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arXiv:1508.03741 · Physical Review A

Strongly driven nonlinear quantum optics in microring resonators

Z. Vernon, John E. Sipe

Published Sep 22, 2015• 57 citations
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Abstract

We present a detailed analysis of strongly driven spontaneous four-wave mixing in a lossy integrated microring resonator side coupled to a channel waveguide. A nonperturbative, analytic solution within the undepleted pump approximation is developed for a cw pump input of arbitrary intensity. In the strongly driven regime self- and cross-phase modulation, as well as multipair generation, lead to a rich variety of power-dependent effects; the results are markedly different than in the low-power limit. The photon-pair generation rate, single-photon spectrum, and joint spectral intensity (JSI) distribution are calculated. Splitting of the generated single-photon spectrum into a doublet structure associated with both pump detuning and cross-phase modulation is predicted, as well as substantial narrowing of the generated signal and idler bandwidths associated with the onset of optical parametric oscillation at intermediate powers. Both the correlated and the uncorrelated contributions to the JSI are calculated, and for sufficient powers the uncorrelated part of the JSI is found to form a quadruplet structure. The pump detuning is found to play a crucial role in all of these phenomena, and a critical detuning is identified which divides the system behavior into distinct regimes, as well as an optimal detuning strategy which preserves many of the low-power characteristics of the generated photons for arbitrary input power.

