiba-Rusinov (YSR) phase, and a local-moment phase with an unscreened impurity, each with its own experimental characteristic. We describe the renormalization-group flow, the excitation spectrum, and the full impurity thermodynamics in each phase. Remarkably, even in the presence of a bulk mass gap, the boundary critical behavior in the Kondo phase is governed by the same exponents as in the gapless theory with the low-energy impurity sector flowing to the SU(2)nSU(2)_nSU(2)n​ Wess-Zumino-Witten (WZW) fixed point, and the impurity entropy monotonically decreasing as a function of temperature. In both the overscreened Kondo and zero-mode phases, the residual impurity entropy is Simp(T→0)=ln⁡[2cos⁡(π/(n+2))]S_{\mathrm{imp}}(T \to 0) = \ln[2\cos(π/(n+2))]Simp​(T→0)=ln[2cos(π/(n+2))]. In the YSR and unscreened phases on the other hand the impurity entropy exhibits non-monotonic temperature dependence and is effectively free at low temperatures with Simp(T→0)=ln⁡2S_{\mathrm{imp}}(T \to 0) = \ln 2Simp​(T→0)=ln2.
A multichannel Kondo model, where two or more equivalent but independent channels of electrons compete to screen a spin-12\frac{1}{2}21​ impurity, shows overcompensation of the impurity spin, leading to the non-Fermi-liquid behavior in various thermodynamic and transport properties. However, when the channel symmetry is broken, an impurity quantum phase transition can occur at zero temperature. Identification of an order parameter describing the impurity quantum phase transition is very difficult since it is beyond the conventional Landau-Ginzburg-Wilson theory. By employing the natural orbitals renormalization group method, we study both two-channel and three-channel Kondo models, from the perspective of spin correlation between the impurity and electrons in electronic channels. Here we demonstrate that by introducing the spin-correlation ratio as an order parameter we can characterize impurity quantum phase transitions driven by channel asymmetry. In particular, the universal critical exponents $\ensuremath{\beta}$ of the spin-correlation ratio and $\ensuremath{\nu}$ of the correlation length are explicitly determined by finite-size-scaling analysis, namely, $\ensuremath{\beta}=0.10(1)$ and $\ensuremath{\nu}=2.0(1)$, and $\ensuremath{\beta}=0.10(1)$ and $\ensuremath{\nu}=2.5(1)$ for the two-channel and three-channel Kondo models, respectively.
Entanglement entropy (EE) is commonly studied using real-space bipartitions. We show that, in quantum impurity models, an energy-space bipartition, equivalent to the momentum-space bipartition of the bath, can display universal behavior. Motivated by poor man's scaling, we logarithmically discretize the bath and partition it into high- and low-energy sectors. For models with Fermi-liquid fixed points, including the Anderson model and fully screened or underscreened Kondo models, the low-energy EE flows to constants independent of model parameters. These constants are integer multiples of ln⁡2\ln 2ln2 plus corrections that depend only on the logarithmic discretization parameter ΛΛΛ. We show that scale invariance of the fixed-point wavefunction in energy space maps to effective translation invariance along a one-dimensional chain, allowing the fixed points to be classified by one-dimensional topological band theory. With low-energy chiral symmetry, each ln⁡2\ln 2ln2 contribution originates from a topological edge mode. We also study transitions between distinct Fermi-liquid fixed points using the local-singlet--Kondo-singlet transition in a two-orbital Anderson model driven by an inter-orbital antiferromagnetic coupling. The local-singlet phase has an effectively decoupled impurity and nearly vanishing EE, whereas the Kondo-singlet phase has finite EE larger than ln⁡2\ln 2ln2 per spin and orbital. When chiral symmetry holds at low energies, this distinction corresponds to a topological transition of the effective bath chain. At the non-Fermi-liquid critical point, the EE develops an unstable plateau. Its ΛΛΛ dependence resembles that of the overscreened two-channel Kondo model, supporting universality within the same non-Fermi-liquid universality class.
