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arXiv:1602.01775 · Physical Review A

Enhanced violation of the Collins-Gisin-Linden-Massar-Popescu inequality with optimized time-bin-entangled ququarts

Takuya Ikuta, Hiroki Takesue

Published Feb 4, 2016• 24 citations
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Abstract

High-dimensional quantum entanglement is drawing attention because it enables us to perform quantum information tasks that are robust against noises. To test the nonlocality of entangled qudits, the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality has been proposed and demonstrated using qudits based on orbital angular momentum, time-energy uncertainty, and frequency bins. Here, we report the generation and observation of time-bin entangled ququarts. We implemented a measurement for the CGLMP inequality test using cascaded delay Mach-Zehnder interferometers fabricated by using planar light-wave circuit technology, with which we achieved a precise and stable measurement for time-bin-entangled ququarts. In addition, we generated an optimized entangled state by modulating the pump pulse intensities, with which we can observe the theoretical maximum violation for the CGLMP inequality test. As a result, we successfully observed a Bell-type parameter ${S}_{4}=2.774\ifmmode\pm\else\textpm\fi{}0.025$ violating the CGLMP inequality for the maximally entangled state and an enhanced Bell-type parameter ${S}_{4}=2.913\ifmmode\pm\else\textpm\fi{}0.023$ for the optimized entangled state.

