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arXiv:2408.12650

The Kondo impurity in the large spin limit

Abijith Krishnan, Max A. Metlitski

Published Aug 22, 2024• 0 citations
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Abstract

The Kondo problem, which describes the interaction of a spin $s$ magnetic impurity with a free Fermi gas, is a classic example of strongly coupled physics. Historically, the problem has been solved by Wilson's numerical renormalization group and later by Bethe ansatz. In this paper, we present an alternate analytic solution of the Kondo problem that combines an expansion in $1/s$ with the renormalization group. We study both the case of an impurity interacting with a single channel $K=1$ of fermions in the $s \rightarrow \infty$ limit and the case with $K$ channels in the double-scaling limit $K \rightarrow \infty$, $s \to \infty$, $K/s$ fixed. Our approach allows us to describe analytically intermediate scales of the Kondo problem at large $s$ and compute thermodynamic observables such as the impurity entropy and susceptibility. We find these observables to agree with the Bethe ansatz results. We also compute the impurity spectral function, finite temperature resistivity and the Kondo screening cloud profile, properties that are not easily accessible from Bethe ansatz. Notably, in the regime $K > 2s$ we access the "non-Fermi-liquid" overscreened fixed point of the multichannel Kondo problem.

DOI
10.48550/arxiv.2408.12650

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The Kondo problem, which describes the interaction of a spin sss magnetic impurity with a free Fermi gas, is a classic example of strongly coupled physics. Historically, the problem has been solved by Wilson's numerical renormalization group and later by Bethe ansatz. In this paper, we present an alternate analytic solution of the Kondo problem that combines an expansion in 1/s1/s1/s with the renormalization group. We study both the case of an impurity interacting with a single channel K=1K=1K=1 of fermions in the s→∞s \rightarrow \inftys→∞ limit and the case with KKK channels in the double-scaling limit K→∞K \rightarrow \inftyK→∞, s→∞s \to \inftys→∞, K/sK/sK/s fixed. Our approach allows us to describe analytically intermediate scales of the Kondo problem at large sss and compute thermodynamic observables such as the impurity entropy and susceptibility. We find these observables to agree with the Bethe ansatz results. We also compute the impurity spectral function, finite temperature resistivity and the Kondo screening cloud profile, properties that are not easily accessible from Bethe ansatz. Notably, in the regime K>2sK > 2sK>2s we access the "non-Fermi-liquid" overscreened fixed point of the multichannel Kondo problem.
We analyze the single-channel Kondo model using the recently developed unitary renormalization-group (URG) method and obtain a comprehensive understanding of the Kondo screening cloud. The fixed-point low-energy Hamiltonian enables the computation of a plethora of thermodynamic quantities (specific heat, susceptibility, Wilson ratio, etc.) as well as spectral functions, all of which are found to be in good agreement with known results. By integrating out the impurity, we obtain an effective Hamiltonian for the excitations of the electrons comprising the Kondo cloud. This is found to contain both kkk-space number diagonal (Fermi liquid) and off-diagonal four-fermion scattering terms. Our conclusions are reinforced by a URG study of the two-particle entanglement and many-body correlations among members of the Kondo cloud and impurity. The entanglement between the impurity and a cloud electron, as well as between any two cloud electrons, is found to increase under flow towards the singlet ground state at the strong-coupling fixed point. Both the number diagonal and off-diagonal correlations within the conduction cloud are also found to increase as the impurity is screened under the flow, and the latter are found to be responsible for the macroscopic entanglement of the Kondo-singlet ground state. The URG flow enables an analytic computation of the phase shifts suffered by the conduction electrons at the strong-coupling fixed point. This reveals an orthogonality catastrophe between the local-moment and strong-coupling ground states and is related to a change in the Luttinger volume of the conduction bath under the crossover to strong coupling. Our results offer fresh insight into the nature of the emergent many-particle entanglement within the Kondo cloud and pave the way for further investigations in more exotic contexts such as the fixed point of the overscreened multichannel Kondo problem.
We propose a possible realization of the overscreened Kondo impurity problem by a magnetic s=1/2s=1/2s=1/2 impurity embedded in a two-dimensional S=1S=1S=1 U(1)U(1)U(1) spin liquid with a Fermi surface. This problem contains an interesting interplay between non-Fermi-liquid behavior induced by a U(1)U(1)U(1) gauge field coupled to fermions and a non-Fermi-liquid fixed point in the overscreened Kondo problem. Using a large-NNN expansion together with an expansion in the dynamical exponent of the gauge field, we find that the coupling to the gauge field leads to weak but observable changes in the physical properties of the system at the overscreened Kondo fixed point. We discuss the extrapolation of this result to a physical case and argue that the realization of overscreened Kondo physics could lead to observations of effects due to gauge fields.
