We investigate the nonequilibrium dynamics of a driven-dissipative spin ensemble with competing power-law interactions. We demonstrate that dynamical phase transitions as well as bistabilities can emerge for asymptotic van der Waals interactions, but critically rely on the presence of a slower decaying potential core. Upon introducing random particle motion, we show that a finite gas temperature can drive a phase transition with regards to the spin degree of freedom and eventually leads to mean-field behavior in the high-temperature limit. Our work reconciles contrasting observations of recent experiments with Rydberg atoms in the cold-gas and hot-vapor domain, and introduces an efficient theoretical framework in the latter regime.
We investigate the nonequilibrium dynamics of a driven-dissipative spin ensemble with competing power-law interactions. We demonstrate that dynamical phase transitions as well as bistabilities can emerge for asymptotic van der Waals interactions, but critically rely on the presence of a slower decaying potential core. Upon introducing random particle motion, we show that a finite gas temperature can drive a phase transition with regards to the spin degree of freedom and eventually leads to mean-field behavior in the high-temperature limit. Our work reconciles contrasting observations of recent experiments with Rydberg atoms in the cold-gas and hot-vapor domain, and introduces an efficient theoretical framework in the latter regime.
Understanding and probing phase transitions in nonequilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a nonfluctuating absorbing phase, e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here, we report the observation of signatures of such a nonequilibrium phase transition in an open driven quantum system. In our experiment, rubidium atoms in a quasi-one-dimensional cold disordered gas are laser excited to Rydberg states under so-called facilitation conditions. This conditional excitation process competes with spontaneous decay and leads to a crossover between a stationary state with no excitations and one with a finite number of excitations. We relate the underlying physics to that of an absorbing-state phase transition in the presence of a field (i.e., off-resonant excitation processes) which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of nonequilibrium phase transitions in open many-body quantum systems.
We experimentally and theoretically investigate the nonequilibrium phase structure of a well-controlled driven-dissipative quantum spin system governed by the interplay of coherent driving, spontaneous decay, and long-range spin-spin interactions. We discover that the rate of population loss provides a convenient macroscopic observable that exhibits power-law scaling with the driving strength over several orders of magnitude. The measured scaling exponents reflect the underlying nonequilibrium phase structure of the many-body system, which includes dissipation-dominated, paramagnetic, and critical regimes as well as an instability which drives the system towards states with high excitation density. This opens up a means to study and classify quantum systems out of equilibrium and extends the domain where scale-invariant behavior may be found in nature.
This thesis explores the effects of decoherence and dephasing on single- and many- body dynamics of spin-systems. A particular realisation of the spin systems that the work focuses on are highly excited, Rydberg states of atoms. A software library ARC (Alkali Rydberg Calculator) for calculating properties of Rydberg states in alkali metals is presented, with particular attention to the multi- atom and multi-level effects that influence many-body dynamics in realistic systems, and properties related to terahertz imaging with alkali atom Rydberg states. Dressed-state electromagnetically induced transparency (EIT) is proposed as a way of preparing uniform-phase spin-waves in ladder excitation schemes, making the collective excitation storage insensitive to motional dephasing. Proof of concept dressed state EIT experiments are presented. Strong resonant dressing is also theoretically analysed as a way of preparing velocity superposition of spin-waves. The developed theoretical model is in a good agreement with existing experimental data on single-photon many-atom quantum beats in diamond excitation schemes. By modelling the strongly driven Rydberg ensembles, many-body dynamics of driven-dissipative spin systems is analysed. Working in the limit of strong dephasing, the effects of fluctuations, the shape of interaction potential, spatial correlations and motion on non-equilibrium phase diagrams and the occurrence of bistability are examined. An ensemble averaged mean field model is introduced as an exact solution for completely uncorrelated ensembles. It is shown that the van der Waals interaction does not allow the occurrence of bistability, for which a finite dipolar core is required. The short-range interaction potential shape is found to have a profound influence on non-equilibrium phase diagrams, controlling the size of fluctuations in the dynamics. For a frozen system, several methods for identifying and quantifying bistable phases are introduced, and phase diagrams are reconstructed. It is shown that the temperature of external degrees of freedom, i.e. spin motion, can drive a non-equilibrium transition into the bistable phase.