DOI
10.1103/physreva.93.022307

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High-dimensional quantum entanglement is drawing attention because it enables us to perform quantum information tasks that are robust against noises. To test the nonlocality of entangled qudits, the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality has been proposed and demonstrated using qudits based on orbital angular momentum, time-energy uncertainty, and frequency bins. Here, we report the generation and observation of time-bin entangled ququarts. We implemented a measurement for the CGLMP inequality test using cascaded delay Mach-Zehnder interferometers fabricated by using planar light-wave circuit technology, with which we achieved a precise and stable measurement for time-bin-entangled ququarts. In addition, we generated an optimized entangled state by modulating the pump pulse intensities, with which we can observe the theoretical maximum violation for the CGLMP inequality test. As a result, we successfully observed a Bell-type parameter S4=2.774\ifmmode±\else\textpm\fi0.025{S}_{4}=2.774\ifmmode\pm\else\textpm\fi{}0.025S4​=2.774\ifmmode±\else\textpm\fi0.025 violating the CGLMP inequality for the maximally entangled state and an enhanced Bell-type parameter S4=2.913\ifmmode±\else\textpm\fi0.023{S}_{4}=2.913\ifmmode\pm\else\textpm\fi{}0.023S4​=2.913\ifmmode±\else\textpm\fi0.023 for the optimized entangled state.
Characterizing high-dimensional entangled states holds pivotal significance in quantum information science and technology. Recent theoretical progress has been made to extend the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality into a general scenario with multisetting and multidimensional systems. Here, by employing two-photon orbital angular momentum entanglement, we conduct an experiment to demonstrate the CGLMP inequality across multiple settings and outcomes. Our experimental results violate the CGLMP inequality by more than 12 standard deviations, demonstrating that the maximum violation increases with both dimension and setting. Furthermore, we reveal, both theoretically and experimentally, the logical connection between the CGLMP inequality and the general Hardy's paradox. Intriguingly, our analysis establishes that, even in high-dimensional systems, Hardy's paradox can be regarded as a special instance of Bell inequality, with their respective bounds aligning under the no-signaling principle and the information causality principle. Our work may advance the foundational understanding of quantum correlations in high-dimensional quantum systems.
The question of how Bell nonlocality behaves in bipartite systems of higher dimensions is addressed. By employing the probability of violation of local realism under random measurements as the figure of merit, we investigate the nonlocality of entangled qudits with dimensions ranging from d=2d=2d=2 up to d=10d=10d=10. We proceed in two complementary directions. First, we study the specific Bell scenario defined by the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality. Second, we consider the nonlocality of the same states under a more general perspective by directly addressing the space of joint probabilities (computing the frequencies of behaviours outside the local polytope). In both approaches we find that the nonlocality decreases as the dimension ddd grows, but in quite distinct ways. While the drop in the probability of violation is exponential in the CGLMP scenario, it presents, at most, a linear decay in the space of behaviors. Furthermore, in the latter approach the states that produce maximal numeric violations in the CGLMP inequality present low probabilities of violation in comparison to maximally entangled states, so no anomaly is observed. Finally, the nonlocality of states with nonmaximal Schmidt rank is investigated.
We present a much simplified version of the Collins-Gisin-Linden-Massar-Popescu inequality for the $2\ifmmode\times\else\texttimes\fi{}2\ifmmode\times\else\texttimes\fi{}d$ Bell scenario. Numerical maximization of the violation of this inequality over all states and measurements suggests that the optimal state is far from maximally entangled, while the best measurements are the same as conjectured best measurements for the maximally entangled state. For very large values of ddd the inequality seems to reach its minimal value given by the probability constraints. This gives numerical evidence for a tight quantum Bell inequality (or generalized Csirelson inequality) for the $2\ifmmode\times\else\texttimes\fi{}2\ifmmode\times\else\texttimes\fi{}\ensuremath{\infty}$ scenario.
Entangled photons play a crucial role in quantum applications, and determining and characterising their entanglement is vital to using them effectively. High-dimensional entangled states offer richer possibilities, but their additional measurement degrees of freedom make them increasingly demanding to characterise. However, adaptive Bell-test methods based on complex simultaneous perturbation stochastic approximation (CSPSA) have so far focused mainly on qubits. Here we numerically investigate a Bell-inequality-violation-based method for detecting entanglement in unknown quantum states. We extend CSPSA to high-dimensional Bell testing by using the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality for bipartite qudits. The resulting protocol can detect Bell-nonlocal correlations in unknown entangled states, whether pure or mixed, without first reconstructing their density matrix. Using 100 optimisation iterations in each of 100 independent finite-shot runs per number of dimensions d, we demonstrate certified CGLMP violations throughout d=2-8. For isotropic mixed states tested at a visibility of just 0.05 above the standard-Fourier violation threshold, we likewise observe confidence-certified CGLMP violations throughout the range of d studied. We compare this direct stochastic approach with quantum state tomography, the standard method for characterising an unknown state. In the matched benchmark, CSPSA uses fewer measurement configurations per attempt from d=6, whereas tomography requires fewer detected pairs per certified result through d=8. We also derive the phase dependence of the CGLMP parameter and clarify the features of its landscape that govern the adaptive search. Because the measurement-setting cost of each CSPSA iteration is independent of dimension, the method offers a particularly attractive route to the certification of high-dimensional entanglement.
We introduce a method of investigating qutrit nonclassicality by translating qutrit operators to symmetric two-qubit operators. We show that this procedure sheds light on the discrepancy between maximal qutrit entanglement and maximal nonclassicality of qutrit correlations. Namely, we express Bell operators corresponding to qutrit Bell inequalities in terms of symmetric two-qubit operators and analyze the maximal quantum violation of a given Bell inequality from the qubit perspective. As an example we show that the two-qutrit Collins-Gisin-Linden-Massar-Popescu (CGLMP) Bell inequality can be seen as a combination of Mermin's and Clauser-Horne-Shimony-Holt CHSH) qubit Bell inequalities, and therefore the optimal state violating this combination differs from the one which corresponds to the maximally entangled state of two qutrits. In addition, we discuss the same problem for a three-qutrit inequality. We also demonstrate that the maximal quantum violation of the CGLMP inequality follows from complementarity of correlations.
We compare entanglement with quantum nonlocality employing a geometric structure of the state space of bipartite qudits. Central object is a regular simplex spanned by generalized Bell states. The Collins-Gisin-Linden-Massar-Popescu-Bell inequality is used to reveal states of this set that cannot be described by local-realistic theories. Optimal measurement settings necessary to ascertain nonlocality are determined by means of a recently proposed parameterization of the unitary group U(d) combined with robust numerical methods. The main results of this paper are descriptive geometric illustrations of the state space that emphasize the difference between entanglement and quantum nonlocality. Namely, it is found that the shape of the boundaries of separability and Bell inequality violation are essentially different. Moreover, it is shown that also for mixtures of states sharing the same amount of entanglement, Bell inequality violations and entanglement measures are non-monotonically related.