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Physical Review A

Experimental test of the Collins-Gisin-Linden-Massar-Popescu inequality for multisetting and multidimensional orbital angular momentum systems

Dongkai Zhang, Xiaodong Qiu, Lixiang Chen

Published Jul 1, 2024• 5 citations
Publisher

Abstract

Characterizing high-dimensional entangled states holds pivotal significance in quantum information science and technology. Recent theoretical progress has been made to extend the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality into a general scenario with multisetting and multidimensional systems. Here, by employing two-photon orbital angular momentum entanglement, we conduct an experiment to demonstrate the CGLMP inequality across multiple settings and outcomes. Our experimental results violate the CGLMP inequality by more than 12 standard deviations, demonstrating that the maximum violation increases with both dimension and setting. Furthermore, we reveal, both theoretically and experimentally, the logical connection between the CGLMP inequality and the general Hardy's paradox. Intriguingly, our analysis establishes that, even in high-dimensional systems, Hardy's paradox can be regarded as a special instance of Bell inequality, with their respective bounds aligning under the no-signaling principle and the information causality principle. Our work may advance the foundational understanding of quantum correlations in high-dimensional quantum systems.

DOI
10.1103/physreva.110.012202

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Characterizing high-dimensional entangled states holds pivotal significance in quantum information science and technology. Recent theoretical progress has been made to extend the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality into a general scenario with multisetting and multidimensional systems. Here, by employing two-photon orbital angular momentum entanglement, we conduct an experiment to demonstrate the CGLMP inequality across multiple settings and outcomes. Our experimental results violate the CGLMP inequality by more than 12 standard deviations, demonstrating that the maximum violation increases with both dimension and setting. Furthermore, we reveal, both theoretically and experimentally, the logical connection between the CGLMP inequality and the general Hardy's paradox. Intriguingly, our analysis establishes that, even in high-dimensional systems, Hardy's paradox can be regarded as a special instance of Bell inequality, with their respective bounds aligning under the no-signaling principle and the information causality principle. Our work may advance the foundational understanding of quantum correlations in high-dimensional quantum systems.
Characterizing high-dimensional entangled states is of crucial importance in quantum information science and technology. Recent theoretical progress has been made to extend Hardy's paradox into a general scenario with multisetting and multidimensional systems, which enables the maximum probability of nonlocal events to surpass the bound that was limited in Hardy's original test. Hitherto, no experimental verification has been conducted to verify Hardy's paradox, as most of the previous experimental efforts were restricted to two-dimensional systems. Here, based on two-photon high-dimensional orbital angular momentum (OAM) entanglement, we report an experiment to demonstrate Hardy's paradox for multiple settings and multiple outcomes. We demonstrate the paradox for two-setting higher-dimensional OAM subspaces up to d=7d=7d=7, which reveals that the nonlocal events increase with dimension. Furthermore, we showcase the nonlocality with an experimentally recorded probability of 36.77% for a five-setting three-dimensional OAM subspace via entanglement concentration, thus showing a sharper contradiction between quantum mechanics and classical theory.
High-dimensional quantum entanglement is drawing attention because it enables us to perform quantum information tasks that are robust against noises. To test the nonlocality of entangled qudits, the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality has been proposed and demonstrated using qudits based on orbital angular momentum, time-energy uncertainty, and frequency bins. Here, we report the generation and observation of time-bin entangled ququarts. We implemented a measurement for the CGLMP inequality test using cascaded delay Mach-Zehnder interferometers fabricated by using planar light-wave circuit technology, with which we achieved a precise and stable measurement for time-bin-entangled ququarts. In addition, we generated an optimized entangled state by modulating the pump pulse intensities, with which we can observe the theoretical maximum violation for the CGLMP inequality test. As a result, we successfully observed a Bell-type parameter ${S}_{4}=2.774\ifmmode\pm\else\textpm\fi{}0.025$ violating the CGLMP inequality for the maximally entangled state and an enhanced Bell-type parameter ${S}_{4}=2.913\ifmmode\pm\else\textpm\fi{}0.023$ for the optimized entangled state.
