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arXiv:1603.00970 · Journal of the Optical Society of America B

An inverted crossover resonance aiding laser cooling of ^171Yb

John J. McFerran

Published May 24, 2016• 12 citations
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Abstract

We observe an inverted crossover resonance in π-driven four-level systems, where F′−F=0,+1. The signal is observed through saturated absorption spectroscopy of the (6s2)S01−(6s6p)P13 transition in Yb171, where the nuclear spin I=1/2. The enhanced absorption signal is used to generate a dispersive curve for 556 nm laser frequency stabilization and the stabilized light cools Yb171 atoms in a two-stage magneto-optical trap, achieving temperatures of 20 μK. The Doppler-free spectroscopy scheme is further used to measure isotopic frequency shifts and hyperfine separations for the inter-combination line in ytterbium.

DOI
10.1364/josab.33.001278

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We observe an inverted crossover resonance in π-driven four-level systems, where F′−F=0,+1. The signal is observed through saturated absorption spectroscopy of the (6s2)S01−(6s6p)P13 transition in Yb171, where the nuclear spin I=1/2. The enhanced absorption signal is used to generate a dispersive curve for 556 nm laser frequency stabilization and the stabilized light cools Yb171 atoms in a two-stage magneto-optical trap, achieving temperatures of 20 μK. The Doppler-free spectroscopy scheme is further used to measure isotopic frequency shifts and hyperfine separations for the inter-combination line in ytterbium.
Anomalous saturated absorption providing a stable laser lock for 171^{171}171Yb laser cooling
We identify an inverted Lamb dip in the saturated absorption spectroscopy of the (6s2)(6s^{2})(6s2) 1S0^{1}S_{0}1S0​ −-− (6s6p)(6s6p)(6s6p) 3P1^{3}P_{1}3P1​ transition in 171^{171}171Yb. The signal has only been observed with the two hyperfine lines of this spin I=12I=\frac{1}{2}I=21​ isotope. For both lines the application of a dc magnetic field transforms a two-level scheme into a four-level scheme, with degeneracy only marginally lifted in the ground state. The atoms are excited through π\piπ transitions, while the de-excitation process completes a simple optical pumping scheme. However, the full explanation of the enhanced absorption is yet to be determined. The anomalous absorption signal is used to generate a dispersive curve for 556 nm laser stabilisation and the stabilised light cools 171^{171}171Yb atoms in a two-stage magneto-optical trap, achieving temperatures below 50 μ\muμK. The Doppler-free spectroscopy scheme is further used to measure isotopic frequency shifts and hyperfine separations for the intercombination line in Yb.
Abstract We carry out investigations of inverted crossover resonances (ICRs) in π -driven four-level systems where Δ F can be zero. Through the use of sub-Doppler frequency modulation spectroscopy of the ( 6 s 2 ) 1 S 0 − ( 6 s 6 p ) 3 P 1 transition in 171 Yb the resonance becomes manifest. The centre frequency is inherently insensitive to first-order Zeeman shifts and equates to the two-level resonance frequency in the absence of a magnetic field. A rate equation model is used to help validate the nature of the resonance. Optical frequency measurements of the F ′ = 1 / 2 hyperfine line recorded over two months demonstrate a statistical uncertainty of 2 × 10 −11 . The ICR found with the F ′ = 3 / 2 line is used for 556 nm laser frequency stabilisation, which is an alternative means when applied to magneto-optical trapping of 171 Yb.
We report on the sub-Doppler laser cooling of neutral Yb171 and Yb173 in a magneto-optical trap (MOT) using the S10−P11 transition at 398.9 nm. We use two independent means to estimate the temperature of the atomic cloud for several of the Yb isotopes. The two methods of MOT cloud imaging and release-and-recapture show consistency with one another. Temperatures below 400 and 200 μK are recorded for Yb171 and Yb173, respectively, while ∼1 mK is measured for both Yb172 and Yb174. By comparison, the associated one-dimensional Doppler cooling temperature limit is 694 μK. The sub-Doppler cooling of the I=1/2Yb171 isotope in a σ+−σ− light-field trap adds further evidence that the Sisyphus cooling mechanism is occurring in such three-dimensional MOTs.
We demonstrate the presence of inverted crossover resonances (ICRs) in the intercombination line of171Yb (I=1/2) with the use of saturated fluorescence spectroscopy on an atomic beam. The principal lines involved in the crossover are symmetrically separated Zeeman transitions. The signals are observed for both the hyperfine lines of the171Yb1S0-3P1line. We use a four-level rate equation model to help validate the nature of the resonance. In the case of F'=3/2 (upper state) the resonance can be used to frequency stabilize laser light for laser cooling of171Yb. While that of the F'=1/2 ICR acts as a rather robust frequency reference with an overall fractional frequency uncertainty in the low 10-11range.
We report the direct excitation of the highly forbidden (6s2) 1S0 <--> (6s6p) 3P0 optical transition in two odd isotopes of neutral ytterbium. As the excitation laser frequency is scanned, absorption is detected by monitoring the depletion from an atomic cloud at approximately 70 microK in a magneto-optical trap. The measured frequency in 171Yb (F=1/2) is 518,295,836,591.6 +/- 4.4 kHz. The measured frequency in 173Yb (F=5/2) is 518,294,576,847.6 +/- 4.4 kHz. Measurements are made with a femtosecond-laser frequency comb calibrated by the National Institute of Standards and Technology cesium fountain clock and represent nearly a 10(6)-fold reduction in uncertainty. The natural linewidth of these J=0 to J=0 transitions is calculated to be approximately 10 mHz, making them well suited to support a new generation of optical atomic clocks based on confinement in an optical lattice.
We calculate and measure the magic wavelengths for the $6{s}^{2}^{1}S_{0}\ensuremath{-}6s6p\phantom{\rule{0.16em}{0ex}}^{3}P_{1}$ intercombination transition of the neutral ytterbium atom. The calculation is performed with the ab initio configuration interaction +++ all-order method. The measurement is done with laser spectroscopy on cold atoms in an optical dipole trap. The magic wavelengths are determined to be 1035.68(4) nm for the $\ensuremath{\pi}$ transition $(\mathrm{\ensuremath{\Delta}}m=0)$ and 1036.12(3) nm for the $\ensuremath{\sigma}$ transitions $(|\mathrm{\ensuremath{\Delta}}m|=1)$ in agreement with the calculated values. Laser cooling on the narrow intercombination transition could achieve better results for atoms in an optical dipole trap when the trap wavelength is tuned to near the magic wavelength.