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arXiv:1604.03557 · Physical Review Letters

Kondo Impurities in the Kitaev Spin Liquid: Numerical Renormalization Group Solution and Gauge-Flux-Driven Screening

Matthias Vojta C, Andrew K. Mitchell, Fabian Zschocke

Published Jul 12, 2016• 37 citations
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Abstract

Kitaev's honeycomb-lattice compass model describes a spin liquid with emergent fractionalized excitations. Here, we study the physics of isolated magnetic impurities coupled to the Kitaev spin-liquid host. We reformulate this Kondo-type problem in terms of a many-state quantum impurity coupled to a multichannel bath of Majorana fermions and present the numerically exact solution using Wilson's numerical renormalization group technique. Quantum phase transitions occur as a function of Kondo coupling and locally applied field. At zero field, the impurity moment is partially screened only when it binds an emergent gauge flux, while otherwise it becomes free at low temperatures. We show how Majorana degrees of freedom determine the fixed-point properties, make contact with Kondo screening in pseudogap Fermi systems, and discuss effects away from the dilute limit.

DOI
10.1103/physrevlett.117.037202

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Kitaev's honeycomb-lattice compass model describes a spin liquid with emergent fractionalized excitations. Here, we study the physics of isolated magnetic impurities coupled to the Kitaev spin-liquid host. We reformulate this Kondo-type problem in terms of a many-state quantum impurity coupled to a multichannel bath of Majorana fermions and present the numerically exact solution using Wilson's numerical renormalization group technique. Quantum phase transitions occur as a function of Kondo coupling and locally applied field. At zero field, the impurity moment is partially screened only when it binds an emergent gauge flux, while otherwise it becomes free at low temperatures. We show how Majorana degrees of freedom determine the fixed-point properties, make contact with Kondo screening in pseudogap Fermi systems, and discuss effects away from the dilute limit.
Geometrically frustrated quantum impurities coupled to metallic leads have been shown to exhibit rich behavior with a quantum phase transition separating Kondo screened and local moment phases. Frustration in the quantum impurity can alternatively be introduced via Kitaev couplings between different spins of the impurity cluster. We use the numerical renormalization group (NRG) to study a range of systems where the quantum impurity comprising a Kitaev cluster is coupled to a bath of noninteracting fermions. The models exhibit a competition between Kitaev and Kondo dominated physics depending on whether the Kitaev couplings are greater or less than the Kondo temperature. We characterize the ground-state properties of the system and determine the temperature dependence of the crossover scale for the emergence of fractionalized degrees of freedom in the model. We also demonstrate qualitatively as well as quantitatively that in the Kondo limit, the complex impurity can be mapped to an effective two-impurity system, where the emergent spin 1/21/21/2 comprises of both Majorana and flux degrees of freedom. For a tetrahedral-shaped Kitaev cluster, an extra orbital degree of freedom closely related to a flux degree of freedom remains unscreened even in the presence of both Heisenberg and Kondo interactions.
We study Kondo physics in the algebraic spin liquid, recently proposed to describe ZnCu3(OH)6Cl2ZnCu_{3}(OH)_{6}Cl_{2}ZnCu3​(OH)6​Cl2​ [Phys. Rev. Lett. {\bf 98}, 117205 (2007)]. Although spin dynamics of the algebraic spin liquid is described by massless Dirac fermions, this problem differs from the Pseudogap Kondo model, because the bulk physics in the algebraic spin liquid is governed by an interacting fixed point where well-defined quasiparticle excitations are not allowed. Considering an effective bulk model characterized by an anomalous critical exponent, we derive an effective impurity action in the slave-boson context. Performing the large-NσN_σNσ​ analysis with a spin index NσN_σNσ​, we find an impurity quantum phase transition from a decoupled local-moment state to a Kondo-screened phase. We evaluate the impurity spin susceptibility and specific heat coefficient at zero temperature, and find that such responses follow power-law dependencies due to the anomalous exponent of the algebraic spin liquid. Our main finding is that the Wilson's ratio for the magnetic impurity depends strongly on the critical exponent in the zero temperature limit. We propose that the Wilson's ratio for the magnetic impurity may be one possible probe to reveal criticality of the bulk system.