DOI
10.1103/physreva.92.033840

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We present a detailed analysis of strongly driven spontaneous four-wave mixing in a lossy integrated microring resonator side coupled to a channel waveguide. A nonperturbative, analytic solution within the undepleted pump approximation is developed for a cw pump input of arbitrary intensity. In the strongly driven regime self- and cross-phase modulation, as well as multipair generation, lead to a rich variety of power-dependent effects; the results are markedly different than in the low-power limit. The photon-pair generation rate, single-photon spectrum, and joint spectral intensity (JSI) distribution are calculated. Splitting of the generated single-photon spectrum into a doublet structure associated with both pump detuning and cross-phase modulation is predicted, as well as substantial narrowing of the generated signal and idler bandwidths associated with the onset of optical parametric oscillation at intermediate powers. Both the correlated and the uncorrelated contributions to the JSI are calculated, and for sufficient powers the uncorrelated part of the JSI is found to form a quadruplet structure. The pump detuning is found to play a crucial role in all of these phenomena, and a critical detuning is identified which divides the system behavior into distinct regimes, as well as an optimal detuning strategy which preserves many of the low-power characteristics of the generated photons for arbitrary input power.
We develop a general Hamiltonian treatment of spontaneous four-wave mixing in a microring resonator side-coupled to a channel waveguide. The effect of scattering losses in the ring is included, as well as parasitic nonlinear effects including self- and cross-phase modulation. A procedure for computing the output of such a system for arbitrary parameters and pump states is presented. For the limit of weak pumping an expression for the joint spectral intensity of generated photon pairs, as well as the singles-to-coincidences ratio, is derived.
In this thesis I study in detail the quantum dynamics of several nonlinear optical processes in microresonator systems. A Heisenberg-picture input-output formalism is developed from first principles that includes the effects of scattering losses and independent quality factors and coupling ratios for different resonances. The task of calculating the device output is then reduced to solving a set of driven, damped, ordinary differential equations for the resonator mode operators alone. This theoretical framework is used to study photon pair generation via spontaneous four-wave mixing in the weakly pumped regime, on which the effects of scattering losses are appraised. A more strongly driven regime is studied for continuous wave pumps, demonstrating when self- and cross-phase modulation and multi-photon pair generation become important, and their effects on the spectral and power scaling properties of the system are examined; A detuning strategy is presented that compensates for some of these effects. The results of the weak-pump regime are applied to study microresonator-based her- alded single photon sources. The impact of scattering losses is studied, revealing that typical systems suffer from low heralding efficiency due to these losses. A technique to improve heralding efficiency is presented through over-coupling the resonator-channel system, and a resultant trade-off between heralding rate and heralding efficiency is un- covered. Limitations to the spectral purity of the heralded single photon output for conventional microresonator systems are also analysed, and a more sophisticated cou- pling scheme presented to overcome the upper bound for spectral purity of 93% that exists in typical systems, permitting the generation of single photons with spectral pu- rity arbitrarily close to 100% without spectral filtering or sophisticated phase-matching techniques. The theory of quantum frequency conversion in microresonators using four-wave mix- ing is then developed in detail, and the spectral conversion probability and conversion efficiency studied. Efficiencies exceeding 90% using less than 100 mW of pump power are predicted to be achievable with current technology. A dressed mode picture is developed to better understand the conversion dynamics. Rabi-like spectral splitting and temporal oscillations of the intraresonator mean photon number are predicted, exhibiting a novel regime of strongly coupled photonic modes.
In this work, we present a quantum theory for pulsed photon pair generation in a single ring resonator. Our approach combines the Heisenberg picture input-output formalism with the Ikeda mapping from classical nonlinear optics. In doing so, we address the high-gain regime by incorporating nonperturbative effects, including self-phase modulation, cross-phase modulation, and time-ordering, which are roots for significantly different behaviors in the low-gain regime. We also account for optical losses by introducing an auxiliary waveguide, allowing for a more accurate representation of experimentally viable scenarios. Numerical simulations reveal that nonperturbative effects significantly distort transfer functions, making desirable operations challenging without careful optimization. We show that appropriate detuning of the pump frequency can mitigate these issues, leading to enhanced brightness and higher spectral purity in the high-gain regime. We further investigate the performance of a single ring resonator as a two-mode squeezer by analyzing various performance metrics under experimentally relevant optical loss conditions.
This thesis presents an analysis of photon pairs generated via either spontaneous parametric downconversion or spontaneous four-wave mixing in channel waveguides as well as in microring resonators side-coupled to channel waveguides. The state of photons exiting a particular device is calculated within a general Hamiltonian formalism that simplifies the link between quantum nonlinear optics experiments and classical nonlinear optics experiments. This state contains information regarding photon pair production efficiency as well as modal and spectral correlations between the two photons, characterized by a two-dimensional spectral distribution function called the biphoton wave function.\n\nIn the limit of a low probability of pair production, photon pair production fficiencies are cast into forms resembling corresponding well-known classical nonlinear optical frequency conversion efficiencies, making it easy to see what plays the role of a classical “seed” field in an un-seeded (quantum) process. This also allows photon pair production efficiencies to be calculated based on the results of classical nonlinear optical experiments. It is further calculated that, unless enerated photons are collected over a very narrow frequency range, their generation efficiency does not scale the same way with device length in a channel waveguide, or resonance quality factor in a microring resonator, as might be expected from the corresponding classical frequency conversion efficiency. Although calculations do not include self- or cross-phase modulation, nor two-photon absorption\nor free-carrier absorption, it is calculated that their neglect is justified in the low pair production probability limit. Linear (scattering) loss is also neglected, though partially addressed in the final chapter of this thesis.\n\nBiphoton wave functions are calculated explicitly, such that their shape and orientation, including approximate analytic expressions for their widths, can easily be determined. This further allows estimation of the suitability of their associated photon pairs for various quantum information processing applications. As an alternative to dispersion engineering a channel waveguide photon pair source, it is calculated that microring resonators can very naturally produce nearly spectrally uncorrelated photon pairs, which behave very much like idealized single-mode photons and are thus useful for applications involving the interference of photons from multiple sources.
We present a self-contained analytical model for biphoton generation in microring resonators. Encompassing both all-pass and add-drop geometries, identical and distinct pump and biphoton coupling coefficients, and continuous-wave and pulsed pumping, our interaction-picture-based approach reveals time-frequency biphoton correlations while also predicting absolute generation rates. Under continuous-wave excitation, we find critical coupling of both the pump and biphoton to maximize the rate of single photons extracted from the microring, whereas critical coupling of the pump but overcoupling of the biphoton maximize the two-photon rate. Under pulsed pumping, overcoupling of both pump and biphoton (to different degrees) maximizes photon extraction probabilities, albeit under a tradeoff with spectral factorability that we quantify via parameter scans over a range of coupler pairings. As a whole, our formalism should prove valuable for the practical design of integrated photon sources, merging a flexible and intuitive biphoton-centric depiction with quantitative predictions closely tied to experimental parameters.
We propose an integrated device, the resonant interferometric coupler, enabling selective control over the coupling condition of a microring resonator. This can be used to tune the resonance linewidths independently, allowing for the targeted engineering of nonlinear optical interactions. We show how this can be applied to spontaneous four-wave mixing for various purposes. In the low-gain regime, we demonstrate the generation of spectrally uncorrelated photon pairs by broadening the pump resonance relative to the signal and idler. In the high-gain regime, we show how parasitic nonlinear processes can be suppressed by inhibiting undesired resonances, leading to a more efficient generation of squeezed light.