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arXiv:2506.20796

Observing High-dimensional Bell Inequality Violations using Multi-Outcome Spectral Measurements

Kiki Dekkers, Laura Serino, Nicola d'Alessandro, Abhinandan Bhattacharjee, Benjamin Brecht, Armin Tavakoli, Christine Silberhorn, Jonathan Leach

Published Jun 25, 2025• 0 citations
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Abstract

Violation of Bell inequalities is an essential requirement for many quantum information and communication protocols. In high-dimensional systems, Bell inequality tests face the challenge of implementing genuinely multi-outcome measurements, since the emulation of these with separate dichotomic projections opens a binarisation loophole that local hidden variable theories can exploit. Here we show that the joint spectral intensity of a two-photon entangled state contains access to the necessary multi-outcome measurements to overcome this obstacle and certify and violate a Bell inequality for high-dimensional states. This result is contrary to the belief that the joint spectral intensity is a phase-insensitive quantity and does not have sufficient information to certify entanglement or Bell-nonlocality. Using this approach, we violate the CGLMP Bell inequality up to dimension d = 8, all with negligible p-values, and for the first time close the binarisation loophole in high-dimensional Bell experiments. Guaranteeing Bell-nonlocal correlations using frequency-only measurements removes the technological hurdle of measurements in the temporal domain, thus greatly simplifying any practical implementation of future high-dimensional quantum information protocols.