We study the effect of coupling magnetic impurities to the honeycomb lattice spin-1/21/21/2 Kitaev model in its spin-liquid phase. We show that a spin-SSS impurity coupled to the Kitaev model is associated with an unusual Kondo effect with an intermediate coupling unstable fixed point ${K}_{c}\ensuremath{\sim}J/S$ separating topologically distinct sectors of the Kitaev model. We also show that the massless spinons in the spin-liquid mediate an interaction of the form ${S}_{i\ensuremath{\alpha}}^{2}{S}_{j\ensuremath{\beta}}^{2}/{R}_{ij}^{3}$ between distant impurities unlike the usual dipolar RKKY interaction ${S}_{i\ensuremath{\alpha}}{S}_{j\ensuremath{\alpha}}/{R}_{ij}^{3}$ noted in various 2D impurity problems with a pseudogapped density of states of the spin bath. Furthermore, this long-range interaction is possible only if the impurities (a) couple to more than one neighboring spin on the host lattice and (b) the impurity spin $S\ensuremath{\ne}1/2$.
We investigate quantum impurity problems, where a local magnetic moment is coupled to the spin density of a bosonic environment, leading to bosonic versions of the standard Kondo and Anderson impurity models. In a physical situation, these bosonic environments can correspond either to deconfined spinons in certain classes of Z2{Z}_{2}Z2​ frustrated antiferromagnets, or to particles in a multicomponent Bose gase (in which case the spin degree of freedom is attributed to hyperfine levels). Using renormalization group techniques, we establish that our impurity models, which feature an exchange interaction analogous to Kondo impurities in Fermi liquids, allow flow toward a stable strong-coupling state. Since the low-energy bosons exist around a single point in momentum space, and there is no Fermi surface, an impurity quantum phase transition occurs at intermediate coupling, separating screened and unscreened phases. This behavior is qualitatively different from previously studied spin-isotropic variants of the spin-boson model, which display stable intermediate-coupling fixed points and no screening.
The Kondo problem, which describes the interaction of a spin sss magnetic impurity with a free Fermi gas, is a classic example of strongly coupled physics. Historically, the problem has been solved by Wilson's numerical renormalization group and later by Bethe ansatz. In this paper, we present an alternate analytic solution of the Kondo problem that combines an expansion in 1/s1/s1/s with the renormalization group. We study both the case of an impurity interacting with a single channel K=1K=1K=1 of fermions in the s→∞s \rightarrow \inftys→∞ limit and the case with KKK channels in the double-scaling limit K→∞K \rightarrow \inftyK→∞, s→∞s \to \inftys→∞, K/sK/sK/s fixed. Our approach allows us to describe analytically intermediate scales of the Kondo problem at large sss and compute thermodynamic observables such as the impurity entropy and susceptibility. We find these observables to agree with the Bethe ansatz results. We also compute the impurity spectral function, finite temperature resistivity and the Kondo screening cloud profile, properties that are not easily accessible from Bethe ansatz. Notably, in the regime K>2sK > 2sK>2s we access the "non-Fermi-liquid" overscreened fixed point of the multichannel Kondo problem.
Paramagnetic impurities in a quantum spin liquid give rise to Kondo effects with highly unusual properties. We have studied the effect of locally coupling a paramagnetic impurity with the spin-12\frac{1}{2}21​ honeycomb Kitaev model in its gapless spin-liquid phase. The (impurity) scaling equations are found to be insensitive to the sign of the coupling. The weak and strong coupling fixed points are stable, with the latter corresponding to a noninteracting vacancy and an interacting, spin-1 defect for the antiferromagnetic and ferromagnetic cases, respectively. The ground state in the strong coupling limit in both cases has a nontrivial topology associated with a finite Z2{Z}_{2}Z2​ flux at the impurity site. For the antiferromagnetic case, this result has been obtained straightforwardly owing to the integrability of the Kitaev model with a vacancy. The strong-coupling limit of the ferromagnetic case is, however, nonintegrable, and we address this problem through exact-diagonalization calculations with finite Kitaev fragments. Our exact diagonalization calculations indicate that the weak-to-strong coupling transition and the topological phase transition occur rather close to each other and are possibly coincident. We also find an intriguing similarity between the magnetic response of the defect and the impurity susceptibility in the two-channel Kondo problem.