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arXiv:2608.28235

Direct Adaptive Certification of High-Dimensional Entanglement with Bell Tests

Xu Kang Tan, Jesvita Menezes, Sanjan D. Murthy, Adetunmise C. Dada

quant-phSubmitted Aug 28, 2026• Announced Aug 31, 2026• 0 citations
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Abstract

Entangled photons play a crucial role in quantum applications, and determining and characterising their entanglement is vital to using them effectively. High-dimensional entangled states offer richer possibilities, but their additional measurement degrees of freedom make them increasingly demanding to characterise. However, adaptive Bell-test methods based on complex simultaneous perturbation stochastic approximation (CSPSA) have so far focused mainly on qubits. Here we numerically investigate a Bell-inequality-violation-based method for detecting entanglement in unknown quantum states. We extend CSPSA to high-dimensional Bell testing by using the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality for bipartite qudits. The resulting protocol can detect Bell-nonlocal correlations in unknown entangled states, whether pure or mixed, without first reconstructing their density matrix. Using 100 optimisation iterations in each of 100 independent finite-shot runs per number of dimensions d, we demonstrate certified CGLMP violations throughout d=2-8. For isotropic mixed states tested at a visibility of just 0.05 above the standard-Fourier violation threshold, we likewise observe confidence-certified CGLMP violations throughout the range of d studied. We compare this direct stochastic approach with quantum state tomography, the standard method for characterising an unknown state. In the matched benchmark, CSPSA uses fewer measurement configurations per attempt from d=6, whereas tomography requires fewer detected pairs per certified result through d=8. We also derive the phase dependence of the CGLMP parameter and clarify the features of its landscape that govern the adaptive search. Because the measurement-setting cost of each CSPSA iteration is independent of dimension, the method offers a particularly attractive route to the certification of high-dimensional entanglement.

Comments
19 pages, 8 figures, 8 tables. Xu Kang Tan and Jesvita Menezes contributed equally