The Kondo problem, which describes the interaction of a spin sss magnetic impurity with a free Fermi gas, is a classic example of strongly coupled physics. Historically, the problem has been solved by Wilson's numerical renormalization group and later by Bethe ansatz. In this paper, we present an alternate analytic solution of the Kondo problem that combines an expansion in 1/s1/s1/s with the renormalization group. We study both the case of an impurity interacting with a single channel K=1K=1K=1 of fermions in the s→∞s \rightarrow \inftys→∞ limit and the case with KKK channels in the double-scaling limit K→∞K \rightarrow \inftyK→∞, s→∞s \to \inftys→∞, K/sK/sK/s fixed. Our approach allows us to describe analytically intermediate scales of the Kondo problem at large sss and compute thermodynamic observables such as the impurity entropy and susceptibility. We find these observables to agree with the Bethe ansatz results. We also compute the impurity spectral function, finite temperature resistivity and the Kondo screening cloud profile, properties that are not easily accessible from Bethe ansatz. Notably, in the regime K>2sK > 2sK>2s we access the "non-Fermi-liquid" overscreened fixed point of the multichannel Kondo problem.
We discuss the two-channel Kondo problem with a pseudogap density of states $\ensuremath{\rho}(\ensuremath{\omega})\ensuremath{\propto}{|\ensuremath{\omega}|}^{r}$ of the bath fermions. Combining both analytical and numerical renormalization group techniques, we characterize the impurity phases and quantum phase transitions of the relevant Kondo and Anderson models. The line of stable points, corresponding to the overscreened non-Fermi-liquid behavior of the metallic r=0r=0r=0 case, is replaced by a stable particle-hole-symmetric intermediate-coupling fixed point for $0<r<{r}_{\mathrm{max}}\ensuremath{\approx}0.23$. For r>rmaxr>{r}_{\mathrm{max}}r>rmax​, this non-Fermi-liquid phase disappears, and instead a critical fixed point with an emergent spin-channel symmetry appears, controlling the quantum phase transition between two phases with stable spin and channel moments, respectively. We propose low-energy field theories to describe the quantum phase transitions, all being formulated in fermionic variables. We employ $\ensuremath{\epsilon}$ expansion techniques to calculate critical properties near the critical dimensions r=0r=0r=0 and 1, the latter being potentially relevant for two-channel Kondo impurities in neutral graphene. We find the analytical results to be in excellent agreement with those obtained from applying Wilson's numerical renormalization group technique.
We investigate quantum transport through the Kondo impurity assuming both a large number of orbital channels $\mathcal{K}\ensuremath{\gg}1$ for the itinerant electrons and a semiclassical spin $\mathcal{S}\phantom{\rule{4pt}{0ex}}\ensuremath{\gg}\phantom{\rule{4pt}{0ex}}1$ for the impurity. The non-Fermi-liquid regime of the Kondo problem is achieved in the overscreened sector K>2S\mathcal{K}>2\mathcal{S}K>2S. We show that there exist two distinct semiclassical regimes for the quantum transport through impurity: (i) $\mathcal{K}\phantom{\rule{4pt}{0ex}}\ensuremath{\gg}\phantom{\rule{4pt}{0ex}}\mathcal{S}\phantom{\rule{4pt}{0ex}}\ensuremath{\gg}\phantom{\rule{4pt}{0ex}}1$, differential conductance vanishes, and (ii) S/K=C\mathcal{S}/\mathcal{K}=\mathcal{C}S/K=C with 0<C<1/20<\mathcal{C}<1/20<C<1/2, differential conductance reaches some nonvanishing fraction of its unitary value. Using the conformal field theory approach we analyze the behavior of the quantum transport observables and residual entropy in both semiclassical regimes. We show that the semiclassical limit (ii) preserves the key features of resonance scattering and the most essential fingerprints of the non-Fermi-liquid behavior. We discuss possible realization of two semiclassical regimes in semiconductor quantum transport experiments.