The feasibility of realizing the overscreened Kondo effect in ultracold Fermi gas of atoms with spin $s\ensuremath{\ge}\frac{3}{2}$ in the presence of a localized magnetic impurity atom is proved realistic. Specifying (as a mere example) a system of ultracold 22Na^{22}\mathrm{Na}22Na Fermi gas and a trapped 6Li^{6}\mathrm{Li}6Li impurity, the mechanism of exchange interaction between the Na and Li atoms is elucidated and the exchange constant is found to be positive (antiferromagnetic). The corresponding exchange Hamiltonian is derived, and the Kondo temperature is estimated at the order of 500 nK. Within a weak-coupling renormalization group scheme, it is shown that the coupling renormalizes to the non-Fermi-liquid fixed point. An observable displaying multichannel features even in the weak-coupling regime is the impurity magnetization that is negative for $T\ensuremath{\gg}{T}_{K}$ and becomes positive with decreasing temperature.
The traditional multichannel Kondo effect takes place when several gapless metallic electronic channels interact with a localized spin-SSS impurity, with the number of channels nnn exceeding the size of the impurity spin, n>2Sn>2Sn>2S, leading to the emergence of non-Fermi liquid impurity behavior at low temperatures. Here, we show that the effect can be realized even when the electronic degrees of freedom are strongly correlated and gapped. The system under consideration consists of a single spin-12\frac{1}{2}21​ impurity coupled isotropically to nnn spin singlet superconducting channels realized by one-dimensional leads with quasi-long-range superconducting order. The competition between the Kondo and superconducting fluctuations induces multiple distinct ground states and boundary phases depending on the relative strengths of the bulk and boundary interactions. Using the Bethe Ansatz technique, we identify four regimes: an overscreened Kondo phase, a zero-mode phase, a Yu-Shiba-Rusinov (YSR) phase, and a local-moment phase with an unscreened impurity, each with its own experimental characteristic. We describe the renormalization-group flow, the excitation spectrum, and the full impurity thermodynamics in each phase. Remarkably, even in the presence of a bulk mass gap, the boundary critical behavior in the Kondo phase is governed by the same exponents as in the gapless theory with the low-energy impurity sector flowing to the SU(2)nSU(2)_nSU(2)n​ Wess-Zumino-Witten (WZW) fixed point, and the impurity entropy monotonically decreasing as a function of temperature. In both the overscreened Kondo and zero-mode phases, the residual impurity entropy is Simp(T→0)=ln⁡[2cos⁡(π/(n+2))]S_{\mathrm{imp}}(T \to 0) = \ln[2\cos(π/(n+2))]Simp​(T→0)=ln[2cos(π/(n+2))]. In the YSR and unscreened phases on the other hand the impurity entropy exhibits non-monotonic temperature dependence and is effectively free at low temperatures with Simp(T→0)=ln⁡2S_{\mathrm{imp}}(T \to 0) = \ln 2Simp​(T→0)=ln2.
We analyze the single-channel Kondo model using the recently developed unitary renormalization group (URG) method, and obtain a comprehensive understanding of the Kondo screening cloud. The fixed-point low-energy Hamiltonian enables the computation of a plethora of thermodynamic quantities (specific heat, susceptibility, Wilson ratio, etc.) as well as spectral functions, all of which are found to be in excellent agreement with known results. By integrating out the impurity, we obtain an effective Hamiltonian for the excitations of the electrons comprising the Kondo cloud. This is found to contain both k-space number-diagonal (Fermi liquid) as well off-diagonal four-fermion scattering terms. Our conclusions are reinforced by a URG study of the two-particle entanglement and many-body correlations among members of the Kondo cloud and impurity. The entanglement between the impurity and a cloud electron, as well as between any two cloud electrons, is found to increase under flow towards the singlet ground state at the strong-coupling fixed point. Both the number-diagonal and off-diagonal correlations within the conduction cloud are also found to increase as the impurity is screened under the flow, and the latter are found to be responsible for the macroscopic entanglement of the Kondo-singlet ground state. The unitary RG flow enables an analytic computation of the phase shifts suffered by the conduction electrons at the strong-coupling fixed point. This reveals an orthogonality catastrophe between the local moment and strong-coupling ground states, and is related to a change in the Luttinger volume of the conduction bath. Our results offer fresh insight on the nature of the emergent many-particle entanglement within the Kondo cloud, and pave the way for further investigations in more exotic contexts such as the fixed point of the over-screened multi-channel Kondo problem.
Kitaev's honeycomb-lattice compass model describes a spin liquid with emergent fractionalized excitations. Here, we study the physics of isolated magnetic impurities coupled to the Kitaev spin-liquid host. We reformulate this Kondo-type problem in terms of a many-state quantum impurity coupled to a multichannel bath of Majorana fermions and present the numerically exact solution using Wilson's numerical renormalization group technique. Quantum phase transitions occur as a function of Kondo coupling and locally applied field. At zero field, the impurity moment is partially screened only when it binds an emergent gauge flux, while otherwise it becomes free at low temperatures. We show how Majorana degrees of freedom determine the fixed-point properties, make contact with Kondo screening in pseudogap Fermi systems, and discuss effects away from the dilute limit.