This thesis presents several experiments investigating the regimes of behaviour of a proto-typical open quantum many-body system far away from equilibrium. The experimental platform is based on ultracold atoms laser-excited to Rydberg states, which we engineer to emulate a strongly interacting, driven-dissipative quantum spin system. The high degree of control over the relevant microscopic processes and their parameters, as well as the ability to widely tune interaction and driving strengths provides the means to address fundamental questions on how different regimes of dynamical behaviour emerge in complex open quantum systems and how they can be characterised. \n \nIn the first part, we discuss how control over the relevant properties of Rydberg spin systems, like temperature, density, long evolution times, strong interactions, tunable driving, and dissipation can be achieved. We introduce the new experimental apparatus developed during this thesis, which combines both single-photon and two-photon Rydberg excitation schemes with high atom densities and long excitation times using an optical dipole trap. Additionally, we investigate theoretically how long coherence times exceeding motional timescales combined with strong many-body interactions can be achieved in such a system. We identify an optimal parameter regime for two-photon excitation where such conditions can be generated with coherence times and interaction strengths comparable to what is achievable for single-photon excitation. \n \nIn the second part we explore the macroscopic non-equilibrium behaviour of our system and devise suitable observables for characterising different regimes of behaviour. We discover that the slow atom loss inherent to our system provides a convenient observable for the many-body state of the system. Focussing on evolution times where the effect of the atom loss on the evolution is small, we discover that the rate of atom loss exhibits powerlaw scaling with the driving strength over several orders of magnitude. The measured scaling exponents reveal the non-equilibrium phase structure of the many-body system and allow us to distinguish dissipation-dominated, paramagnetic and critical regimes, as well as an instability. In the observed critical regime, collectively enhanced driving dominates over dissipation, leading to scaling associated to the critical point of the non-dissipative equilibrium Rydberg spin system. Based on the known microscopic processes of our system, we perform classical many-body rate equation simulations, which agree well with the observed phase structure as well as the position and associated scaling exponents of the individual regimes. These findings open up new means to study and classify out of equilibrium systems based on slow particle loss and powerlaw scaling. \n \nIn the last part of this thesis we reveal a second type of criticality in our system, which is genuinely non-equilibrium in character and arises from an absorbing state phase transition. The critical state of this phase transition dominates the system evolution at late times where particle loss is no longer negligible. We identify self-organisation as the mechanism driving the system to this critical state, which we observe through powerlaw scaling of the non-equilibrium steady-state. These experiments establish Rydberg atoms as a well controlled platform for implementing and exploring models of absorbing state phase transitions and self-organised criticality with unprecedented access to the underlying microscopic properties of the system.
We study the nonequilibrium many-body dynamics of a cold gas of ground-state alkali-metal atoms weakly admixed by Rydberg states with laser light. On a time scale shorter than the lifetime of the dressed states, effective dipole-dipole or van der Waals interactions between atoms can lead to the formation of strongly correlated phases, such as atomic crystals. Using a semiclassical approach, we study the long-time dynamics where decoherence and dissipative processes due to spontaneous emission and blackbody radiation dominate, leading to heating and melting of atomic crystals as well as particle losses. These effects can be substantially mitigated by performing active laser cooling in the presence of atomic dressing.
Dark states are stationary states of a dissipative, Lindblad-type time evolution with zero von Neumann entropy, therefore representing examples of pure steady states. Nonequilibrium dynamics featuring a dark state recently gained a lot of attraction since their implementation in the context of driven-open quantum systems represents a viable possibility to engineer unique, pure states. Inspired by recent experimental progress with ultracold Rydberg ensembles, we analyze a driven many-body spin system, which displays a mean-field bistability between a dark steady state and a mixed steady state. As a function of the driving strength one observes a discontinuous phase transition that connects the zero entropy (dark) state with a finite entropy (mixed) state. The transition is characterized by a jump of the von Neumann entropy from zero to a finite value, which is of genuine nonequilibrium character. We analyze the relevant long wavelength fluctuations driving this transition by means of the renormalization group. This allows us to approach the nonequilibrium dark-state transition and identify similarities and clear differences to common, equilibrium phase transitions, to establish the phenomenology for a first-order dark-state phase transition, and to relate it to the dynamics in driven dissipative Rydberg ensembles.