We experimentally and theoretically investigate the nonequilibrium phase structure of a well-controlled driven-dissipative quantum spin system governed by the interplay of coherent driving, spontaneous decay, and long-range spin-spin interactions. We discover that the rate of population loss provides a convenient macroscopic observable that exhibits power-law scaling with the driving strength over several orders of magnitude. The measured scaling exponents reflect the underlying nonequilibrium phase structure of the many-body system, which includes dissipation-dominated, paramagnetic, and critical regimes as well as an instability which drives the system towards states with high excitation density. This opens up a means to study and classify quantum systems out of equilibrium and extends the domain where scale-invariant behavior may be found in nature.
We experimentally and theoretically investigate the nonequilibrium phase structure of a well-controlled driven-dissipative quantum spin system governed by the interplay of coherent driving, spontaneous decay, and long-range spin-spin interactions. We discover that the rate of population loss provides a convenient macroscopic observable that exhibits power-law scaling with the driving strength over several orders of magnitude. The measured scaling exponents reflect the underlying nonequilibrium phase structure of the many-body system, which includes dissipation-dominated, paramagnetic, and critical regimes as well as an instability which drives the system towards states with high excitation density. This opens up a means to study and classify quantum systems out of equilibrium and extends the domain where scale-invariant behavior may be found in nature.
This thesis presents several experiments investigating the regimes of behaviour of a proto-typical open quantum many-body system far away from equilibrium. The experimental platform is based on ultracold atoms laser-excited to Rydberg states, which we engineer to emulate a strongly interacting, driven-dissipative quantum spin system. The high degree of control over the relevant microscopic processes and their parameters, as well as the ability to widely tune interaction and driving strengths provides the means to address fundamental questions on how different regimes of dynamical behaviour emerge in complex open quantum systems and how they can be characterised. \n \nIn the first part, we discuss how control over the relevant properties of Rydberg spin systems, like temperature, density, long evolution times, strong interactions, tunable driving, and dissipation can be achieved. We introduce the new experimental apparatus developed during this thesis, which combines both single-photon and two-photon Rydberg excitation schemes with high atom densities and long excitation times using an optical dipole trap. Additionally, we investigate theoretically how long coherence times exceeding motional timescales combined with strong many-body interactions can be achieved in such a system. We identify an optimal parameter regime for two-photon excitation where such conditions can be generated with coherence times and interaction strengths comparable to what is achievable for single-photon excitation. \n \nIn the second part we explore the macroscopic non-equilibrium behaviour of our system and devise suitable observables for characterising different regimes of behaviour. We discover that the slow atom loss inherent to our system provides a convenient observable for the many-body state of the system. Focussing on evolution times where the effect of the atom loss on the evolution is small, we discover that the rate of atom loss exhibits powerlaw scaling with the driving strength over several orders of magnitude. The measured scaling exponents reveal the non-equilibrium phase structure of the many-body system and allow us to distinguish dissipation-dominated, paramagnetic and critical regimes, as well as an instability. In the observed critical regime, collectively enhanced driving dominates over dissipation, leading to scaling associated to the critical point of the non-dissipative equilibrium Rydberg spin system. Based on the known microscopic processes of our system, we perform classical many-body rate equation simulations, which agree well with the observed phase structure as well as the position and associated scaling exponents of the individual regimes. These findings open up new means to study and classify out of equilibrium systems based on slow particle loss and powerlaw scaling. \n \nIn the last part of this thesis we reveal a second type of criticality in our system, which is genuinely non-equilibrium in character and arises from an absorbing state phase transition. The critical state of this phase transition dominates the system evolution at late times where particle loss is no longer negligible. We identify self-organisation as the mechanism driving the system to this critical state, which we observe through powerlaw scaling of the non-equilibrium steady-state. These experiments establish Rydberg atoms as a well controlled platform for implementing and exploring models of absorbing state phase transitions and self-organised criticality with unprecedented access to the underlying microscopic properties of the system.
