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arXiv:1603.05425 · Physical Review A

Linear and nonlinear magneto-optical rotation on the narrow strontium intercombination line

Kanhaiya Pandey, Chang Chi Kwong, Mysore Srinivas Pramod, David Wilkowski

Published May 31, 2016• 15 citations
arXivHTMLPDF

Abstract

In the presence of an external static magnetic field, an atomic gas becomes optically active, showing magneto-optical rotation. In the saturated regime, the coherences among the excited substates give a nonlinear contribution to the rotation of the light polarization. In contrast with the linear magneto-optical rotation, the nonlinear counterpart is insensitive to Doppler broadening. By varying the temperature of a cold strontium gas, we observe both regimes by driving the $J=0\ensuremath{\rightarrow}J=1$ transition on the intercombination line. For this narrow transition, the sensitivity to the static magnetic field is typically three orders of magnitude larger than for a standard broad alkali-metal transition.

DOI
10.1103/physreva.93.053428

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In the presence of an external static magnetic field, an atomic gas becomes optically active, showing magneto-optical rotation. In the saturated regime, the coherences among the excited substates give a nonlinear contribution to the rotation of the light polarization. In contrast with the linear magneto-optical rotation, the nonlinear counterpart is insensitive to Doppler broadening. By varying the temperature of a cold strontium gas, we observe both regimes by driving the J=0\ensuremath→J=1J=0\ensuremath{\rightarrow}J=1J=0\ensuremath→J=1 transition on the intercombination line. For this narrow transition, the sensitivity to the static magnetic field is typically three orders of magnitude larger than for a standard broad alkali-metal transition.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
We theoretically investigate magneto-optical rotation (MOR) of a linearly polarized probe field in the four-level N-type cold atoms. By applying a static magnetic field and a weak coupling field, it is shown that the birefringence enhancement is induced in the system. Moreover, we show that the static magnetic field has a major role in switching the dichroism to enhanced birefringence in the system. We also obtain a large intensity for the output field with nearly perpendicular MOR angle by 88 degrees with subnatural width. It is demonstrated that Doppler broadening has a destructive effect on the MOR of the polarization direction of the probe field. The results of our study can be used for selecting narrow band of wavelengths and polarization converter for efficient switching of TM/TE polarization modes in optical communication, the depolarization backscattering lidar, polarization spectroscopy and precision measurements.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
We study the coherent transmission of light through cold strontium atomic clouds, using the narrow intercombination line. In the first part of the thesis, the cooperative emission in the coherent transmission is studied experimentally. By applying fast changes to the incident probe field, flashes of light are observed in the forward direction. The peak intensity of the flashes can be much larger than the incident intensity. These flashes are called superflashes. Due to cooperative effect, the time scale of the flashes are shortened with respect to the single scatterer lifetime. By packing these flashes, we generate a pulse train with short repetition time, where the dynamics can almost be fully governed by cooperative effect. The effect of atomic density on the coherent transmission of light is also studied theoretically and numerically. The effective refractive index of the cloud is calculated up to the second order in atomic density. It is eventually validated with a numerical simulation of the coherent light transmission. The second part of the thesis focuses on the effect of magnetic field on the coherent transmission of light. The strontium intercombination line has a sensitivity in the milligauss regime, which is the typical value of stray magnetic field in the lab. An active magnetic field control system is implemented to cancel the low frequency and AC 50~Hz stray magnetic field. Using this control system, we study the nonlinear magneto-optical rotation (NMOR) effect due to a high intensity light field transmitting through a dilute and thin cloud of strontium atom. Interestingly, at sufficiently high cloud temperature, the NMOR effect can have a higher sensitivity to the magnetic field, compared to its linear counterpart at the same cloud temperature.
Nonlinear in laser power, near-resonant light-atom interaction leads to a number of spectacular modifications of a well-known effect -polarization plane rotation in a magnetic field applied along the direction of light propagation.In particular, the rotation can be enhanced by up to nine orders of magnitude compared to the linear case.Faraday effect [ 1 ] is the rotation of the plane of linear light polarization by a medium in a magnetic field applied in the direction of light propagation.In 1898, Macaluso and Corbino eJ, studying absorption spectra of the alkali atoms in the presence of magnetic fields, discovered that the Faraday effect in the vicinity of resonance absorption lines also had a distinct resonant character.The essence of the Macaluso-Corbino effect can be illustrated by considering a simple case of a F= 1 ~ F'=O transition (Fig. 1 ).Linearly polarized light incident on the sample can be resolved into two counter-rotating circular components ( cr~.In the absence of a magnetic field, the M=±l sublevels are degenerate and the optical resonance
We present, experimentally and theoretically, nonlinear magneto-optical rotation (NMOR) using two spatially separated laser beams, the pump laser beam for creation and the probe laser beam for detection of the coherence between ground Zeeman sublevels. Both pump and probe lasers are tuned to ${F}_{g}=2\ensuremath{\rightarrow}{F}_{e}=1$ transition in 87Rb^{87}\text{R}\text{b}87Rb. With the specially designed spatial configuration of the pump and the probe beams we were able to obtain dispersively shaped probe laser NMOR resonances in the Rb vacuum gas cell. The theory indicates that the obtained line shapes are due to the interference between prepared atomic states and the probe laser field. The interference nature of the resonances is supported by narrowing of NMOR resonances with increased separation between laser beams, and by the shift of the central fringe from the zero magnetic field with increased angle between initial orientation of electric vectors of linearly polarized pump and probe beams.