Understanding the doped Mott insulator is a central challenge in condensed matter physics. In this work, we first explicitly identify a new sign structure in the $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model on the square lattice that replaces the conventional Fermi statistics for weakly interacting electrons. Then we show that the singular, i.e., the phase-string part of the sign structure in the partition function can be precisely turned off in a modified model. The density matrix renormalization group method is then employed to study these two models comparatively on finite-size systems, which is designed to unveil the consequences of the phase-string component. We find that the hole pairing is present not only in the quasi-long-range superconducting phase but also in the stripe phase of the $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model. However, once the phase-string is switched off, both the superconducting and stripe orders together with the underlying hole pairing disappear. The corresponding ground state reduces to a trivial Fermi-liquid-like state with small hole Fermi pockets that is decoupled from the antiferromagnetic spin background. It is in sharp contrast to the original $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model where large Fermi surfaces can be restored in the stripe phase found at ${t}^{\ensuremath{'}}/t<0$ or the superconducting phase at ${t}^{\ensuremath{'}}/t>0$ in the six-leg ladder calculation. Our study clearly demonstrates that the strong correlation effect in doped Mott insulator should be mainly attributed to the long-range quantum entanglement between the spin and charge, which is, nonperturbatively, beyond a simple spin-charge separation under the no double occupancy constraint.
We study a ground-state ansatz for the single-hole-doped $t\text{\ensuremath{-}}J$ model in two dimensions via a variational Monte Carlo method. Such a single-hole wave function possesses finite angular momenta generated by hidden spin currents, which give rise to a novel ground-state degeneracy in agreement with recent exact diagonalization (ED) and density matrix renormalization group (DMRG) results. We further show that the wave function can be decomposed into a quasiparticle component and an incoherent momentum distribution in excellent agreement with the DMRG results up to an $8\ifmmode\times\else\texttimes\fi{}8$ lattice. Such a two-component structure indicates the breakdown of Landau's one-to-one correspondence principle, and in particular, the quasiparticle spectral weight vanishes by a power law in the large sample size limit. By contrast, turning off the phase string induced by the hole hopping in the so-called $\ensuremath{\sigma}\ifmmode\cdot\else\textperiodcentered\fi{}t\text{\ensuremath{-}}J$ model, a conventional Bloch-wave wave function with a finite quasiparticle spectral weight can be recovered, also in agreement with the ED and DMRG results. The present study shows that a singular effect already takes place in the single-hole-doped Mott insulator, by which the bare hole is turned into a non-Landau quasiparticle with translational-symmetry breaking. Generalizations to pairing and finite doping are briefly discussed.
For the
t-
J model, variational wave functions can generally be constructed based on an accurate description of antiferromagnetism (AFM) at half-filling and an exact phase-string sign structure under doping. The single-hole-doped and two-hole-doped states, as determined by variational Monte Carlo (VMC) simulations, display sharply contrasting behaviors. The single-hole state constitutes a ``cat state'' that resonates strongly between a quasiparticle component and a local loop-current component, with approximately equal weights. In the ground state, the quasiparticle spectral weight
Zk peaks at momenta
k0≡(±2π,±2π). The total-energy dispersion versus
k agrees remarkably well with the Green function Monte Carlo results. However, Landau's one-to-one correspondence hypothesis for quasiparticles breaks down here with the incoherent component exhibiting intrinsic magnetization originating from a minimal
2×2 loop current that forms a
4×4 pattern on the square lattice--a finding in excellent agreement with density matrix renormalization group (DMRG) calculations. In the two-hole ground state, a new pairing mechanism is revealed: the two holes are automatically fused into a tightly bound object consisting of an incoherent
dxy pairing along the diagonal direction by compensating the local loop currents. This hole pair is again a ``cat state'' that resonates strongly between the incoherent
dxy and a coherent
dx2−y2 Cooper channel to gain substantial hopping energy. Its size extends over an area of about
4×4 lattice spacings, much smaller than the divergent AFM correlation length, implying that it should survive as a minimal superconducting building block even in the dilute doping regime. Experimental implications and the generalization to the finite-doping case are briefly addressed.
The mechanism of superconductivity in a purely interacting electron system has been one of the most challenging issues in condensed matter physics. In the BCS theory, the Landau's Fermi liquid is the ground state of weakly interacting fermions dictated by the fermion sign structure, and the superconducting instability only occurs when an additional pairing force is added. By contrast, as shown by density matrix renormalization group calculation, a quasi-one-dimensional superconducting state (specifically a Luther-Emery state) is an intrinsic ground state of the $t\ensuremath{-}J$ two-leg ladder and four-leg cylinder at finite doping. Such a Luther-Emery state with pairing can be directly turned into a Fermi-gas-like normal state without pairing by merely switching off the phase-string signs hidden in the model via two schemes, which reduce the sign structure to the trivial fermion signs associated with doped holes. It thus demonstrates a new pairing paradigm in a model-doped Mott insulator as due to the generic phase-string sign structure. Finally, as an example, the latter is explicitly shown to lead to a ``stringlike'' pairing force after adiabatically connecting to a strong anisotropic limit of the model.
Cooper pairing instability in a Fermi liquid is well understood by the BCS theory, but pairing mechanism for doped Mott insulators still remains elusive. Previously it has been shown by density matrix renormalization group (DMRG) method that a single doped hole is always self-localized due to the quantum destructive interference of the phase string signs hidden in the t-J ladders. Here we report a DMRG investigation of hole binding in the same model, where a novel pairing-glue scheme beyond the BCS realm is discovered. Specifically, we show that, in addition to spin pairing due to superexchange interaction, the strong frustration of the phase string signs on the kinetic energy gets effectively removed by pairing the charges, which results in strong binding of two holes. By contrast, if the phase string signs are "switched off" artificially, the pairing strength diminishes significantly even if the superexchange coupling remains the same. In the latter, unpaired holes behave like coherent quasiparticles with pairing drastically weakened, whose sole origin may be attributed to the resonating-valence-bond (RVB) pairing of spins. Such non-BCS pairing mechanism is therefore beyond the RVB picture and may shed important light on the high-T(c) cuprate superconductors.
We reexamine the problem of a hole moving in an antiferromagnetic spin background and find that the injected hole will always pick up a sequence of nontrivial phases from the spin degrees of freedom. Previously unnoticed, such a stringlike phase originates from the hidden Marshall signs which are scrambled by the hopping of the hole. We can rigorously show that this phase string is nonrepairable at low energy and give a general proof that the spectral weight Z must vanish at the ground-state energy due to the phase-string effect. Thus, the quasiparticle description fails here and the quantum interference effect of the phase string dramatically affects the long-distance behavior of the injected hole. We introduce a so-called phase-string formulation of the t-J model for a general number of holes in which the phase-string effect can be explicitly tracked. As an example, by applying this new mathematical formulation in one dimension, we reproduce the well-known Luttinger-liquid behaviors of the asymptotic single-electron Green's function and the spin-spin correlation function. We can also use the present phase-string theory to justify previously developed spin-charge separation theory in two dimensions, which offers a systematic explanation for the transport and magnetic anomalies in the high-
Tc cuprates.