DOI
10.48550/arxiv.2506.20796

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Violation of Bell inequalities is an essential requirement for many quantum information and communication protocols. In high-dimensional systems, Bell inequality tests face the challenge of implementing genuinely multi-outcome measurements, since the emulation of these with separate dichotomic projections opens a binarisation loophole that local hidden variable theories can exploit. Here we show that the joint spectral intensity of a two-photon entangled state contains access to the necessary multi-outcome measurements to overcome this obstacle and certify and violate a Bell inequality for high-dimensional states. This result is contrary to the belief that the joint spectral intensity is a phase-insensitive quantity and does not have sufficient information to certify entanglement or Bell-nonlocality. Using this approach, we violate the CGLMP Bell inequality up to dimension d = 8, all with negligible p-values, and for the first time close the binarisation loophole in high-dimensional Bell experiments. Guaranteeing Bell-nonlocal correlations using frequency-only measurements removes the technological hurdle of measurements in the temporal domain, thus greatly simplifying any practical implementation of future high-dimensional quantum information protocols.
Abstract Violation of Bell inequalities is an essential requirement for many quantum information and communication protocols. In high-dimensional systems, Bell inequality tests face the challenge of implementing genuinely multi-outcome measurements, since the emulation of these with separate dichotomic projections opens a binarisation loophole that local hidden variable theories can exploit. Here we show that the joint spectral intensity of a two-photon entangled state contains access to the necessary multi-outcome measurements to overcome this obstacle and certify nonlocality for high-dimensional states. This result is contrary to the belief that the joint spectral intensity is a phase-insensitive quantity and does not have sufficient information to certify entanglement or nonlocality. Using this approach, we violate the CGLMP Bell inequality up to dimension d = 8, all with negligible p-values, and for the first time close the binarisation loophole in high-dimensional Bell experiments. Guaranteeing nonlocal correlations using frequency-only measurements removes the technological hurdle of measurements in the temporal domain, thus greatly simplifying any practical implementation of future high-dimensional quantum information protocols.
Bell inequality tests based on high-dimensional entanglement usually require measurements that can resolve multiple possible outcomes. However, the implementation of high-dimensional multi-outcome measurements is often only emulated via a collection of ``click or no-click'' measurements. This reduction of multi-outcome measurements to binary-outcome measurements opens a loophole in high-dimensional tests Bell inequalities which can be exploited by local hidden variable models [Tavakoli et al., Phys. Rev. A 111, 042433 (2025)]. Here, we close this loophole by using four-dimensional photonic path-mode entanglement and multi-outcome detection. We test both the well-known Collins-Gisin-Linden-Massar-Popescu inequality and a related Bell inequality tailored for maximally entangled states in high-dimension. We observe violations that are large enough to also rule out any quantum model based on entanglement of lower dimension, thereby demonstrating genuinely high-dimensional nonlocality free of the binarisation loophole.
Bell inequality testing, a well-established method to demonstrate quantum non-locality between remote two-partite entangled systems, is playing an important role in the field of quantum information. The extension to high-dimensional entangled systems, using the so-called Bell-CGLMP inequality, points the way in measuring joint probabilities, the kernel block to construct high dimensional Bell inequalities. Here we show that in theory the joint probability of a two-partite system entangled in a Hilbert space can be measured by choosing a set of basis vectors in its dual space that are related by a Fourier transformation. We next propose an experimental scheme to generate a high-dimensional position-entangled two-photon state aided by a combination of a multiple-slit and a 4 f system, and describe a method to test Bell's inequality using correlated diffraction. Finally, we discuss in detail consequences of such Bell-test violations and experimental requirements.
Many solid-state quantum platforms do not permit sharp, projective measurements but instead yield continuous voltage or field traces under weak, non-demolition readout. In such systems, standard Bell tests based on dichotomic projective measurements are not directly applicable, raising the question of how quantum nonlocality can be certified from continuous time-series data. Here we develop a general theoretical framework showing that Bell-CHSH inequality violation can be extracted from continuous, non-projective measurements without assuming any specific collapse model or phase distribution. We show that sufficiently long continuous measurements of a single entangled pair sample its internal phase-probability structure, enabling effective dichotomic observables to be constructed through phase-sensitive projections and coarse-graining. The resulting Bell correlator is governed by two experimentally accessible resources: intrinsic single-qubit phase spread and nonlocal phase locking between qubits. We benchmark the resulting estimator against conventional projective-measurement CHSH tests implemented via quantum-circuit simulations using Qiskit, finding quantitative agreement in the Bell-violating regime without parameter fitting. Classical deterministic correlations cannot violate the CHSH bound, whereas quantum phase-locked systems recover the nonlinear angular dependence characteristic of entanglement. Our results provide a practical route to demonstrating Bell nonlocality in platforms where measurements are inherently continuous and weak.
Entangled photons play a crucial role in quantum applications, and determining and characterising their entanglement is vital to using them effectively. High-dimensional entangled states offer richer possibilities, but their additional measurement degrees of freedom make them increasingly demanding to characterise. However, adaptive Bell-test methods based on complex simultaneous perturbation stochastic approximation (CSPSA) have so far focused mainly on qubits. Here we numerically investigate a Bell-inequality-violation-based method for detecting entanglement in unknown quantum states. We extend CSPSA to high-dimensional Bell testing by using the Collins-Gisin-Linden-Massar-Popescu (CGLMP) inequality for bipartite qudits. The resulting protocol can detect Bell-nonlocal correlations in unknown entangled states, whether pure or mixed, without first reconstructing their density matrix. Using 100 optimisation iterations in each of 100 independent finite-shot runs per number of dimensions d, we demonstrate certified CGLMP violations throughout d=2-8. For isotropic mixed states tested at a visibility of just 0.05 above the standard-Fourier violation threshold, we likewise observe confidence-certified CGLMP violations throughout the range of d studied. We compare this direct stochastic approach with quantum state tomography, the standard method for characterising an unknown state. In the matched benchmark, CSPSA uses fewer measurement configurations per attempt from d=6, whereas tomography requires fewer detected pairs per certified result through d=8. We also derive the phase dependence of the CGLMP parameter and clarify the features of its landscape that govern the adaptive search. Because the measurement-setting cost of each CSPSA iteration is independent of dimension, the method offers a particularly attractive route to the certification of high-dimensional entanglement.
Entanglement, describing the inseparability of a quantum multiparty system, is one of the most intriguing features of quantum mechanics. Violation of Bell inequality, for ruling out the possibility of local hidden variable theories, is commonly used as a strong witness for quantum entanglement. In previous Bell test experiments with photonic entanglement based on two-photon coincidence measurement, the photon temporal wave packets are absorbed completely by the detectors. That is, the photon coherence time is much shorter than the detection time window. Here we demonstrate generation of frequency-bin entangled narrowband biphotons, and for the first time, test the Clauser-Horne-Shimony-Holt (CHSH) Bell inequality |S|<= 2 for their nonlocal temporal correlations with time-resolved detection. We obtain a maximum |S| value of 2.52+/-0.48 that violates the CHSH inequality. Our result will have applications in quantum information processing involving time-frequency entanglement.