Due to the variety of tools available to control atomic, molecular, and optical (AMO) systems, they provide a versatile platform for studying many-body physics, quantum simulation, and quantum computation. Although extensive efforts are employed to reduce coupling between the system and the environment, the effects of the environment can never fully be avoided, so it is important to develop a comprehensive understanding of open quantum systems. The system-environment coupling often leads to loss via dissipation, which can be countered by a coherent drive. Open quantum systems subject to dissipation and drive are known as driven-dissipative systems, and they provide an excellent platform for studying many-body nonequilibrium physics. The first part of this dissertation will focus on driven-dissipative phase transitions. Despite the nonequilibrium nature of these systems, the corresponding phase transitions tend to exhibit emergent equilibrium behavior. However, we will show that in the vicinity of a multicritical point where multiple phase transitions intersect, genuinely nonequilibrium criticality can emerge, even though the individual phase transitions on their own exhibit equilibrium criticality. These nonequilibrium multicritical points can exhibit a variety of exotic phenomena not possible for their equilibrium counterparts, including the emergence of complex critical exponents, which lead to discrete scale invariance and spiraling phase boundaries. Furthermore, the Liouvillian gap can take on complex values, and the fluctuation-dissipation theorem is violated, corresponding to an effective temperature which gets "hotter" and "hotter" at longer and longer wavelengths. The second part of this dissertation will focus on Rydberg atoms. In particular, we study how the spontaneous generation of contaminant Rydberg states drastically modifies the behavior of a driven-dissipative Rydberg system due to the resultant dipole-dipole interactions. These interactions lead to a complicated competition of both blockade and anti-blockade effects, leading to strongly enhanced Rydberg populations for far-detuned drive and reduced Rydberg populations for resonant drive.
Understanding and probing phase transitions in nonequilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a nonfluctuating absorbing phase, e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here, we report the observation of signatures of such a nonequilibrium phase transition in an open driven quantum system. In our experiment, rubidium atoms in a quasi-one-dimensional cold disordered gas are laser excited to Rydberg states under so-called facilitation conditions. This conditional excitation process competes with spontaneous decay and leads to a crossover between a stationary state with no excitations and one with a finite number of excitations. We relate the underlying physics to that of an absorbing-state phase transition in the presence of a field (i.e., off-resonant excitation processes) which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of nonequilibrium phase transitions in open many-body quantum systems.
Summary form only given. Understanding and probing phase transitions in non-equilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a non-fluctuating absorbing phase [1], e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here we report the observation of signatures of such a non-equilibrium phase transition in an open driven quantum system. In our experiment rubidium atoms in a quasi one-dimensional cold disordered gas are laser-excited to Rydberg states under so-called facilitation conditions [2]. This conditional excitation process competes with spontaneous decay (see Fig. 1a) and leads to a crossover between a stationary state with no excitations and one with a finite number of Rydberg excitations (see Fig. 1b, where the phase diagram is plotted as a function of the driving strength and detuning from resonance) [3]. We relate the underlying physics to that of an absorbing state phase transition in the presence of a field which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of non-equilibrium phase transitions in open many-body quantum systems.
We study the nonequilibrium dynamics of a many-body bosonic system on a lattice, subject to driving and dissipation. The time evolution is described by a master equation, which we treat within a generalized Gutzwiller mean field approximation for density matrices. The dissipative processes are engineered such that the system, in the absence of interaction between the bosons, is driven into a homogeneous steady state with off-diagonal long-range order. We investigate how the coherent interaction affects the properties of the steady state of the system qualitatively and derive a nonequilibrium phase diagram featuring a phase transition into a steady state without long-range order. The phase diagram also exhibits an extended domain where an instability of the homogeneous steady state gives rise to a persistent density pattern with spontaneously broken translational symmetry. In the limit of low particle density, we provide a precise analytical description of the time evolution during the instability. Moreover, we investigate the transient following a quantum quench of the dissipative processes and we elucidate the prominent role played by collective topological variables in this regime.
We explore the nonequilibrium evolution and stationary states of an open many-body system that displays epidemic spreading dynamics in a classical and a quantum regime. Our study is motivated by recent experiments conducted in strongly interacting gases of highly excited Rydberg atoms where the facilitated excitation of Rydberg states competes with radiative decay. These systems approximately implement open quantum versions of models for population dynamics or disease spreading where species can be in a healthy, infected or immune state. We show that in a two-dimensional lattice, depending on the dominance of either classical or quantum effects, the system may display a different kind of nonequilibrium phase transition. We moreover discuss the observability of our findings in laser driven Rydberg gases with particular focus on the role of long-range interactions.