Bell inequality tests based on high-dimensional entanglement usually require measurements that can resolve multiple possible outcomes. However, the implementation of high-dimensional multi-outcome measurements is often only emulated via a collection of ``click or no-click'' measurements. This reduction of multi-outcome measurements to binary-outcome measurements opens a loophole in high-dimensional tests Bell inequalities which can be exploited by local hidden variable models [Tavakoli et al., Phys. Rev. A 111, 042433 (2025)]. Here, we close this loophole by using four-dimensional photonic path-mode entanglement and multi-outcome detection. We test both the well-known Collins-Gisin-Linden-Massar-Popescu inequality and a related Bell inequality tailored for maximally entangled states in high-dimension. We observe violations that are large enough to also rule out any quantum model based on entanglement of lower dimension, thereby demonstrating genuinely high-dimensional nonlocality free of the binarisation loophole.
Recent advancements have expanded Hardy's nonlocality arguments into multisetting and multidimensional systems to enhance quantum correlations. In comparison with Hardy's nonlocality argument, Cabello's nonlocality argument (CNA) emerges as a superior choice for illustrating nonlocal features. An open question persists regarding the potential extension of CNA to arbitrary (k,dk, dk,d) scenarios. Here, we answer this question both in theory and experiment. Theoretically, by utilizing compatibility graphs, we construct a new logical framework for multisetting and multidimensional CNA, demonstrating an increase in the maximum successful probability with setting kkk and dimension ddd. Experimentally, by employing controllable photonic orbital angular momentum entanglement, we exhibit nonlocality with an experimentally recorded probability of 20.29% in the (2, 4) scenario and 28.72% in the (6, 2) scenario. Our work showcases a sharper contradiction between quantum mechanics and classical theory, surpassing the bound limited by the original version.
Recent years have witnessed a rapidly growing interest in high-dimensional quantum entanglement for fundamental studies as well as towards novel applications. Therefore, the ability to verify entanglement between physical qudits, ddd-dimensional quantum systems, is of crucial importance. To show nonclassicality, Hardy's paradox represents ``the best version of Bell's theorem'' without using inequalities. However, so far it has only been tested experimentally for bidimensional vector spaces. Here, we formulate a theoretical framework to demonstrate the ladder proof of Hardy's paradox for arbitrary high-dimensional systems. Furthermore, we experimentally demonstrate the ladder proof by taking advantage of the orbital angular momentum of high-dimensionally entangled photon pairs. We perform the ladder proof of Hardy's paradox for dimensions 3 and 4, both with the ladder up to the third step. Our paper paves the way towards a deeper understanding of the nature of high-dimensionally entangled quantum states and may find applications in quantum information science.
Entangled photons play a crucial role in quantum applications, and determining and characterising their entanglement is vital to using them effectively. High-dimensional entangled states offer richer possibilities, but their additional measurement degrees of freedom make them increasingly demanding to characterise. However, adaptive Bell-test methods based on complex simultaneous perturbation stochastic approximation (CSPSA) have so far focused mainly on qubits. Here we numerically investigate a Bell-inequality-violation-based method for detecting entanglement in unknown quantum states. We extend CSPSA to high-dimensional Bell testing by using the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality for bipartite qudits. The resulting protocol can detect Bell-nonlocal correlations in unknown entangled states, whether pure or mixed, without first reconstructing their density matrix. Using 100 optimisation iterations in each of 100 independent finite-shot runs per number of dimensions d, we demonstrate certified CGLMP violations throughout d=2-8. For isotropic mixed states tested at a visibility of just 0.05 above the standard-Fourier violation threshold, we likewise observe confidence-certified CGLMP violations throughout the range of d studied. We compare this direct stochastic approach with quantum state tomography, the standard method for characterising an unknown state. In the matched benchmark, CSPSA uses fewer measurement configurations per attempt from d=6, whereas tomography requires fewer detected pairs per certified result through d=8. We also derive the phase dependence of the CGLMP parameter and clarify the features of its landscape that govern the adaptive search. Because the measurement-setting cost of each CSPSA iteration is independent of dimension, the method offers a particularly attractive route to the certification of high-dimensional entanglement.