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Entangled photons play a crucial role in quantum applications, and determining and characterising their entanglement is vital to using them effectively. High-dimensional entangled states offer richer possibilities, but their additional measurement degrees of freedom make them increasingly demanding to characterise. However, adaptive Bell-test methods based on complex simultaneous perturbation stochastic approximation (CSPSA) have so far focused mainly on qubits. Here we numerically investigate a Bell-inequality-violation-based method for detecting entanglement in unknown quantum states. We extend CSPSA to high-dimensional Bell testing by using the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality for bipartite qudits. The resulting protocol can detect Bell-nonlocal correlations in unknown entangled states, whether pure or mixed, without first reconstructing their density matrix. Using 100 optimisation iterations in each of 100 independent finite-shot runs per number of dimensions d, we demonstrate certified CGLMP violations throughout d=2-8. For isotropic mixed states tested at a visibility of just 0.05 above the standard-Fourier violation threshold, we likewise observe confidence-certified CGLMP violations throughout the range of d studied. We compare this direct stochastic approach with quantum state tomography, the standard method for characterising an unknown state. In the matched benchmark, CSPSA uses fewer measurement configurations per attempt from d=6, whereas tomography requires fewer detected pairs per certified result through d=8. We also derive the phase dependence of the CGLMP parameter and clarify the features of its landscape that govern the adaptive search. Because the measurement-setting cost of each CSPSA iteration is independent of dimension, the method offers a particularly attractive route to the certification of high-dimensional entanglement.
Bell inequality tests based on high-dimensional entanglement usually require measurements that can resolve multiple possible outcomes. However, the implementation of high-dimensional multi-outcome measurements is often only emulated via a collection of ``click or no-click'' measurements. This reduction of multi-outcome measurements to binary-outcome measurements opens a loophole in high-dimensional tests Bell inequalities which can be exploited by local hidden variable models [Tavakoli et al., Phys. Rev. A 111, 042433 (2025)]. Here, we close this loophole by using four-dimensional photonic path-mode entanglement and multi-outcome detection. We test both the well-known Collins-Gisin-Linden-Massar-Popescu inequality and a related Bell inequality tailored for maximally entangled states in high-dimension. We observe violations that are large enough to also rule out any quantum model based on entanglement of lower dimension, thereby demonstrating genuinely high-dimensional nonlocality free of the binarisation loophole.
Violation of Bell inequalities is an essential requirement for many quantum information and communication protocols. In high-dimensional systems, Bell inequality tests face the challenge of implementing genuinely multi-outcome measurements, since the emulation of these with separate dichotomic projections opens a binarisation loophole that local hidden variable theories can exploit. Here we show that the joint spectral intensity of a two-photon entangled state contains access to the necessary multi-outcome measurements to overcome this obstacle and certify and violate a Bell inequality for high-dimensional states. This result is contrary to the belief that the joint spectral intensity is a phase-insensitive quantity and does not have sufficient information to certify entanglement or Bell-nonlocality. Using this approach, we violate the CGLMP Bell inequality up to dimension d = 8, all with negligible p-values, and for the first time close the binarisation loophole in high-dimensional Bell experiments. Guaranteeing Bell-nonlocal correlations using frequency-only measurements removes the technological hurdle of measurements in the temporal domain, thus greatly simplifying any practical implementation of future high-dimensional quantum information protocols.
Quantum entanglement is the ability of joint quantum systems to possess global properties (correlation among systems) even when subsystems have no definite individual property. Whilst the 2-dimensional (qubit) case is well-understood, currently, tools to characterise entanglement in high dimensions are limited. We experimentally demonstrate a new procedure for entanglement certification that is suitable for large systems, based entirely on information-theoretics. It scales more efficiently than Bell's inequality and entanglement witness. The method we developed works for arbitrarily large system dimension d and employs only two local measurements of complementary properties. This procedure can also certify whether the system is maximally entangled. We illustrate the protocol for families of bipartite states of qudits with dimension up to 32 composed of polarisation-entangled photon pairs.
Quantum entanglement is the ability of joint quantum systems to possess global properties (correlation among systems) even when subsystems have no definite individual property. Whilst the 2-dimensional (qubit) case is well-understood, currently, tools to characterise entanglement in high dimensions are limited. We experimentally demonstrate a new procedure for entanglement certification that is suitable for large systems, based entirely on information-theoretics. It scales more efficiently than Bell's inequality and entanglement witness. The method we developed works for arbitrarily large system dimension d and employs only two local measurements of complementary properties. This procedure can also certify whether the system is maximally entangled. We illustrate the protocol for families of bipartite states of qudits with dimension up to 32 composed of polarisation-entangled photon pairs.
Bell inequality testing, a well-established method to demonstrate quantum non-locality between remote two-partite entangled systems, is playing an important role in the field of quantum information. The extension to high-dimensional entangled systems, using the so-called Bell-CGLMP inequality, points the way in measuring joint probabilities, the kernel block to construct high dimensional Bell inequalities. Here we show that in theory the joint probability of a two-partite system entangled in a Hilbert space can be measured by choosing a set of basis vectors in its dual space that are related by a Fourier transformation. We next propose an experimental scheme to generate a high-dimensional position-entangled two-photon state aided by a combination of a multiple-slit and a 4 f system, and describe a method to test Bell's inequality using correlated diffraction. Finally, we discuss in detail consequences of such Bell-test violations and experimental requirements.
Bell’s inequality plays an important role in quantum mechanics. Many experiments have been made to test the Bell’s inequality by using various bipartite entangled sources. However, the maximal violation of the Bell inequality (i.e., the Cirel’son’s limit) has not been reached yet, due to various practically-existing imperfections (e.g., entangled source is not the pure maximally-entangled state, and the measurement settings used are not the best ones). In this paper, we investigate experimentally an approach to enhance the violation degree of Bell’s inequality with the commercialized entangled photons by optimizing the measurement settings for the experimentally-reconstructed density matrix of the entangled photons. It is shown that the measurement setting related to the pure entangled state can not get maximally violation generally. However, upon the density matrix reconstructed by tomographic technique, optimal measurement settings can be found. With these optimal settings, we consequently found that the violation degree of the Bell’s inequality can be increased. This suggests a possible approach to optimize the test of Bell’s inequality.